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We theoretically investigate the interplay between charge ordering and magnetic states in quasi-one-dimensional molecular conductors TMTTF$_2X$, motivated by the observation of a complex variation of competing and/or coexisting phases. We…

强关联电子 · 物理学 2012-03-26 Kazuyoshi Yoshimi , Hitoshi Seo , Shoji Ishibashi , Stuart E. Brown

We have investigated the charge ordering phase of the quasi one dimensional quantum antiferromagnet (TMTTF)$_2X$ ($X=$ SbF$_6$, AsF$_6$ and PF$_6$) using high fields/frequencies electron paramagnetic resonance. In addition to the uniform…

强关联电子 · 物理学 2021-05-07 C-E Dutoit , A. Stepanov , J. VanTol , M. Orio , S. Bertaina

Charge order affects most of the electronic properties but is believed not to alter the spin arrangement since the magnetic susceptibility remains unchanged. We present electron-spin-resonance experiments on quasi-one-dimensional (TMTTF)2X…

强关联电子 · 物理学 2013-03-19 M. Dressel , M. Dumm , T. Knoblauch , B. Köhler , B. Salameh , S. Yasin

Using a combination of Density Functional Theory, mean-field analysis and exact diagonalization calculations we reveal the emergence of a dimerized charge ordered state in TMTTF$_2$-PF$_6$ organic crystal. The interplay between charge and…

强关联电子 · 物理学 2015-03-19 Gianluca Giovannetti , Sanjeev Kumar , Jean-Paul Pouget , Massimo Capone

High-resolution thermal expansion measurements have been performed for exploring the mysterious "structureless transition" in (TMTTF)$_{2}$X (X = PF$_{6}$ and AsF$_{6}$), where charge ordering at $T_{CO}$ coincides with the onset of…

强关联电子 · 物理学 2008-11-24 M. de Souza , P. Foury-Leylekian , A. Moradpour , J. -P. Pouget , M. Lang

(TMTTF)2AsF6 and (TMTTF)2SbF6 are both known to undergo a charge ordering phase transition, though their ground states are different. The ground state of the first is Spin-Peierls, and the second is an antiferromagnet. We study the effect…

强关联电子 · 物理学 2009-11-10 W. Yu , F. Zamborszky , B. Alavi , A. Baur , C. A. Merlic , S. E. Brown

Motivated by recent experimental suggestions of charge-order-driven ferroelectricity in organic charge-transfer salts, such as $\kappa$-(BEDT-TTF)$_2$Cu[N(CN)$_2$]Cl, we investigate magnetic and charge-ordered phases that emerge in an…

强关联电子 · 物理学 2017-10-30 Ryui Kaneko , Luca F. Tocchio , Roser Valentí , Federico Becca

We present the results of our theoretical study on the effects of geometrical frustration and the interplay between spin and orbital degrees of freedom in vanadium spinel oxides $A$V$_2$O$_4$ ($A$ = Zn, Mg or Cd). Introducing an effective…

强关联电子 · 物理学 2015-06-24 Yukitoshi Motome , Hirokazu Tsunetsugu

The effects of spin and charge fluctuations and electron-phonon couplings on charge ordering in \alpha-(BEDT-TTF)_2I_3 (BEDT-TTF=bis(ethylenedithio)-tetrathiafulvalence) are investigated theoretically for an anisotropic triangular lattice…

强关联电子 · 物理学 2009-11-13 Satoshi Miyashita , Kenji Yonemitsu

Charge-ordering phenomena have been highly topical over the last few years. A phase transition towards a charge ordered state has been observed experimentally in several classes of materials. Among them, many studies have been devoted to…

强关联电子 · 物理学 2013-08-01 Mariano de Souza , Jean-Paul Pouget

We study the effect of spin anisotropies on a frustrated quantum antiferromagnet using the J_1-J_2^{XXZ} model on the square lattice. The T=0 and finite-T phase diagrams of this model are obtained utilizing spin-wave theory, exact…

强关联电子 · 物理学 2009-11-10 Tommaso Roscilde , Adrian Feiguin , Alexander L. Chernyshev , Shiu Liu , Stephan Haas

It has been shown experimentally a long time ago that the magnetic ordering causes an anomalous behavior of the electron resistivity in ferromagnetic crystals. Phenomenological explanations based on the interaction between itinerant…

材料科学 · 物理学 2009-11-13 K. Akabli , H. T. Diep

The $1/4$-filled organic compound, $\delta$-(EDT-TTF-CONMe$_{2}$)$_{2}$AsF$_6$ is a frustrated two-dimensional triangular magnetic system as shown by high-frequency (111.2 and 222.4 GHz) electron spin resonance (ESR) and structural data in…

强关联电子 · 物理学 2016-11-22 B. Náfrádi , A. Antal , T. Fehér , L. F. Kiss , C. Mézière , P. Batail , L. Forró , A. Jánossy

Using various transport and magnetotransport probes we study the coexistence of spin-density wave and superconductor states in (TMTSF)2ClO4 at various degrees of ClO4 anions ordering. In the two-phase complex state when both…

We examine the various instabilities of quarter-filled strongly correlated electronic chains in the presence of a coupling to the underlying lattice. To mimic the physics of the (TMTTF)$_2$X Bechgaard-Fabre salts we also include…

强关联电子 · 物理学 2009-11-07 Jose Riera , Didier Poilblanc

Frustration refers to competition between different interactions that cannot be simultaneously satisfied, a familiar feature in many magnetic solids. Strong frustration results in highly degenerate ground states, and a large suppression of…

强关联电子 · 物理学 2007-07-03 Doron Bergman , Jason Alicea , Emanuel Gull , Simon Trebst , Leon Balents

The quasi-one-dimensional organic conductors (TMTTF)$_2X$ with non-centrosymmetric anions commonly undergo charge- and anion-order transitions upon cooling. While for compounds with tetrahedral anions ($X$ = BF$_4^-$, ReO$_4^-$, and…

We give a short review of our recent works on the first-order quantum phase transitions in frustrated spin chains with orthogonal-dimer structure. When the ratio of the competing antiferromagnetic exchange couplings is varied, a first-order…

强关联电子 · 物理学 2009-11-07 Akihisa Koga , Akira Kawaguchi , Kouichi Okunishi , Norio Kawakami

The origin of the spin gap behavior in the low-temperature dimerized phase of theta-(BEDT-TTF)_2RbZn(SCN)_4 has been theoretically studied based on the Hartree-Fock approximation for the on-site Coulomb interaction at absolute zero.…

强关联电子 · 物理学 2009-10-31 Hitoshi Seo , Hidetoshi Fukuyama

We present the results of muon-spin relaxation ($\mu^{+}$SR) measurements on antiferromagnetic and ferromagnetic spin chains. In antiferromagnetic CuF$_{2}$(pyz) we identify a transition to long range magnetic order taking place at…

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