相关论文: Paramagnetic NMR chemical shift in a spin state su…
We present a theory for the temperature-dependent nuclear magnetic shielding tensor of molecules with arbitrary electronic structure. The theory is a generalization of Ramsey's theory for closed-shell molecules. The shielding tensor is…
We present a theory of nuclear magnetic resonance (NMR) shielding tensors for electronic states with arbitrary degeneracy. The shieldings are here expressed in terms of generalized Zeeman ($g^{(k)}$) and hyperfine ($A^{(k)}$) tensors, of…
We present a simple derivation of the nuclear shielding in paramagnetic molecules, extendable to strong spin-orbit coupling cases of relevance to lanthanides and actinides, as well as encompassing contributions from excited multiplets.…
Recently, Yu, Brown, and Chuang [Phys. Rev. A {\bf 71}, 032341 (2005)] investigated the entanglement attainable from unitary transformed thermal states in liquid-state nuclear magnetic resonance (NMR). Their research gave an insight into…
In this paper we use the Nuclear Magnetic Resonance (NMR) to write eletronic states of a ferromagnetic system into a high-temperature paramagnetic nuclear spins. Through the control of phase and duration of radiofrequency pulses we set the…
In high spin molecules metal ions are coupled by ferro or antiferromagnetic short range interactions so that their magnetic moments are parallel or antiparallel to each other at temperatures (T) much smaller than the coupling constant J.…
The magnetic state of the single-component molecular compound, [Cu(tmdt)$_{2}$], is investigated by means of $^{1}$H-NMR. An abrupt spectral broadening below 13 K and a sharp peak in nuclear spin-lattice relaxation rate, $T_{1}^{-1}$, at 13…
We study theoretically the formation of the nuclear-spin polaron state in semiconductor nanosystems within the Lindblad equation approach. To this end, we derive a general Lindblad equation for the density operator that complies with the…
As a nuclear spin model of scalable quantum register, the one-dimensional chain of the magnetic atoms with nuclear spins 1/2 substituting the basic atoms in the plate of nuclear spin free easy-axis 3D antiferromagnet is considered. It is…
We present theoretical studies of temperature dependent diamagnetic-paramagnetic transitions in thin quantum rings. Our studies show that the magnetic susceptibility of metal/semiconductor rings can exhibit multiple sign flips at…
We use recent developments in the framework of time dependent matrix product state method (t-MPS) to compute the NMR relaxation rate $1/T_1$ for spin-1/2 chains under magnetic field and for different Hamiltonians (XXX, XXZ, isotropically…
We present the general theory of clean, two-dimensional, quantum Heisenberg antiferromagnets which are close to the zero-temperature quantum transition between ground states with and without long-range N\'{e}el order. For N\'{e}el-ordered…
Nuclear Magnetic Resonance (NMR) is a powerful local quantum probe of the electronic structure of materials, but in the absence of reliable theory the interpretation of the NMR data can be challenging. This is true in particular for the…
The NMR relaxation rate and the static spin susceptibility in graphene are studied within a tight-binding description. At half filling, the NMR relaxation rate follows a power law as $T^2$ on the particle-hole symmetric side, while with a…
We demonstrate ionization of a molecule with the bias voltage of a Scanning Tunnelling Microscope (STM) resulting in a coexistence of a neutral and ionic molecules, i.e. radical (paramagnetic) and non-radical (diamagnetic) states. This…
We solve the $S=1/2$ infinite-range random Heisenberg Hamiltonian in the paramagnetic phase using quantum Monte Carlo and analytical techniques. We find that the spin-glass susceptibility diverges at a finite temperature $T_g$ which…
$^{75}$As NMR measurements were performed on a polycrystalline sample of spin-1/2 alternating-spin-chain Heisenberg antiferromagnet AgVOAsO$_4$. Temperature-dependent NMR shift $K(T)$, which is a direct measure of the intrinsic spin…
This paper studies spin glass to paramagnetic transition in the Spherical Sherrington-Kirkpatrick model with ferromagnetic Curie-Weiss interaction with coupling constant $J$ and inverse temperature $\beta$. The disorder of the system is…
Here we demonstrate how para-hydrogen can be used to prepare a two-spin system in an almost pure state which is suitable for implementing nuclear magnetic resonance (NMR) quantum computation. A 12ns laser pulse is used to initiate a…
Very recently, there has been significant progress with establishing a common phenomenology of the superconducting cuprates in terms of nuclear magnetic resonance (NMR) shift and relaxation. Different from the old interpretation, it was…