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A recent theory of magnetoresistance in positionally disordered organic semiconductors is extended to include exchange and dipolar couplings between polarons. Analytic results are discovered when the hyperfine, exchange, and dipolar…

无序系统与神经网络 · 物理学 2012-06-25 N. J. Harmon , M. E. Flatté

We explore the possibility that hyperfine interaction causes the recently discovered organic magnetoresistance (OMAR) effect. Our study employs both experiment and theoretical modelling. An excitonic pair mechanism model based on hyperfine…

软凝聚态物质 · 物理学 2016-08-16 Y. Sheng , D. T. Nguyen , G. Veeraraghavan , Ö. Mermer , M. Wohlgenannt , U. Scherf

We derive the kinetic equations for polaron hopping in organics that explicitly take into account the double occupation possibility and pair intersite correlations. The equations include simplified phenomenological spin dynamics and provide…

无序系统与神经网络 · 物理学 2018-04-04 A. V. Shumilin , V. V. Kabanov , V. I. Dediu

Magnetic nanoparticles (MNPs) exhibiting superparamagnetic properties might generate large magnetic dipole-dipole interaction with electron spins in organic semiconductors (OSECs). This concept could be considered analogous to the effect of…

The effect of a magnetic field on the electroluminescence of organic light emitting devices originates from the hyperfine interaction between the electron/hole polarons and the hydrogen nuclei of the host molecules. In this paper, we…

A universal mechanism for strong magnetic-field effects of nonmagnetic organic semiconductors is presented. A weak magnetic field (less than hundreds mT) can substantially change the charge carrier hopping coefficient between two…

介观与纳米尺度物理 · 物理学 2015-05-14 X. R. Wang , S. J. Xie

We derive kinetic equations describing injection and transport of spin polarized carriers in organic semiconductors with hopping conductivity via an impurity level. The model predicts a strongly voltage dependent magnetoresistance, defined…

介观与纳米尺度物理 · 物理学 2015-02-06 A. V. Shumilin , V. V. Kabanov , V. A. Dediu

A small magnetic field (~30 mT) can effectively modulate the electroluminescence, conductance and/or photocurrent of organic semiconductor based devices, up to 10% at room temperature. This organic magnetic field effect (OMFE) is one of the…

材料科学 · 物理学 2010-03-25 B. K. Li , H. T. He , W. J. Chen , M. K. Lam , K. W. Cheah , J. N. Wang

The magneto-electronic field effects in organic semiconductors at high magnetic fields are described by field-dependent mixing between singlet and triplet states of weakly bound charge carrier pairs due to small differences in their Land\'e…

介观与纳米尺度物理 · 物理学 2018-08-15 G. Joshi , M. Y. Teferi , S. Jamali , M. Groesbeck , J. van Tol , R. McLaughlin , Z. V. Vardeny , J. M. Lupton , H. Malissa , C. Boehme

The controllability of charge transport through an organic molecular spin-valve system is theoretically investigated on the basis of a Su-Schrieffer-Heeger model combined with the non-equilibrium Green's function formalism. We show how the…

材料科学 · 物理学 2007-05-23 J. H. Wei , S. J. Xie , L. M. Mei , YiJing Yan

It is shown that in organic semiconductors where organic magnetoresistance (OMAR) is observed, the exchange interaction between electrons and holes localized at different molecules leads to dynamic spin polarization in the direction of the…

无序系统与神经网络 · 物理学 2022-04-06 A. V. Shumilin

A universal mechanism for strong magnetic-field effects of nonmagnetic organic semiconductors is presented. A weak magnetic field (less than hundreds mT) can substantially change the charge carrier hopping coefficient between two…

介观与纳米尺度物理 · 物理学 2010-06-29 X. R. Wang , S. J. Xie

Based on the spin-blockade model for organic magnetoresistance we present an analytic expression for the polaron-bipolaron transition rate, taking into account the effective nuclear fields on the sites. We reveal the physics producing…

介观与纳米尺度物理 · 物理学 2015-06-15 Jeroen Danon , Xuhui Wang , Aurélien Manchon

The origin of magnetoresistance is bipolar organic materials is the influence of magnetic field on the dynamics of recombination within localized electron-hole pairs. Recombination from the $S$ spin-state of the pair in preceded by the…

无序系统与神经网络 · 物理学 2023-06-14 M. E. Raikh

Organic Magnetoresistance is defined as the change of resistance in an organic material, such as a conducting polymer, as a function of an imposed magnetic field. We demonstrate this effect in a Polypyrrole/ Polydimethylsiloxane complex by…

软凝聚态物质 · 物理学 2025-12-29 Paul Ben Ishai , Roshlin Kiruba , Amos Bardea

We develop a theory of magnetoresistance based on variable-range hopping. An exponentially large, low-field and necessarily positive magnetoresistance effect is predicted in the presence of Hubbard interaction and spin-dynamics under…

软凝聚态物质 · 物理学 2007-05-23 M. Wohlgenannt

A novel magnetoresistance effect, due to the injection of a spin-polarized electron current from a dilute magnetic into a non-magnetic semiconductor, is presented. The effect results from the suppression of a spin channel in the…

介观与纳米尺度物理 · 物理学 2009-11-07 G. Schmidt , G. Richter , P. Grabs , C. Gould , D. Ferrand , L. W. Molenkamp

Random hyperfine fields are essential to mechanisms of low-field magnetoresistance in organic semiconductors. Recent experiments have shown that another type of random field --- fringe fields due to a nearby ferromagnet --- can also…

介观与纳米尺度物理 · 物理学 2013-04-12 Nicholas J. Harmon , Ferran Macià , Fujian Wang , Markus Wohlgenannt , Andrew D. Kent , Michael E. Flatté

Whereas spintronics brings the spin degree of freedom to electronic devices, molecular/organic electronics adds the opportunity to play with the chemical versatility. Here we show how, as a contender to commonly used inorganic materials,…

The unique properties of organic semiconductors make them versatile base materials for many applications ranging from light emitting diodes to transistors. The low spin-orbit coupling typical for carbon-based materials and the resulting…

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