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Alkali superoxides differ from conventional transition metal magnets, exhibit magnetism from partially occupied oxygen molecular $\pi^*$-orbitals. Among them, CsO$_2$ stands out for its potential to exhibit novel quantum collective…

强关联电子 · 物理学 2024-11-12 Ryota Ono , Ravi Kaushik , Sergey Artyukhin , Martin Jansen , Igor Solovyev , Russell A. Ewings

The electronic structures of the cubic and tetragonal $\mathrm{MnV}_2\mathrm{O}_4$ have been studied by using hybrid-exchange density functional theory. The computed electronic structure of the tetragonal phase shows an anti-ferro orbital…

强关联电子 · 物理学 2015-05-08 Wei Wu

Exchange interaction tends to favor collinear or coplanar magnetic orders in rotationally invariant spin systems. Indeed, such magnetic structures are usually selected by thermal or quantum fluctuations in highly frustrated magnets. Here we…

强关联电子 · 物理学 2010-11-25 Gia-Wei Chern

The magnetic excitations of the iron pnictides are explained within a degenerate double-exchange model. The local-moment spins are coupled by superexchanges $J_1$ and $J_2$ between nearest and next-nearest neighbors, respectively, and…

强关联电子 · 物理学 2015-05-18 Weicheng Lv , Frank Krüger , Philip Phillips

First principles density functional calculations within the local spin density approximation (LSDA) and the generalized gradient approximation (GGA) are reported for pyrochlore Cd$_2$Os$_2$O$_7$ and Cd$_{2}$Re$_{2}$O$_7$. The transition…

凝聚态物理 · 物理学 2009-11-07 D. J. Singh , P. Blaha , K. Schwarz , J. O. Sofo

A spin-orbital superexchange Hamiltonian in a Mott insulator with $t_{2g}$ orbital degeneracy is investigated. More specifically, we focus on a spin ferromagnetic state of the model and study a collective behavior of orbital angular…

强关联电子 · 物理学 2009-11-11 G. Khaliullin , S. Okamoto

Spinel compounds AB$_{2}$X$_{4}$ consist of both tetrahedral (AX$_{4}$) and octahedral (BX$_{6}$) environments with the former forming a diamond lattice and the latter a geometrically frustrated pyrochlore lattice. Exploring the fascinating…

化学物理 · 物理学 2023-03-29 Qiang Zhang , Wei Tian , Roshan K. Nepal , Ashfia Huq , Stephen Nagler , J. F. DiTusa , Rongying Jin

The recent discovery of Spin-ice is a spectacular example of non-coplanar spin arrangements that can arise in the pyrochlore A2B2O7 structure. We present magnetic and thermodynamic studies on the metallic-ferromagnet pyrochlore Sm2Mo2O7.…

强关联电子 · 物理学 2009-11-13 Surjeet Singh , R. Suryanarayanan , R. Tackett , G. Lawes , A. K. Sood , P. Berthet , A. Revcolevschi

Two-dimensional metallic altermagnets are rare, and no correlated 2D material has been established to host large nonrelativistic spin splitting. Here we show that spontaneous orbital order, driven by electronic correlations and Fermi…

介观与纳米尺度物理 · 物理学 2026-03-27 Nirmalya Jana , Atasi Chakraborty , Anamitra Mukherjee , Amit Agarwal

In contrast to the previous reports that the divalent perovskite SrCrO$_3$ was believed to be cubic structure and nonmagnetic metal, recent measurements suggest coexistence of majority tetragonally distorted weak antiferromagnetic phase and…

强关联电子 · 物理学 2009-10-01 K. -W. Lee , W. E. Pickett

Frustration in spin system can give rise to unique ordered states and as a consequence several physical phenomena are expected such as multiferroics, high temperature superconductors and anomalous hall effect. Here we report the "new…

强关联电子 · 物理学 2018-08-01 GiBaik Sim , SungBin Lee

Neutron scattering has been used to study the magnetic order and spin dynamics of the colossal magnetoresistive pyrochlore Tl_2Mn_2O_7. On cooling from the paramagnetic state, magnetic correlations develop and appear to diverge at T_C (123…

强关联电子 · 物理学 2009-10-31 J. W. Lynn , L. Vasiliu-Doloc , M. A. Subramanian

Neutron scattering studies on powder and single crystals have provided new evidences for unconventional magnetism in Cu2Te2O5Cl2. The compound is built from tetrahedral clusters of S=1/2 Cu2+ spins located on a tetragonal lattice. Magnetic…

强关联电子 · 物理学 2009-11-11 O. Zaharko , H. M. Ronnow , A. Daoud-Aladine , S. Streule , F. Juranyi , J. Mesot , H. Berger , P. J. Brown

Noncollinear and noncoplanar magnetic textures including skyrmions and vortices act as emergent electromagnetic fields and give rise to novel electronic and transport properties. We here report a unified understanding of noncoplanar…

强关联电子 · 物理学 2017-06-28 Satoru Hayami , Ryo Ozawa , Yukitoshi Motome

The question of structural disorder and its effects on magnetism is relevant to a number of spin liquid candidate materials. Although commonly thought of as a route to spin glass behavior, here we describe a system in which the structural…

We review neutron scattering investigations of the crystal structures, magnetic structures, and spin dynamics of the iron-based RFe(As,P)O (R=La, Ce, Pr, Nd), (Ba,Sr,Ca)Fe2As2, and Fe1+x(Te-Se) systems. On cooling from room temperature all…

超导电性 · 物理学 2009-05-20 Jeffrey W. Lynn , Pengcheng Dai

MgV$_{2}$O$_{4}$ is a spinel based on magnetic V$^{3+}$ ions which host both spin ($S=1$) and orbital ($l_{eff}=1$) moments. Owing to the underlying pyrochlore coordination of the magnetic sites, the spins in MgV$_{2}$O$_{4}$ only…

Using Monte Carlo techniques, we show that the recently experimentally observed transitionlike phenomena in the transverse spin-ordering close to the anomalies in the antiferromagnetic phase of FeBr2 (Petracic et al. [Phys. Rev. B 57,…

凝聚态物理 · 物理学 2009-10-31 M. Pleimling , W. Selke

We consider the superstructures, which can be formed in spinels containing on B-sites the transition-metal ions with partially filled t2g levels. We show that, when such systems are close to itinerant state (e.g. have an insulator-metal…

强关联电子 · 物理学 2009-11-10 D. I. Khomskii , T. Mizokawa

The Stoner instability remains a cornerstone for understanding metallic ferromagnets. This instability captures the interplay of Coulomb repulsion, Pauli exclusion, and two-fold fermionic spin degeneracy. In materials with spin-orbit…

强关联电子 · 物理学 2024-11-13 Yue Yu , Tatsuya Shishidou , Shuntaro Sumita , Michael Weinert , Daniel F. Agterberg
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