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The H$_2$+H$_2$ system has long been considered as a benchmark system for ro-vibrational energy transfer in bimolecular collisions. However, most studies thus far have focused on collisions involving H$_2$ molecules in the ground…

化学物理 · 物理学 2022-12-20 James F. E. Croft , Pablo G. Jambrina , F. Javier Aoiz , Hua Guo , N. Balakrishnan

We report quantum-mechanical close-coupling calculations for rotational state resolved cross sections for p-H2+HD collisions. The low temperature limit of p-H2+HD is investigated, which is of significant astrophysical interest in regard to…

化学物理 · 物理学 2015-06-26 Renat A. Sultanov , Dennis Guster

Rotational transitions in molecular hydrogen collisions are computed. The two most recently developed potential energy surfaces for the H2-H2 system are used from the following works: 1) A.I. Boothroyd, P.G. Martin, W.J. Keogh, M.J.…

化学物理 · 物理学 2009-11-11 Renat A. Sultanov , Dennis Guster

Experimental measurements and theoretical calculations of state-to-state rate coefficients for rotational energy transfer of CO in collision with H$_2$ are reported at the very low temperatures prevailing in dense interstellar clouds (5 -…

Full-dimensional quantum scattering calculations are reported for ro-vibrational transitions in HD+HD collisions using a highly accurate interaction potential for the H$_2$-H$_2$ system. Several near-resonant ro-vibrational transitions are…

原子物理 · 物理学 2026-03-06 Bikramaditya Mandal , Hubert Jóźwiak , Piotr Wcisło , Naduvalath Balakrishnan

We present a rigorous study of vibrational relaxation in p-H2 + p-H2 collisions at cold and ultracold temperatures and identify an efficient mechanism of ro-vibrational energy transfer. If the colliding molecules are in different rotational…

量子物理 · 物理学 2008-04-02 Goulven Quéméner , Naduvalath Balakrishnan , Roman V. Krems

We present quantum mechanical close-coupling calculations of collisions between two hydrogen molecules over a wide range of energies, extending from the ultracold limit to the super-thermal region. The two most recently published potential…

原子物理 · 物理学 2009-11-13 Teck-Ghee Lee , N. Balakrishnan , R. C. Forrey , P. C. Stancil , D. R. Schultz , Gary J. Ferland

In this work we report the results concerning calculations for quantum-mechanical rotational transitions in molecular hydrogen, H$_2$, induced by an ultra-cold ground state anti-hydrogen atom $\bar{H}_{1s}$. The calculations are…

原子物理 · 物理学 2015-05-14 Renat A. Sultanov , Sadhan K. Adhikari , Dennis Guster

Results for quantum mechanical calculations of the integral cross sections and corresponding thermal rate coefficients for para-/ortho-H2+HD collisions are presented. Because of significant astrophysical interest in regard to the cooling of…

化学物理 · 物理学 2015-05-13 Renat A. Sultanov , Avas V. Khugaev , Dennis Guster

We use the time-independent quantum-mechanical formulation of reactive collisions in order to investigate the state-to-state $\mathrm{H}^+ + \mathrm{HD} \to \mathrm{D}^+ + \mathrm{H}_2$ chemical reaction. We compute cross sections for…

宇宙学与河外天体物理 · 物理学 2019-07-10 Maxence Lepers , Grégoire Guillon , Pascal Honvault

A series of Multichannel Quantum Defect Theory-based computations have been performed, in order to produce the cross sections of rotational transitions (excitations $N_{i}^{+}-2 \rightarrow$ $N_{i}^{+}$, de-excitations $N_{i}^{+}$…

天体物理仪器与方法 · 物理学 2024-05-13 O. Motapon , N. Pop , F. Argoubi , J. Zs. Mezei , M. D. Epée Epée , A. Faure , M. Telmini , J. Tennyson , I. F. Schneider

State-selected total cross sections and thermal rate coefficients are computed for the HD + $ortho$-/$para$-H$_2$ rotational energy transfer collision at low temperatures: 2 K $\lesssim$ T $\lesssim$ 300 K. A modified H$_2$-H$_2$ potential…

化学物理 · 物理学 2016-01-28 Renat A. Sultanov , Dennis Guster , S. K. Adhikari

Rate coefficients for rotational transitions in H_2 induced by H_2 impact are presented. Extensive quantum mechanical coupled-channel calculations based on a recently published (H_2)_2 potential energy surface were performed. The potential…

天体物理学 · 物理学 2009-11-13 T. -G. Lee , N. Balakrishnan , R. C. Forrey , P. C. Stancil , G. Shaw , D. R. Schultz , G. J. Ferland

The Diep and Johnson (DJ) H$_2$-H$_2$ potential energy surface (PES) obtained from the first principles [P. Diep, K. Johnson, J. Chem. Phys. 113, 3480 (2000); 114, 222 (2000)], has been adjusted through appropriate rotation of the…

化学物理 · 物理学 2015-03-19 Renat A. Sultanov , Dennis Guster , S. K. Adhikari

Quantum-mechanical close-coupling calculations for state-to-state cross sections and thermal rates are reported for H2+H2 collisions. Two recently developed potential energy surfaces (PES) for the H2-H2 system are applied, namely, the…

化学物理 · 物理学 2009-11-11 Renat A. Sultanov , Dennis Guster

Two different ab initio potential energy surfaces are employed to investigate the efficiency of the rotational excitation channels for the polar molecular ion HeH$^+$ interacting with He atoms. We further use them to investigate the quantum…

Cross sections have been computed for rotational transitions of H2, induced by collisions with H atoms, using a recent H - H2 potential calculated by Mielke et al. [1]. These results are compared with those obtained with earlier potentials.…

天体物理学 · 物理学 2009-11-11 S A Wrathmall , D R Flower

The low-temperature (up to about 100K) collisional (de)excitation cross sections are computed using the full coupled-channel (CC) quantum dynamics for both Li$_2$ and Li$_2^+$ molecular targets in collision with $^4$He. The interaction…

化学物理 · 物理学 2007-07-13 M. Wernli. E. Bodo , F. A. Gianturco

Cold molecules are important for many applications, from fundamental precision measurements, quantum information processing, quantum-controlled chemistry, to understanding the cold interstellar medium. Molecular ions are known to be cooled…

Radiative decay processes at cold and ultra cold temperatures for Sulfur atoms colliding with protons are investigated. The MOLPRO quantum chemistry suite of codes was used to obtain accurate potential energies and transition dipole…

原子物理 · 物理学 2015-02-26 G Shen , P C Stancil , J G Wang , J F McCann , B M McLaughlin
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