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We introduce a new, highly sensitive, and simple heterodyne optical method for imaging individual non-fluorescent nano-objects. A two orders of magnitude improvement of the signal is achieved compared to previous methods. This allows for…

其他凝聚态物理 · 物理学 2007-05-23 Stephane Berciaud , Laurent Cognet , Gerhard Blab , Brahim Lounis

We introduce a new, highly sensitive, and simple heterodyne optical method for imaging individual nonfluorescent nanoclusters and nanocrystals. A 2 order of magnitude improvement of the signal is achieved compared to previous methods. This…

光学 · 物理学 2007-05-23 Stéphane Berciaud , Laurent Cognet , Gerhard A Blab , Brahim Lounis

Photothermal microscopy has recently complemented single molecule fluorescence microscopy by the detection of individual nano-objects in absorption. Photothermal techniques gain their superior sensitivity by exploiting a heat induced…

光学 · 物理学 2015-05-28 Markus Selmke , Marco Braun , Frank Cichos

We present the theoretical and detailed experimental characterizations of Photothermal Heterodyne Imaging. An analytical expression of the photothermal heterodyne signal is derived using the theory of light scattering from a fluctuating…

In nanomechanical photothermal absorption spectroscopy and microscopy, the measured substance becomes a part of the detection system itself, inducing a nanomechanical resonance frequency shift upon thermal relaxation. Suspended,…

仪器与探测器 · 物理学 2023-06-30 Robert G. West , Kostas Kanellopulos , Silvan Schmid

Photothermal heterodyne detection is used to record the first room-temperature absorption spectra of single CdSe/ZnS semiconductor nanocrystals. These spectra are recorded in the high cw excitation regime, and the observed bands are…

光学 · 物理学 2007-05-23 Stéphane Berciaud , Laurent Cognet , Brahim Lounis

Photothermal therapies are based on the optical excitation of plasmonic nanoparticles in the biological environment. The effects of the irradiation on the biological medium depend critically on the heat transfer process at the nanoparticle…

计算物理 · 物理学 2017-11-21 Andrea Torchi , Federica Simonelli , Riccardo Ferrando , Giulia Rossi

Single-molecule microscopy has become an indispensable tool for biochemical analysis. The capability of characterizing distinct properties of individual molecules without averaging has provided us with a different perspective for the…

应用物理 · 物理学 2020-05-21 Miao-Hsuan Chien , Silvan Schmid

We propose a new approach to understand the time-dependent temperature increasing process of gold-silica core-shell nanoparticles injected into chicken tissues under near-infrared laser irradiation. Gold nanoshells strongly absorb…

介观与纳米尺度物理 · 物理学 2018-04-04 Vu T. T. Duong , Anh D. Phan , Nghiem T. H. Lien , Do T. Hue , Do Q. Hoa , Do T. Nga , Tran H. Nhung , Nguyen A. Viet

Advances in integrated photonics open exciting opportunities for batch-fabricated optical sensors using high quality factor nanophotonic cavities to achieve ultra-high sensitivities and bandwidths. The sensitivity improves with higher…

光学 · 物理学 2021-07-09 Mingkang Wang , Diego J. Perez-Morelo , Vladimir Aksyuk

Integrated photodetectors are crucial for their high speed, sensitivity, and efficient power consumption. In these devices, photocurrent generation is primarily attributed to the photovoltaic (PV) effect, driven by electron hole…

Absorption microscopy is a powerful technique, enabling the detection of single non- fluorescent molecules at room temperature. So far, the molecular absorption has been probed optically via the attenuation of a probing laser. The…

应用物理 · 物理学 2018-11-21 Miao-Hsuan Chien , Mario Brameshuber , Gerhard J. Schütz , Silvan Schmid

The action of a nanoscopic spherically symmetric refractive index profile on a focused Gaussian beam may easily be envisaged as the action of a phase-modifying element, i.e. a lens: Rays traversing the inhomogeneous refractive index field…

光学 · 物理学 2011-09-14 Selmke Markus , Braun Marco , Cichos Frank

Label-free detection techniques for single particles and molecules play an important role in basic science, disease diagnostics, and nanomaterial investigations. While traditional fluorescence-based methods offer powerful tools for single…

光学 · 物理学 2024-08-20 Shuang Hao , Sartanee Suebka , Judith Su

Currently available temperature measurements or imaging at nano-micro scale are limited to fluorescent molecules and luminescent nanocrystals, whose spectral properties respond to temperature variation. The principle of operation of these…

Understanding light-matter interaction at the nanoscale requires probing the optical properties of matter at the individual nano-absorber level. To this end, we have developed a nanomechanical photothermal sensing platform that can be used…

光学 · 物理学 2024-06-07 Kostas Kanellopulos , Robert G. West , Silvan Schmid

With increasing interest in utilizing nanostructures as nanoscale heat sources, the ability to precisely measure photothermal effects at the nanoscale has become increasingly significant. Techniques based on fluorescence or Raman signals…

光学 · 物理学 2025-06-10 Seongmin Im , Wei Hong , Gayatri Chandran , Xing Wang , Yang Zhao

Thermal transport in nanostructures plays a critical role in modern technologies. As devices shrink, techniques that can measure thermal properties at nanometer and nanosecond scales are increasingly needed to capture transient,…

The selective optical detection of individual metallic nanoparticles (NPs) with high spatial and temporal resolution is a challenging endeavour, yet is key to the understanding of their optical response and their exploitation in…

介观与纳米尺度物理 · 物理学 2012-06-05 Francesco Masia , Wolfgang Langbein , Paola Borri

Imaging of the optical properties of individual nanosystems beyond fluorescence can provide a wealth of information. However, the minute signals for absorption and dispersion are challenging to observe, and only specialized techniques…

光学 · 物理学 2015-09-10 Matthias Mader , Jakob Reichel , Theodor W. Hänsch , David Hunger
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