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We recently introduced an efficient methodology to perform density-corrected Hartree-Fock density functional theory (DC(HF)-DFT) calculations and an extension to it we called "corrected" HF DFT (C(HF)-DFT). In this work, we take a further…

化学物理 · 物理学 2023-11-10 Daniel Graf , Alex J. W. Thom

The Random Phase Approximation (RPA) and its variations and extensions are, without any doubt, the most widely used tools to describe Giant Resonances within a microscopic theory. In this chapter, we will start by discussing how RPA comes…

核理论 · 物理学 2022-01-13 Gianluca Colo'

The Hartree-Fock-RPA approach is applied to the 1D anti-ferromagnetic Heisenberg model in the Jordan-Wigner representation. Somewhat contrary to expectation, this leads to reasonable results for spectral functions and sum rules in the…

强关联电子 · 物理学 2009-11-11 A. Rabhi , P. Schuck , J. Da Providencia

The Hartree-Fock approximation to the many-fermion problem can break exact symmetries, and in some cases by changing a parameter in the interaction one can drive the Hartree-Fock minimum from a symmetry-breaking state to a…

核理论 · 物理学 2009-09-11 Calvin W. Johnson , Ionel Stetcu

Mixing single and triple fermions an exact killing operator of the Coupled Cluster Doubles (CCD) wave function with good symmetry was found in \cite{Tohy13}. Using these operators with the equation of motion (EOM) method the so-called…

核理论 · 物理学 2020-10-26 Mohsen Jemaï , Peter Schuck

In this work, we consider the particle-hole random phase approximation (phRPA), an approximation to the correlation energy in electronic structure, and show that the phRPA energy of the H2 molecule correctly dissociates. That is, as the…

偏微分方程分析 · 数学 2022-10-11 Mi-Song Dupuy , Kyle Thicke

A limitation common to all extensions of random-phase approximation including only particle-hole configurations is that they violate to some extent the energy weighted sum rules. Considering one such extension, the improved RPA (IRPA),…

核理论 · 物理学 2009-11-07 M. Grasso , F. Catara

A new Quasiparticle Random Phase Approximation approach is presented. The corresponding ground state is variationally determined and exhibits a minimum energy. New solutions for the ground state, some with spontaneously broken symmetry, of…

核理论 · 物理学 2008-11-26 F. Simkovic , M. Smotlak , A. A. Raduta

We present a comparative study of particle-hole and particle-particle channels of random-phase approximation (RPA) for molecular dissociations of different bonding types. We introduced a \textit{direct} particle-particle RPA scheme, in…

材料科学 · 物理学 2019-06-05 Muhammad N. Tahir , Xinguo Ren

The ground-state correlation energy calculated in the random-phase approximation (RPA) is known to be identical to that calculated using a subset of terms appearing in coupled-cluster theory with double excitations. In particular, this…

化学物理 · 物理学 2019-04-16 Timothy C. Berkelbach

The random phase approximation (RPA) as formulated as an orbital-dependent, fifth-rung functional within the density functional theory (DFT) framework offers a promising approach for calculating the ground-state energies and the derived…

计算物理 · 物理学 2023-07-25 Rong Shi , Peize Lin , Min-Ye Zhang , Lixin He , Xinguo Ren

We present an extension of the random--phase approximation (RPA) where the RPA phonons are used as building blocks to construct the excited states. In our model, that we call double RPA (DRPA), we include up to two RPA phonons. This is an…

核理论 · 物理学 2016-02-17 D. Gambacurta , F. Catara , M. Grasso , M. Sambataro , M. V. Andrés , E. G. Lanza

A characteristic feature of collective and particle-hole excitations in neutron-rich nuclei is that many of them couple to unbound neutron in continuum single-particle orbits. The continuum random phase approximation (cRPA) is a powerful…

核理论 · 物理学 2021-09-15 Teruyuki Saito , Masayuki Matsuo

The random phase approximation (RPA) to the correlation energy is extended to fractional occupations and its performance examined for exact conditions on fractional charges and fractional spins. RPA satisfies the constancy condition for…

其他凝聚态物理 · 物理学 2009-03-26 Paula Mori-Sánchez , Aron J. Cohen , Weitao Yang

The random phase approximation (RPA) has received a considerable interest in the field of modeling systems where noncovalent interactions are important. Its advantages over widely used density functional theory (DFT) approximations are the…

化学物理 · 物理学 2019-12-04 Marcin Modrzejewski , Sirous Yourdkhani , Jiri Klimes

We present an analytic proof demonstrating the equivalence between the Random Phase Approximation (RPA) to the ground state correlation energy and a ring-diagram simplification of the Coupled Cluster Doubles (CCD) equations. In the CCD…

其他凝聚态物理 · 物理学 2009-11-13 Gustavo E. Scuseria , Thomas M. Henderson , Danny C. Sorensen

We explore different variants of the random phase approximation (RPA) to the correlation energy derived from closed-shell ring-diagram approximations to coupled cluster doubles theory. We implement these variants in range-separated…

化学物理 · 物理学 2011-09-01 Julien Toulouse , Wuming Zhu , Andreas Savin , Georg Jansen , János G. Angyán

Relativistic Continuum Random Phase Approximation (CRPA) is used to investigate collective excitation phenomena in several spherical nuclei along the periodic table. We start from relativistic mean field calculations based on a covariant…

核理论 · 物理学 2011-03-21 J. Daoutidis , P. Ring

A computer code for quasiparticle random phase approximation-QRPA and projected quasiparticle random phase approximation-PQRPA models of nuclear structure is explained in details. An important application of the code consists in evaluating…

核理论 · 物理学 2010-04-22 F. Krmpotic , A. R. Samana , C. A. Bertulani

In this thesis are shown developments in the random phase approximation (RPA) in the context of range-separated theories. We present advances in the formalism of the RPA in general, and particularly in the "dielectric matrix" formulation of…

化学物理 · 物理学 2015-11-24 B. Mussard