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The endohedral fullerene Er3N@C80 shows characteristic 1.5 micron photoluminescence at cryogenic temperatures associated with radiative relaxation from the crystal-field split Er3+ 4I13/2 manifold to the 4I15/2 manifold. Previous…

We report data on the luminescence spectra associated with photochromic centers in X-ray irradiated calcium fluoride crystals doped with Lu ions. Irradiation in low energy photochromic centers absorption band excites emission, which can be…

材料科学 · 物理学 2015-12-31 Roman Shendrik , Alexandra Myasnikova , Tatiana Sizova , Evgeny Radzhabov

In atomically thin semiconductors based on transition metal dichalcogenides, photoexcitation can be used to generate high densities of electron-hole pairs. Due to optical nonlinearities, which originate from Pauli blocking and many-body…

介观与纳米尺度物理 · 物理学 2020-12-15 Daniel Erben , Alexander Steinhoff , Michael Lorke , Frank Jahnke

Light-sheet microscopy (LSM) is a powerful imaging technique that uses a planar illumination oriented orthogonally to the detection axis. Two-photon (2P) LSM is a variant of LSM that exploits the 2P absorption effect for sample excitation.…

We study an integrated silicon photonic chip, composed of several sub-wavelength ridge waveguides, and immersed in a micro-cell with rubidium vapor. Employing two-photon excitation, including a telecom wavelength, we observe that the…

Ultrashort long-wave infrared (LWIR) laser pulses can resonantly excite vibrations in N2 and O2 through a two-photon transition. The absorptive, vibrational component of the ultrafast optical nonlinearity grows in time, starting smaller…

We demonstrate a two-photon transition of rubidium (Rb) atoms from the ground state (5$S_{1/2}$) to the excited state (4$D_{5/2}$), using a home-built ytterbium (Yb)-doped fiber amplifier at 1033 nm. This is the first demonstration of an…

原子物理 · 物理学 2017-04-06 Ritayan Roy , Paul C. Condylis , Yik Jinen Johnathan , Björn Hessmo

BaMnF$_4$ microsheets have been prepared by hydrothermal method. Strong room-temperature blue-violet photoluminescence has been observed (absolute luminescence quantum yield 67%), with two peaks located at 385 nm and 410 nm, respectively.…

材料科学 · 物理学 2016-01-20 Shuang Zhou , Yakui Weng , Zhangting Wu , Jinlong Wang , Lingzhi Wu , Zhenhua Ni , Qingyu Xu , Shuai Dong

The parity-allowed two-photon transitions between the ground state 3A2(T2) of the configuration 3d8 in cubical symmetry and the excited states of the same configuration are obtained via a simple model. This model is developed in a symmetry…

原子与分子团簇 · 物理学 2009-10-31 J. Sztucki , M. Daoud , M. Kibler

We describe numerically the ionization process induced by linearly and circularly polarized XUV attosecond laser pulses on an aligned atomic target, specifically, the excited state…

原子物理 · 物理学 2021-05-26 Juan J. Omiste , Lars Bojer Madsen

The first continuous-wave two-photon absorption laser-induced stimulated emission (CTALISE) is demonstrated. The 7^1S-6^1P transition in mercury at 1014nm wavelength is used and selective lasing of different isotopes is observed.

光学 · 物理学 2015-03-17 Daniel Kolbe , Martin Scheid , Andreas Koglbauer , Jochen Walz

We investigate the excitation of the 5D_{5/2} level in Rb atoms using counter-propagating laser beams, which are nearly resonant to the one-photon 5S_{1/2} - 5P_{3/2} and 5P_{3/2} - 5D_{5/2} transitions, ensuring that a sum of the optical…

原子物理 · 物理学 2015-05-28 A. M. Akulshin , B. V. Hall , V. Ivannikov , A. A. Orel , A. I. Sidorov

The $^{229}$Th nucleus has a long-lived isomeric state $A^*$ at 8.338(24) eV [Kraemer et al, Nature, \textbf{617}, 706 (2023)]. This state is connected to the ground state by an M1 transition. For a hydrogenlike Th ion in the $1s$ state the…

In this paper we investigate the coherence properties of a quantum dot under two-photon resonant excitation in combination with an additional photo-neutralization laser. The photo-neutralization increases the efficiency of the excitation…

量子物理 · 物理学 2016-09-21 Tobias Huber , Ana Predojević , Glenn S. Solomon , Gregor Weihs

We report coherent enhancement of two-photon emission from the excited vibrational state of molecular hydrogen triggered by irradiating mid-infrared pulses externally. We previously observed the two-photon emission triggered by the…

Angular distribution of photoelectrons released by the ionization of randomly-oriented molecules with two laser fields of carrier frequencies $\omega$ and $2\omega$, which are linearly polarized in two mutually-orthogonal directions, is…

量子物理 · 物理学 2019-06-11 Philipp V. Demekhin

Ultrafast light-matter interaction has emerged as a powerful tool to control and probe the macroscopic properties of functional materials, especially two-dimensional transition metal dichalcogenides which can form different structural…

介观与纳米尺度物理 · 物理学 2023-10-10 XinYu Zhou , H Wang , Q M Liu , S J Zhang , S X Xu , Q Wu , R S Li , L Yue , T C Hu , J Y Yuan , S S Han , T Dong , D Wu , N L Wang

The 8 eV first nuclear excited state in $^{229}$Th is a candidate for implementing an nuclear clock. Doping $^{229}$Th into ionic crystals such as CaF$_2$ is expected to suppress non-radiative decay, enabling nuclear spectroscopy and the…

We present studies of resonance-enhanced photo-ionization for isotope-selective loading of Ca+ into a Paul trap. The 4s^2 ^1S_0 <-> 4s4p ^1P_1 transition of neutral calcium is driven by a 423nm laser and the atoms are photo-ionized by a…

Despite inherently complex multiphoton dynamics, our observations show that Ba double ionization with an infrared laser (8800-8920 cm^{-1}) resembles a single-photon process; namely, its probability is proportional to the laser intensity.…

原子物理 · 物理学 2013-08-13 I. I. Bondar , V. V. Suran , D. I. Bondar