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PrV$_2$Al$_{20}$ is a rare example of a heavy fermion system based on strong hybridization between conduction electrons and nonmagnetic quadrupolar moments of the cubic $\Gamma_3$ ground doublet. Here, we report that a high-quality single…

强关联电子 · 物理学 2015-06-22 Masaki Tsujimoto , Yosuke Matsumoto , Takahiro Tomita , Akito Sakai , Satoru Nakatsuji

Our single crystal study reveals that PrTr2Al20 (Tr = Ti and V) provides the first examples of a cubic {\Gamma}3 nonmagnetic ground doublet system that shows the Kondo effect including a -ln T dependent resistivity. The {\Gamma}3…

强关联电子 · 物理学 2015-03-19 Akito Sakai , Satoru Nakatsuji

Heavy fermion metals hosting multipolar local moments set a new stage for exploring exotic spin-orbital entangled quantum phases. In such systems, the quadrupolar Kondo effect serves as the key ingredient in the orbital-driven non-Fermi…

强关联电子 · 物理学 2020-01-14 Mingxuan Fu , Akito Sakai , Naoki Sogabe , Masaki Tsujimoto , Yosuke Matsumoto , Satoru Nakatsuji

Origin of the non-magnetic phase transition in PrTi$_2$Al$_{20}$, reported earlier in the macroscopic study, has been asserted microscopically using elastic and inelastic neutron scattering techniques. It has been shown spectroscopically…

强关联电子 · 物理学 2013-05-03 Taku J Sato , Soshi Ibuka , Yusuke Nambu , Teruo Yamazaki , Akito Sakai , Satoru Nakatsuji

Orbital degrees of freedom in condensed matters could play important roles in forming a variety of exotic electronic states by interacting with conduction electrons. In 4f electron systems, because of strong intra-atomic spin-orbit…

PrV2Al20 is the heavy fermion superconductor based on the cubic Gamma3 doublet that exhibits non- magnetic quadrupolar ordering below ~ 0.6 K. Our magnetotransport study on PrV2Al20 reveals field-induced quadrupolar quantum criticality at…

强关联电子 · 物理学 2016-10-31 Yasuyuki Shimura , Masaki Tsujimoto , Bin Zeng , Luis Balicas , Akito Sakai , Satoru Nakatsuji

Superconductivity is observed in the filled skutterudite compound \PrOsSb{} below a critical temperature temperature $T_\mathrm{c} = 1.85$ K and appears to develop out of a nonmagnetic heavy Fermi liquid with an effective mass $m^{*}…

Multipolar Kondo systems offer unprecedented opportunities for designing astonishing quantum phases and functionalities beyond spin-only descriptions. A model material platform of this kind is the cubic heavy-fermion system…

Superconducting and antiferroquadrupolar (AFQ) transitions in a Pr-based compound PrRh2Zn20 have been found to occur simultaneously at Tc=TQ=0.06 K. The superconducting transition manifests itself by zero resistance and large diamagnetic…

Among heavy fermion materials, there is a set of rare-earth intermetallics with non-Kramers Pr$^{3+}$ $4f^2$ moments which exhibit a rich phase diagram with intertwined quadrupolar orders, superconductivity, and non-Fermi liquid behavior.…

强关联电子 · 物理学 2018-03-08 Frederic Freyer , Jan Attig , SungBin Lee , Arun Paramekanti , Simon Trebst , Yong Baek Kim

Electrical resistivity, magnetic susceptibility, and specific heat measurements on single crystals of La$Tr_{2}$Al$_{20}$ ($Tr$ = Ti, V, Nb, and Ta) revealed that these four compounds exhibit weak-coupling superconductivity with transition…

超导电性 · 物理学 2018-02-22 Akira Yamada , Ryuji Higashinaka , Tatsuma D. Matsuda , Yuji Aoki

CeRh2As2 has recently been reported to be a rare case of multi-phase unconventional superconductor [S. Khim et al., arXiv:2101.09522] close to a quantum critical point (QCP). Here, we present a comprehensive study of its normal state…

Multipolar moments entail a new route to tackle frontier problems in superconductivity (SC). A key progress in the search for multipolar SC is the discovery of Pr$Tr_2$Al$_{20}$ ($Tr =$ Ti, V), which possesses quadrupolar and octupolar but…

We have measured the specific heat of PrV$_2$Al$_{20}$ at very low temperatures, using high quality single crystals with the residual resistivity ratio ~ 20. The high-quality single crystals exhibit clear double transitions at $T_{\rm Q} =$…

强关联电子 · 物理学 2015-06-23 Masaki Tsujimoto , Yosuke Matsumoto , Satoru Nakatsuji

Superconductivity in PrIr$_{2}$Zn$_{20}$ appears at $T_{\rm c} = 0.05$ K in the presence of an antiferroquadrupolar order below $T_{\rm Q} = 0.11$ K. We have studied pressure dependences of $T_{\rm c}$, $T_{\rm Q}$, and non-Fermi liquid…

To examine the thermodynamic properties of Pr$_{2}$Ba$_{4}$Cu$_{7}$O$_{15-\delta }$ compounds with metallic CuO double chains, we measured the specific heats of superconducting and non-superconducting polycrystalline samples at low…

超导电性 · 物理学 2016-03-23 Takahisa Konno , Michiaki Matsukawa , Keisuke Sugawara , Haruka Taniguchi

In this study, ultrasonic measurements were performed on a single crystal of cubic PrNi$_2$Cd$_{20}$, down to a temperature of 0.02 K, to investigate the crystalline electric field ground state and search for possible phase transitions at…

The filled skutterudite compound \PrOsSb{} exhibits superconductivity below a critical temperature $T_\mathrm{c} = 1.85$ K that develops out of a nonmagnetic heavy Fermi liquid with an effective mass $m^{*} \approx 50 m_\mathrm{e}$, where…

超导电性 · 物理学 2007-05-23 M. B. Maple , P. -C. Ho , N. A. Frederick , V. S. Zapf , W. M. Yuhasz , E. D. Bauer

Superconductivity is observed with critical temperature $T_{c}$ = 2.0 K in self-flux-grown single crystals of $CaBi_{2}$. This material adopts the $ZrSi_{2}$ structure type with lattice parameters a = 4.696(1) $\AA$, b = 7.081(2) $\AA$ and…

The two-channel Anderson lattice model which has $SU(2)\otimes SU(2)$ symmetry is of relevance to understanding of the magnetic, quadrupolar and superconducting phases in U$_{1-x}$Th$_x$Be$_{13}$ or Pr base skutterudite compounds such as…

超导电性 · 物理学 2007-05-23 Frithjof B Anders
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