相关论文: A new type of light with enhanced optical chiralit…
Plasmonic chirality exhibits great potential for novel nanooptical devices due to the generation of a strong chiroptical response. Previous reports on plasmonic chirality explanations are mainly based on phase retardation and coupling. We…
Structured x-rays carrying an orbital angular momentum break spatial inversion symmetry and have been proposed as a means to probe chirality. We theoretically investigate twisted non-resonant x-ray diffraction from chiral molecules and…
In this study, we apply the monitoring master equation describing decoherence of internal states to an optically active molecule prepared in a coherent superposition of nondegenerate internal states interacting with thermal photons at low…
We demonstrate that rotationally symmetric chiral metasurfaces can support arbitrarily sharp resonances with the maximum optical chirality determined by precise shaping of bound states in the continuum (BICs). Being uncoupled from one…
We demonstrate that electric-dipole scatterers can mimic chiral light-matter interaction by generating far-field circular polarization upon scattering, even though the optical chirality of the incident field as well as that of the scattered…
Topology, a well-established concept in mathematics, has nowadays become essential to describe condensed matter. At its core are chiral electron states on the bulk, surfaces and edges of the condensed matter systems, in which spin and…
Optically active achiral metasurfaces offer a promising way to detect chiral molecules based on chiroptic methods. The combination of plasmonic enhanced circular dichroism and reversible optical activity would boost the sensitivity and…
We explore experimentally if the light's orbital angular momentum (OAM) interacts with chiral nematic polymer films. Specifically, we measure the circular dichroism of such a material using light beams with different OAM. We investigate the…
In the present work we theoretically analyze electroluminescence occurring in a biased single-molecule junction with a chiral bridge imitated by a helical chain. We show that optical transitions between electron states of the chiral linker…
We demonstrate that higher order Poincare modes of order m are super-chiral, displaying enhancement factors proportional to $m$ and $m^2$ in their helicity/chirality. With m having arbitrarily large integer values, such modes, in principle,…
Artificial nanostructures enable fine control of electromagnetic fields at the nanoscale, a possibility that has recently been extended to the interaction between polarised light and chiral matter. The theoretical description of such…
We introduce a definition of the electromagnetic chirality of an object and show that it has an upper bound. Reciprocal objects attain the upper bound if and only if they are transparent for all the fields of one polarization handedness…
Chiral excited electronic states of molecules have an intrinsic sense of handedness, or twist, and are the active component in energy efficient display technologies and in new photosynthetic routes to produce pharmaceuticals. Creating…
Light scattering from chiral plasmonic structures can create near fields with an asymmetry greater than the equivalent circularly polarised light, a property sometimes referred to as superchirality. These near fields with enhanced chiral…
Circular dichroism, arising from interactions with light fields of opposite spin angular momentum, has become a fundamental tool for molecular characterization. Meanwhile, helical dichroism (HD) - the dichroic response to vortex beams…
We implement a paraxial azimuthally-radially polarized beam (ARPB), a novel class of structured light beams that can be optimal chiral (OC), leading to maximum chirality density at a given energy density. By using vectorial light shaping…
Optical chirality plays an essential role in chiral light-matter interactions with broad applications in sensing and spectroscopy. Conventional methods of generating optical chirality usually employ chiral structures or chiral excitations.…
Chirality is a pervasive form of symmetry that is intimately connected to the physical properties of solids, as well as the chemical and biological activity of molecular systems. However, its control with light is challenging, because…
This paper presents a first-principle and global perspective of electromagnetic chirality. It follows for this purpose a bottom-up construction, from the description of chiral particles or metaparticles (microscopic scale), through the…
Chirality-driven optical properties in charge density waves are of fundamental and practical importance. Here, we investigate the interaction between circularly polarized light and emergent chiral stacking orders in quasi-one-dimensional…