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Based on the reduced density matrix method, we compare two different approaches to calculate the dynamics of the electron transfer in systems with donor, bridge, and acceptor. In the first approach a vibrational substructure is taken into…

量子物理 · 物理学 2009-10-31 M. Schreiber , D. Kilin , U. Kleinekathoefer

This paper presents a possible explanation for the enhanced singlet exciton yield in light emitting polymers. We propose a theory of electron-hole recombination via inter-molecular inter-conversion from inter-molecular weakly bound polaron…

化学物理 · 物理学 2009-11-10 William Barford

The population dynamics of single- and bi-exciton states in semiconductor nanocrystals is modeled numerically in the presence of Coulomb coupling between single- and two-exciton states and a dissipation channel in order to study the…

介观与纳米尺度物理 · 物理学 2013-09-11 Maryam Azizi , Paweł Machnikowski

Exciton-polaritons emerging from the interaction of photons and excitons in the strong coupling regime are intriguing quasiparticles for the potential exchange of energy during light-matter interaction processes such as light harvesting.…

In order to discuss the exciton fine-structure of transition-metal dichalcogenides mono-layers, excitons are first defined in the subspace of electron- and hole states, including the lowest conduction band (LCB) and the uppermost valence…

介观与纳米尺度物理 · 物理学 2019-06-25 Pierre Gilliot , Mathieu Gallart , Bernd Hönerlage

As a platform for optoelectronic devices based on exciton dynamics, monolayer transition metal dichalcogenides (TMDCs) are often placed near metal interfaces or inside planar cavities. While the radiative properties of point dipoles at…

介观与纳米尺度物理 · 物理学 2022-03-02 Grace H. Chen , David Z. Li , Amy Butcher , Alexander A. High , Darrick E. Chang

Non-radiative optical energy transfer from a GaAs quantum well to a thin overlayer of an infrared organic semiconductor dye is unambiguously demonstrated. The dynamics of exciton transfer are studied in the time-domain using pump-probe…

其他凝聚态物理 · 物理学 2009-11-13 S. Chanyawadee , P. G. Lagoudakis , R. T. Harley , D. G. Lidzey , M. Henini

Singlet fission, an exciton multiplication process in organic semiconductors which converts one singlet exciton into two triplet excitons is a promising way to reduce thermalization losses in conventional solar cells. One way to harvest…

应用物理 · 物理学 2018-10-09 Moritz H. Futscher , Akshay Rao , Bruno Ehrler

Models of organic bulk heterojunction photovoltaics which include the effect of spatially varying composition of donor/acceptor materials are developed and analyzed. Analytic expressions for the current-voltage relation in simplified cases…

介观与纳米尺度物理 · 物理学 2015-05-27 Paul M. Haney

Excitons play an essential role in the optical response of two-dimensional materials. These are bound states showing up in the band gaps of many-body systems and are conceived as quasiparticles formed by an electron and a hole. By…

光学 · 物理学 2024-06-21 Mikhail Malakhov , Giovanni Cistaro , Fernando Martín , Antonio Picón

The existence of bound charge transfer (CT) excitons at the interface of monolayer lateral heterojunctions has been debated in literature, but contrary to the case of interlayer excitons in vertical heterostructure their observation still…

The rates of exciton transfer within dyads of perylene diimide and terrylene diimide connected by oligophenylene bridge units have been shown to deviate significantly from those of F\"{o}rster's resonance energy transfer theory, according…

化学物理 · 物理学 2026-01-13 Lei Yang , Seogjoo J. Jang

In organic semiconductor based bulk heterojunction solar cells, the presence of acceptor increases the formation of charge transfer (CT) excitons, thereby leading to higher exciton dissociation probabilities. In this work we used steady…

We calculate radiative lifetimes of collective electronic excitations of atoms in an infinite one dimensional lattice. The translational symmetry along the lattice restricts the photon wave vector component parallel to the lattice to the…

量子物理 · 物理学 2010-05-20 Hashem Zoubi , Helmut Ritsch

We have investigated the exciton dynamics in transition metal dichalcogenide mono-layers using time-resolved photoluminescence experiments performed with optimized time-resolution. For MoSe2 monolayers, we measure $\tau_{rad}=1.8\pm0.2$ ps…

材料科学 · 物理学 2016-05-18 C. Robert , D. Lagarde , F. Cadiz , G. Wang , B. Lassagne , T. Amand , A. Balocchi , P. Renucci , S. Tongay , B. Urbaszek , X. Marie

Strong light--matter interactions forming hybrid quasiparticles termed polaritons can specifically tailor molecular photophysics. In this spirit, enhancing energy transport has recently been of special interest. Exciton--exciton…

化学物理 · 物理学 2026-01-14 Luca Nils Philipp , Julian Lüttig , Roland Mitric

Low-dimensional materials differ from their bulk counterpart in many respects. In particular, the screening of the Coulomb interaction is strongly reduced, which can have important consequences such as the significant increase of exciton…

We enlarge our results from the study of the hopping mechanism of the oscillation excitation transport in 1D model of one biology-like macromolecular chain to the case of a system composed from two 1D parallel macromolecular chains with…

介观与纳米尺度物理 · 物理学 2016-01-12 D. Čevizović , S. Petković , S. Galović , A. Chizhov , A. Reshetnyak

The analytically tractable model employing Quantum Markovian Master Equations, derived by weak coupling procedure and satisfying complete positivity, is proposed to describe a model of molecular battery charged by a non-equilibrium…

量子物理 · 物理学 2019-06-26 Robert Alicki

The 248nm and 193nm photodissociation of submonolayer quantities of CH$_3$Br and CH$_3$I adsorbed on thin layers of n-hexane indicate that the dissociation is caused by dissociative electron attachment from sub-vacuum level photoelectrons…

化学物理 · 物理学 2009-11-13 E. T. Jensen
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