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We perform extensive monomer-resolved computer simulations of suitably-designed amphiphilic dendritic macromolecules over a broad range of densities, proving the existence and stability of cluster crystals formed in these systems, as…

软凝聚态物质 · 物理学 2013-05-06 Dominic A. Lenz , Ronald Blaak , Christos N. Likos , Bianca M. Mladek

Formation of highly ordered structures usually needs to overcome a high free-energy barrier that is greatly beyond the ability of thermodynamic fluctuation, such that the system would be easily trapped into a state with many defects and the…

材料科学 · 物理学 2020-01-08 Yunfei Du , Huijun Jiang , Zhonghuai Hou

Advances in nanotechnology lead to an increasing interest in how nanoparticles interact with biomembranes. Nanoparticles are wrapped spontaneously by biomembranes if the adhesive interactions between the particles and membranes compensate…

亚细胞过程 · 定量生物学 2016-09-16 Michael Raatz , Thomas R. Weikl

A versatile system to construct polymeric phononic crystals by using ultrasound is described. In order to fabricate this material a customised cavity device fitted with a 2 MHz acoustic transducer and an acoustic reflector is employed for…

应用物理 · 物理学 2018-02-01 Nan Li , Christopher R. Lowe , Adrian C. Stevenson

External control of the swimming speed of `active particles' can be used to self assemble designer structures in situ on the micrometer to millimeter scale. We demonstrate such reconfigurable templated active self assembly in a fluid…

软凝聚态物质 · 物理学 2018-02-23 Jochen Arlt , Vincent A Martinez , Angela Dawson , Teuta Pilizota , Wilson C K Poon

We study the self-assembly behaviour of patchy particles with `protein-like' interactions that can be considered as a minimal model for the assembly of viral capsids and other shell-like protein complexes. We thoroughly explore the…

软凝聚态物质 · 物理学 2010-01-21 Alex W. Wilber , Jonathan P. K. Doye , Ard A. Louis , Anna C. F. Lewis

Spontaneous self-assembly in molecular systems is a fundamental route to both biological and engineered soft matter. Simple micellisation, emulsion formation, and polymer mixing principles are well understood. However, the principles behind…

软凝聚态物质 · 物理学 2021-09-21 Alberto Scacchi , Sousa Javan Nikkhah , Maria Sammalkorpi , Tapio Ala-Nissila

The self-assembly of submerged cold-plasma-treated polyethylene beads is reported. The plasma-treated immersed millimetrically-sized polyethylene beads formed well-ordered 2D quasi-crystalline structures. The submerged floating of light…

We investigate the phase behavior of symmetric AB diblock copolymers confined into a thin film. The film boundaries are parallel, impenetrable and attract the A component of the diblock copolymer. Using a self-consistent field technique…

统计力学 · 物理学 2009-10-31 Thorsten Geisinger , Marcus Mueller , Kurt Binder

The ordering of nanoparticles into predetermined configurations is of importance to the design of advanced technologies. In this work, we moderate the surface anchoring against the bulk elasticity of liquid crystals to dynamically shape…

软凝聚态物质 · 物理学 2023-12-01 Lisa Tran , Hye-Na Kim , Ningwei Li , Shu Yang , Kathleen J. Stebe , Randall D. Kamien , Martin F. Haase

The structure of a polystyrene matrix filled with tightly cross-linked polystyrene nanoparticles, forming an athermal nanocomposite system, is investigated by means of a Monte Carlo sampling formalism. The polymer chains are represented as…

软凝聚态物质 · 物理学 2014-01-17 Georgios G. Vogiatzis , Evangelos Voyiatzis , Doros N. Theodorou

The shape of the building blocks plays a crucial role in directing self-assembly towards desired architectures. Out of the many different shapes, helix has a unique position. Helical structures are ubiquitous in nature and a helical shape…

软凝聚态物质 · 物理学 2016-04-27 Hima Bindu Kolli , Giorgio Cinacchi , Alberta Ferrarini , Achille Giacometti

Nanoparticles tethered with DNA strands are promising building blocks for bottom-up nanotechnology, and a theoretical understanding is important for future development. Here we build on approaches developed in polymer physics to provide…

软凝聚态物质 · 物理学 2014-11-03 Chia Wei Hsu , Francesco Sciortino , Francis W. Starr

Polymers with both soluble and insoluble blocks typically self-assemble into micelles, aggregates of a finite number of polymers where the soluble blocks shield the insoluble ones from contact with the solvent. Upon increasing…

软凝聚态物质 · 物理学 2009-11-13 J. A. Anderson , C. D. Lorenz , A. Travesset

Au nanoparticles with near perfect monodispersity in shape and size self-assemble, very slowly and at room temperature, on polystyrene films for film thickness < 4R_{g}$, R_{g} being unperturbed polymer gyration radius. Nanoparticle shape…

材料科学 · 物理学 2007-05-23 Sudeshna Chattopadhyay , Alokmay Datta

In recent years, experimental and theoretical investigations have shown that anisotropic colloids can self-organise into ordered porous monolayers, where the interplay of localised bonding sites, so called patches, with the particle's shape…

软凝聚态物质 · 物理学 2024-05-03 Carina Karner , Emanuela Bianchi

We analyze diffusion of small particles in a solid polymeric medium taking into account a short range particle-polymer interaction. The system is modeled by a particle diffusion on a ternary lattice where the sites occupied by polymer…

统计力学 · 物理学 2015-06-11 Federico Camboni , Andreas Koher , Igor M. Sokolov

From understanding the sand on the beach to the foam on your beer, soft sphere simulations have been crucial to the study of the amorphous world around us. However, many of the materials we interact with on a daily basis aren't comprised of…

软凝聚态物质 · 物理学 2024-03-18 R. C. Dennis

We report many different nano-structures which are formed when model nano-particles of different sizes (diameter {\sigma} n ) are allowed to aggregate in a background matrix of semi-flexible self assembled polymeric worm like micellar…

软凝聚态物质 · 物理学 2015-06-23 Shaikh Mubeena , Apratim Chatterji

We investigate by scattering techniques the structure of water-based soft composite materials comprising a crystal made of Pluronic block-copolymer micelles arranged in a face-centered cubic lattice and a small amount (at most 2% by volume)…

软凝聚态物质 · 物理学 2012-06-07 Elisa Tamborini , Neda Ghofraniha , Julian Oberdisse , Luca Cipelletti , Laurence Ramos