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We present a quantitative confocal-microscopy study of the transient and final microstructure of particle-stabilised emulsions formed via demixing in a binary liquid. To this end, we have developed an image-analysis method that relies on…

软凝聚态物质 · 物理学 2010-11-04 Job H J Thijssen , Paul S Clegg

Helium nanodroplets ("HNDs") are widely used for forming tailor-made clusters and molecular complexes in a cold, transparent, and weakly-interacting matrix. Characterization of embedded species by mass spectrometry is often complicated by…

原子与分子团簇 · 物理学 2024-01-15 S. De , A. R. Abid , J. D. Asmussen , L. Ben Ltaief , K. Sishodia , A. Ulmer , H. B. Pedersen , S. R. Krishnan , M. Mudrich

We present results of molecular dynamics simulations of the electron system on the surface of liquid helium. The simulations are done for 1600 electrons with periodic boundary conditions. Electron scattering by capillary waves and phonons…

介观与纳米尺度物理 · 物理学 2018-09-03 K. Moskovtsev amd M. I. Dykman

Femtosecond pump-probe spectroscopy has been used to study vibrational dynamics of potassium dimers attached to superfluid helium nanodroplets. Comparing the measured data with theoretical results based on dissipative quantum dynamics we…

原子与分子团簇 · 物理学 2009-09-28 Martin Schlesinger , Marcel Mudrich , Frank Stienkemeier , Walter T. Strunz

Using numerical simulations, we investigate the gravitational evolution of filamentary molecular cloud structures and their condensation into dense protostellar cores. One possible process is the so called 'edge effect', the pile-up of…

星系天体物理 · 物理学 2023-04-06 Elena Hoemann , Stefan Heigl , Andreas Burkert

We investigate electrostatic stability of charged droplets, modeled as permeable, charged spheres, and their encapsidation in thin, arbitrarily charged nano-shells, immersed in a neutralizing asymmetric electrolyte background. The latter…

软凝聚态物质 · 物理学 2013-11-15 Leili Javidpour , Anže Lošdorfer Božič , Ali Naji , Rudolf Podgornik

We present a simple quantum mechanical model describing excited rotational states of molecules in superfluid helium nanodroplets, as recently studied in non-adiabatic molecular alignment experiments [Cherepanov et al., Phys. Rev. A 104,…

Atomic collapse is a phenomenon inherent to relativistic quantum mechanics where electron states dive in the positron continuum for highly charged nuclei. This phenomenon was recently observed in graphene. Here we investigate a novel…

介观与纳米尺度物理 · 物理学 2019-09-04 Robbe Van Pottelberge , Dean Moldovan , S. P. Milovanovic , Francois M. Peeters

We have produced a Bose-Einstein condensate of metastable helium (4He*) containing over 1.5x10^7 atoms, which is a factor of 25 higher than previously achieved. The improved starting conditions for evaporative cooling are obtained by…

其他凝聚态物理 · 物理学 2007-05-23 A. S. Tychkov , T. Jeltes , J. M. McNamara , P. J. J. Tol , N. Herschbach , W. Hogervorst , W. Vassen

We report on the Bose-Einstein condensation of metastable Helium-4 atoms using a hybrid approach, consisting of a magnetic quadrupole and a crossed optical dipole trap. In our setup we cross the phase transition with 2x10^6 atoms, and we…

量子气体 · 物理学 2015-06-23 Q. Bouton , R. Chang , A. L. Hoendervanger , F. Nogrette , A. Aspect , C. I. Westbrook , D. Clément

Ionization is a fundamental process in intense laser-matter interactions, and is known to cause plasma defocusing and intensity clamping. Here, we investigate theoretically the propagation dynamics of an intense laser pulse in a helium gas…

光学 · 物理学 2020-11-25 Xiaohui Gao , Bonggu Shim

The observation of chemical reactions on the time scale of the motion of electrons and nuclei has been made possible by lasers with ever shortened pulse lengths. Superfluid helium represents a special solvent that permits the synthesis of…

Spectroscopic data on alkali-atom dimers residing on the surface of liquid helium nanodroplets have revealed that they are detected primarily in the weakly bound, metastable, spin-triplet state. Here, by measuring the magnetic Stern-Gerlach…

原子与分子团簇 · 物理学 2025-05-16 Thomas H. Villers , Benjamin S. Kamerin , Vitaly V. Kresin

While photodissociation of molecular systems has been extensively studied, the photoinduced formation of chemical bonds remains largely unexplored. Especially for larger aggregates, the electronic and nuclear dynamics involved in the…

化学物理 · 物理学 2024-12-03 Michael Stadlhofer , Bernhard Thaler , Pascal Heim , Josef Tiggesbäumker , Markus Koch

Coherent topologically close-packed nanoplates in magnesium alloys can effectively improve strength and creep resistance.However, the formation mechanisms of several metastable TCP nanoplates remain unclear, and the traditional…

材料科学 · 物理学 2025-04-03 Junyuan Bai , Xueyong Pang , Gaowu Qin

Single-shot coherent diffractive imaging (CDI) with intense short-wavelength light pulses enables the structural characterization of individual nanoparticles in free flight with high spatial and temporal resolution. Conventional CDI assumes…

Two-component nanoplasmas generated by strong-field ionization of doped helium nanodroplets are studied in a pump-probe experiment using few-cycle laser pulses in combination with molecular dynamics simulations. High yields of helium ions…

This article provides a review of recent work in the field of helium nanodroplet spectroscopy with emphasis on the dynamical aspects of the interactions between molecules in helium as well as their interaction with this unique quantum…

化学物理 · 物理学 2009-11-11 Frank Stienkemeier , Kevin K Lehmann

Metal-fullerene compounds are characterized by significant electron transfer to the fullerene cage, giving rise to an electric dipole moment. We use the method of electrostatic beam deflection to verify whether such reactions take place…

Mixed $^3$He-$^4$He droplets created by hydrodynamic instability of a cryogenic fluid-jet may acquire angular momentum during their passage through the nozzle of the experimental apparatus. These free-standing droplets cool down to very low…

量子气体 · 物理学 2020-08-12 Marti Pi , Francesco Ancilotto , Jose' Maria Escartin , Ricardo Mayol , Manuel Barranco