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We study ultrafast ionization dynamics using orthogonally polarized two-color (OTC) laser pulses involving the resonant "first plus second" ($\omega+2\omega$) scheme. The scheme is illustrated by numerical simulations of the time-dependent…

原子物理 · 物理学 2019-12-16 Hicham Agueny

We study the interaction of intense ultrashort laser pulses with cryogenic He jets using 2d/3v relativistic Particle-in-Cell simulations (XOOPIC). Of particular interest are laser intensities $(10^{15}-10^{20})$ W/cm$^2$, pulse lengths $\le…

等离子体物理 · 物理学 2017-04-05 M. Shihab , T. Bornath , R. Redmer

The interference of matter waves is one of the intriguing features of quantum mechanics that has impressed researchers and laymen since it was first suggested almost a century ago. Nowadays, attosecond science tools allow us to utilize it…

化学物理 · 物理学 2021-11-03 Kasra Amini , Alexis Chacón , Sebastian Eckart , Benjamin Fetić , Matthias Kübel

We study the ionization of atomic hydrogen in the direction of polarization due to a linearly polarized XUV pulse in the presence a strong field IR. We describe the photoelectron spectra as an interference problem in the time domain.…

原子物理 · 物理学 2016-11-15 Ana Alicia Gramajo , Renata Della Picca , Carlos Roberto Garibotti , Diego Arbó

Amplitude and phase of wavepackets encode the dynamics of quantum systems. However, the rapidity of electron dynamics on the attosecond timescale has precluded their complete measurement in the time domain. Here, we demonstrate that…

Photoassociation of ultracold rubidium atoms with femtosecond laser pulses is studied theoretically. The spectrum of the pulses is cut off in order to suppress pulse amplitude at and close to the atomic resonance frequency. This leads to…

We theoretically study time-resolved photoemission in atoms as probed by attosecond streaking. We review recent advances in the study of the photoelectric effect in the time domain and show that the experimentally accessible time shifts can…

原子物理 · 物理学 2015-03-06 Stefan Nagele , Renate Pazourek , Michael Wais , Georg Wachter , Joachim Burgdörfer

The femtosecond evolution of the electronic temperature of laser-excited gold nanoparticles is measured, by means of ultrafast time-resolved photoemission spectroscopy induced by extreme-ultraviolet radiation pulses. The temperature of the…

An ab initio molecular dynamics study of femtosecond laser processing of germanium is presented in this paper. The method based on the finite temperature density functional theory is adopted to probe the structural change, thermal motion of…

计算物理 · 物理学 2016-02-02 Pengfei Ji , Yuwen Zhang

During multi-photon ionization of an atom it is well understood how the involved photons transfer their energy to the ion and the photoelectron. However, the transfer of the photon linear momentum is still not fully understood. Here, we…

原子物理 · 物理学 2020-02-19 Benjamin Willenberg , Jochen Maurer , Benedikt W. Mayer , Ursula Keller

We analyze the attosecond electron dynamics in hydrogen molecular ion driven by an external intense laser field using ab-initio numerical simulations of the corresponding time-dependent Schr{\"{o}}dinger equation and Bohmian trajectories.…

化学物理 · 物理学 2015-05-20 Norio Takemoto , Andreas Becker

Electron motion on the (sub-)femtosecond time scale constitutes the fastest response in many natural phenomena such as light-induced phase transitions and chemical reactions. Whereas static electron densities in single molecules can be…

Strong-field manipulation of autoionizing states is a crucial aspect of electronic quantum control. Recent measurements of the attosecond transient absorption spectrum of helium dressed by a few-cycle visible pulse [Ott et al.,…

原子物理 · 物理学 2012-11-13 Luca Argenti , Christian Ott , Thomas Pfeifer , Fernando Martín

The processes of ionization and energy transfer in a quantum system composed of two distant H atoms with an initial internuclear separation of 100 atomic units (5.29 nm) have been studied by the numerical solution of the time-dependent…

量子物理 · 物理学 2017-09-13 Guennaddi K. Paramonov , Andre D. Bandrauk , Oliver Kühn

Photoionization by attosecond (as) extreme ultraviolet (xuv) pulses into the laser-dressed continuum of the ionized atom is commonly described in strong-field approximation (SFA), neglecting the Coulomb interaction between the emitted…

原子与分子团簇 · 物理学 2015-05-20 C. -H. Zhang , U. Thumm

We present theoretical studies on real-time probing the electron density evolution of an atom in a strong infrared (IR) laser field with few-cycle near-infrared (NIR) and attosecond extreme-ultraviolet (XUV) pulses. Our results indicate…

原子物理 · 物理学 2015-06-04 Yunpei Deng , Xinhua Xie

In a recent experiment by Eichmann et al., polarization-sensitive measurements of the fluorescence from two four-level ions driven by a linearly polarized laser were made. Depending on the polarization chosen, different degrees of…

原子物理 · 物理学 2009-10-30 T. Wong , S. M. Tan , M. J. Collett , D. F. Walls

Photoelectron holography constitutes a powerful tool for the ultrafast imaging of matter, as it combines high electron currents with subfemtosecond resolution, and gives information about transition amplitudes and phase shifts. Similarly to…

原子物理 · 物理学 2020-02-19 C. Figueira de Morisson Faria , A. S. Maxwell

We report on a theoretical study of a Cs$_2$ molecule illuminated by two lasers and show how it can result in novel quantum dynamics. We reveal that these interactions facilitate the bypass of the non-crossing rule, forming Light-Induced…

化学物理 · 物理学 2024-05-21 Edgar Barriga , Luis E. F. Foa Torres , Carlos Cárdenas