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We present a theoretical model of the "isostructural" \gamma-\alpha phase transition in Ce which is based on quadrupolar interactions due to coupled charge density fluctuations of 4f electrons and of conduction electrons. Conduction…

强关联电子 · 物理学 2009-10-31 A. V. Nikolaev , K. H. Michel

We report direct experimental evidence for long-range antiferro ordering of the electric-quadrupole moments on the U ions. Resonant x-ray scattering experiments at the uranium $M_{4}$ absorption edge show a characteristic dependence in the…

强关联电子 · 物理学 2014-09-25 S. B. Wilkins , R. Caciuffo , C. Detlefs , J. Rebizant , E. Colineau , F. Wastin , G. H. Lander

We report the results of magnetic, heat-capacity, electrical and magnetoresistance measurements on Ho4RhAl and Er4RhAl, characterized by 3 sites for rare-earths (R). Antiferromagnetic ordering sets in at (T_N =) about 8.8 and 4.0 K…

强关联电子 · 物理学 2021-08-18 Ram Kumar , E. V. Sampathkumaran

The large number of low-lying states of d- and f-shells supports a variety of order parameters. The effective dimensionality of the local Hilbert space depends on the strength, and kind, of intersite interactions. This gives rise to…

强关联电子 · 物理学 2007-05-23 P. Fazekas , A. Kiss

CuFeO_2 is one of the multiferroic materials and is the first case that the electric polarization is not explained by the magnetostriction model or the spin-current model. We have studied this material using soft x-ray resonant diffraction…

SrHo2O4 is a geometrically frustrated magnet in which the magnetic Ho3+ ions form honeycomb layers connected through a network of zigzag chains. At low-temperature two distinct types of short-range magnetic order can be inferred from single…

强关联电子 · 物理学 2013-06-10 O. Young , A. R. Wildes , P. Manuel , B. Ouladdiaf , D. D. Khalyavin , G. Balakrishnan , O. A. Petrenko

The ground-state phase diagrams of the three-orbital t2g Hubbard model are studied using a Hartree-Fock approximation. First, a complete set of multipolar order parameters for t2g models defined in terms of the effective total angular…

强关联电子 · 物理学 2022-01-05 Naoya Chikano , Shintaro Hoshino , Hiroshi Shinaoka

Neutron scattering experiments have revealed a field-induced antiferroquadrupolar order parameter in the Pr-based heavy-fermion superconductor PrOs$_4$Sb$_{12}$. We observed the field-induced antiferromagnetic dipole moment with the…

强关联电子 · 物理学 2007-05-23 K. Kaneko , N. Metoki , R. Shiina , T. D. Matsuda , M. Kohgi , K. Kuwahara , N. Bernhoeft

The complex interplay between the 3d and 4f moments in hexagonal ErMnO3 is investigated by magnetization, optical second harmonic generation, and neutron-diffraction measurements. We revise the phase diagram and provide a microscopic model…

强关联电子 · 物理学 2012-11-14 D. Meier , H. Ryll , K. Kiefer , B. Klemke , J. -U. Hoffmann , R. Ramesh , M. Fiebig

We report a soft x-ray resonant magnetic scattering study of the spin configuration in multiferroic thin films of Co$_{0.975}$Ge$_{0.025}$Cr$_2$O$_4$ (Ge-CCO) and CoCr$_2$O$_4$ (CCO), under low- and high-magnetic fields, from 0.2 T up to…

Superconductivity, magnetic order, and quadrupolar order have been investigated in the filled skutterudite system Pr$_{1-x}$Nd$_{x}$Os$_4$Sb$_{12}$ as a function of composition $x$ in magnetic fields up to 9 tesla and at temperatures…

We have carried out a unified microscopic study of electric monopole, quadrupole and magnetic dipole excitations in fast rotating nuclei undergoing backbending, with special attention at the magnetic excitations. We found, among other…

核理论 · 物理学 2007-05-23 J. Kvasil , N. Lo Iudice , R. G. Nazmitdinov , A. Porrino , F. Knapp

High-resolution resonant inelastic X-ray scattering (RIXS) at the oxygen K-edge has been used to study the orbital excitations of Ca2RuO4 and Sr2RuO4. In combination with linear dichroism X-ray absorption spectroscopy, the ruthenium…

Neutron scattering measurements on the spin-ice candidate material Ho$_2$Ru$_2$O$_7$ have revealed two magnetic transitions at T $\sim$ 95 K and T $\sim$ 1.4 K to long-range ordered states involving the Ru and Ho sublattices, respectively.…

Hard x-ray scattering (HXS) experiments with a photon energy of 100keV were performed as a function of temperature and applied magnetic field on selected compounds of the RFe$_3$(BO$_3$)$_4$ family. The results show the presence of several…

This article reports a detailed x-ray resonant scattering study of the bilayer iridate compound, Sr3Ir2O7, at the Ir L2 and L3 edges. Resonant scattering at the Ir L3 edge has been used to determine that Sr3Ir2O7 is a long-range ordered…

The nature of multiple electronic orders in skutterudite PrFe_4P_{12} is discussed on the basis of a model with antiferro-quadrupole (AFQ) interaction of \Gamma_3 symmetry. The high-field phase can be reproduced qualitatively provided (i)…

强关联电子 · 物理学 2009-11-11 Annamaria Kiss , Yoshio Kuramoto

Single crystals of iron(IV) rich oxides SrFeO(3-x) with controlled oxygen content have been studied by Moessbauer spectroscopy, magnetometry, magnetotransport measurements, Raman spectroscopy, and infrared ellipsometry in order to relate…

强关联电子 · 物理学 2009-11-11 P. Adler , A. Lebon , V. Damljanovic , C. Ulrich , C. Bernhard , A. V. Boris , A. Maljuk , C. T. Lin , B. Keimer

Neutron scattering experiments were performed on single crystals of layered cobalt-oxides La2-xCaxCoO4 (LCCO) to characterize the charge and spin orders in a wide hole-doping range of 0.3<x<0.8. For a commensurate value of x=0.5 in (H,0,L)…

强关联电子 · 物理学 2009-11-13 K. Horigane , H. Hiraka , T. Uchida , K. Yamada , J. Akimitsu

We have employed resonant x-ray magnetic scattering to specifically probe the magnetic order of the rare-earth ions in multiferroic $\mathrm{TbMn_2O_5}$. Two energy resonances were observed, one originated from the E1-E1 dipolar transition…

强关联电子 · 物理学 2009-11-13 R. D. Johnson , S. R. Bland , C. Mazzoli , T. A. W. Beale , C. H. Du , C. Detlefs , S. B. Wilkins , P. D. Hatton