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The local interaction of charges and light in organic solids is the basis of distinct and fundamental effects. We here observe, at the single molecule scale, how a focused laser beam can locally shift by hundreds-time their natural…

The dissociation dynamics of diatomic molecules interacting with (near) optical laser pulses of different duration is investigated by an elaborate discussion of the electric field of the laser and by a direct solution of the time-dependent…

原子物理 · 物理学 2019-08-14 T. Fiedlschuster , J. Handt , E. K. U. Gross , R. Schmidt

We study the interaction of strong femtosecond laser pulses with the C$_{60}$ molecule employing time-dependent density functional theory with the ionic background treated in a jellium approximation. The laser intensities considered are…

原子与分子团簇 · 物理学 2009-11-07 D. Bauer , F. Ceccherini , A. Macchi , F. Cornolti

The kinetic energy distribution of D$^+$ ions resulting from the interaction of a femtosecond laser pulse with D$_2$ molecules is calculated based on the rescattering model. From analyzing the molecular dynamics, it is shown that the…

原子物理 · 物理学 2009-11-10 X. M. Tong , Z. X. Zhao , C. D. Lin

Double electron ionisation process occurs when an intense laser pulse interacts with atoms or molecules. Exact {\it ab initio} numerical simulation of such a situation is extremely computer resources demanding, thus often one is forced to…

Realistic attosecond wave packets have complex profiles that, in dispersive conditions, rapidly broaden or split into multiple components. Such behaviors are encoded in sharp features of the wave packet spectral phase. Here, we exploit the…

Multiphoton ionization provides a clear window into the nature of electron correlations in the helium atom. In the present study, the final state energy range extends up to the region near the $N=2$ and $N=3$ ionization thresholds, where…

原子物理 · 物理学 2021-03-10 Yimeng Wang , Chris H. Greene

We apply the convergent close-coupling (CCC) formalism to analyse the processes of laser assisted electron impact ionisation of He, and the attosecond time delay in the photodetachment of the H^{-} ion and the photoionisation of He. Such…

原子物理 · 物理学 2016-11-04 Alexander William Bray

We theoretically investigate the scattering of an attosecond electron wave packet launched by an attosecond pulse under the influence of an infrared laser field. As the electron scatters inside a spatially extended system, the dressing…

量子物理 · 物理学 2015-05-19 Justin Gagnon , Ferenc Krausz , Vladislav S. Yakovlev

We report attosecond-scale probing of the laser-induced dynamics in molecules. We apply the method of high-harmonic spectroscopy, where laser-driven recolliding electrons on various trajec- tories record the motion of their parent ion.…

Ionization of atoms and molecules by absorption of a light pulse results in electron wavepackets carrying information on the atomic or molecular structure as well as on the dynamics of the ionization process. These wavepackets can be…

We calculate the photoionization with excitation-to photoionization ratios for atomic helium and heliumlike ions at intermediate values of the photon energies. The final state interactions between the electrons are included in the lowest…

量子物理 · 物理学 2009-11-13 E. G. Drukarev , E. Z. Liverts , M. Ya. Amusia , R. Krivec , V. B. Mandelzweig

We investigate the possibility to use transient absorption of a coherent bound electron wave packet in hydrogen as an attosecond pulse characterization technique. In recent work we have shown that photoionization of such a coherent bound…

光学 · 物理学 2017-11-22 Jan Marcus Dahlström , Stefan Pabst , Eva Lindroth

Few-photon induced breakup of helium is studied using a newly developed ab initio numerical framework for solving the six-dimensional time-dependent Schroedinger equation. We present details of the method and calculate (generalized) cross…

原子物理 · 物理学 2010-06-11 R. Nepstad , T. Birkeland , M. Førre

Multiphoton ionization of sodium by femtosecond laser pulses of 800 nm wavelength in the range of laser peak intensities entering over-the-barrier ionization domain is studied. Photoelectron momentum distributions and the energy spectra are…

原子物理 · 物理学 2021-02-24 A. Bunjac , D. B. Popovic , N. S. Simonovic

We demonstrate a two-dimensional time-domain spectroscopy method to extract amplitude and phase modifications of excited atomic states caused by the interaction with ultrashort laser pulses. The technique is based on Fourier analysis of the…

原子物理 · 物理学 2015-06-19 Alexander Blättermann , Christian Ott , Andreas Kaldun , Thomas Ding , Thomas Pfeifer

Polyatomic molecules in strong laser fields can undergo substantial nuclear motion within tens of femtoseconds. Ion imaging methods based on dissociation or Coulomb explosion therefore have difficulty faithfully recording the geometry…

The introduction of mid-IR optical parametric chirped pulse amplifiers (OPCPAs) has catalyzed interest in multi-millijoule, infrared femtosecond pulse-based filamentation. As tunneling ionization is a fundamental first stage in these…

We revisit a recently proposed scheme [M.F. Ciappina et al 2019 Phys. Rev. A 99 043405] for accurate measurement of electromagnetic radiation intensities in a focus of high-power laser beams. The method is based on the observation of…

原子物理 · 物理学 2020-02-19 M. F. Ciappina , S. V. Popruzhenko

We develop a time-dependent theory to investigate electron dynamics and photoionization processes of diatomic molecules interacting with strong laser fields including electron-electron correlation effects. We combine the recently formulated…

化学物理 · 物理学 2016-02-02 Henrik R. Larsson , Sebastian Bauch , Lasse Kragh Sørensen , Michael Bonitz