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The nature of multiple electronic orders in skutterudite PrFe_4P_{12} is discussed on the basis of a model with antiferro-quadrupole (AFQ) interaction of \Gamma_3 symmetry. The high-field phase can be reproduced qualitatively provided (i)…

强关联电子 · 物理学 2009-11-11 Annamaria Kiss , Yoshio Kuramoto

Specific heat and magnetization measurements have been performed on high-quality single crystals of filled-skutterudite PrFe_4P_{12} in order to study the high-field heavy-fermion state (HFS) and low-field ordered state (ODS). From a broad…

强关联电子 · 物理学 2009-11-07 Y. Aoki , T. Namiki , T. D. Matsuda , K. Abe , H. Sugawara , H. Sato

Characteristics of hybridization and multipole orders of $4f$-electrons in Pr skutterudites are explained in terms of a pseudo-quartet composed of crystalline electric field (CEF) singlet and the triplet. It is shown that the contrasting…

强关联电子 · 物理学 2015-06-25 Yoshio Kuramoto , Annamaria Kiss , Junya Otsuki , Hiroaki Kusunose

We report on systematic study of superconducting characteristics and Pr crystalline-electric-field (CEF) levels of filled-skutterudite \pra ($T_{\rm c}$ = 2.33 K). The temperature dependences of the upper critical field $H_{\rm c2}$ and the…

强关联电子 · 物理学 2007-10-03 T. Namiki , Y. Aoki , H. Sato , C. Sekine , I. Shirotani , T. D. Matsuda , Y. Haga , T. Yagi

Magnetization, specific heat, and electrical resistivity measurements were made on single crystals of the filled skutterudite compound PrOs$_{4}$As$_{12}$. Specific heat measurements indicate an electronic specific heat coefficient $\gamma$…

We report the electronic and superconducting properties in the Pr-based filled-skutterudite superconductor PrRu$_4$Sb$_{12}$ with $T_c = 1.3$ K via the measurements of nuclear-quadrupole-resonance (NQR) frequency $\nu_Q$ and…

超导电性 · 物理学 2009-11-10 M. Yogi , H. Kotegawa , Y. Imamura , G. -q. Zheng , Y. Kitaoka , H. Sugawara , H. Sato

Rare-earth metal filled skutterudites RPt4Ge12 with R=La-Nd, and Eu exhibit a variety of different ground states, e.g., conventional and unconventional superconductivity in LaPt4Ge12 and PrPt4Ge12, respectively, and intermediate valence…

强关联电子 · 物理学 2011-03-03 M. Nicklas , R. Gumeniuk , W. Schnelle , H. Rosner , A. Leithe-Jasper , F. Steglich , Yu. Grin

Superconductivity is observed in the filled skutterudite compound \PrOsSb{} below a critical temperature temperature $T_\mathrm{c} = 1.85$ K and appears to develop out of a nonmagnetic heavy Fermi liquid with an effective mass $m^{*}…

Thermal conductivity measurements were performed on single crystal samples of the superconducting filled skutterudite compounds PrOs$_4$Sb$_{12}$ and PrRu$_4$Sb$_{12}$ both as a function of temperature and magnetic field applied…

超导电性 · 物理学 2007-09-28 R. W. Hill , Shiyan Li , M. B. Maple , Louis Taillefer

The compound PrFe$_2$Al$_8$ possesses a three-dimensional network structure resulting from the packing of Al polyhedra centered at the transition metal element Fe and the rare earth Pr. Along the $c$-axis, Fe and Pr form {\em chains} which…

强关联电子 · 物理学 2015-12-24 Harikrishnan S. Nair , Sarit K. Ghosh , Ramesh Kumar K , André M. Strydom

We use neutron scattering to study the Pr$^{3+}$ crystalline electric field (CEF) excitations in the filled skutterudite PrOs$_4$As$_{12}$. By comparing the observed levels and their strengths under neutron excitation with the theoretical…

强关联电子 · 物理学 2008-10-22 Songxue Chi , Pengcheng Dai , T. Barnes , H. J. Kang , J. W. Lynn , R. Bewley , F. Ye , M. B. Maple , Z. Henkie , A. Pietraszko

In order to clarify magnetic properties of filled skutterudites, we analyze the Anderson model including seven $f$ orbitals hybridized with an $a_{\rm u}$ conduction band using a numerical technique. For $n$=2 corresponding to Pr-based…

强关联电子 · 物理学 2009-11-10 Takashi Hotta

The low-carrier ordered phase below the metal-non-metal transition temperature T_MI ~ 63 K of PrRu4P12 is explored by probing magnetoresistance, magnetic susceptibility, thermoelectric power, and Hall effect on high quality single crystals.…

强关联电子 · 物理学 2009-08-06 S. R. Saha , H. Sugawara , T. Namiki , Y. Aoki , H. Sato

New germanium-platinum compounds with the filled-skutterudite crystal structure were synthesized. The structure and composition were investigated by X-ray diffraction and microprobe analysis. Magnetic susceptibility, specific heat, and…

超导电性 · 物理学 2009-03-26 R. Gumeniuk , W. Schnelle , H. Rosner , M. Nicklas , A. Leithe-Jasper , Yu. Grin

The filled skutterudite compound \PrOsSb{} exhibits superconductivity below a critical temperature $T_\mathrm{c} = 1.85$ K that develops out of a nonmagnetic heavy Fermi liquid with an effective mass $m^{*} \approx 50 m_\mathrm{e}$, where…

超导电性 · 物理学 2007-05-23 M. B. Maple , P. -C. Ho , N. A. Frederick , V. S. Zapf , W. M. Yuhasz , E. D. Bauer

Rare 4f^2-based heavy-fermion behaviors have been revealed recently in Pr-based filled skutterudites PrFe4P12 and PrOs4Sb12. Recent studies on the thermal properties on both compounds are reported, putting emphasis on the field-induced…

强关联电子 · 物理学 2007-05-23 Y. Aoki , T. Namiki , T. Kanayama , S. Ohsaki , S. R. Saha , H. Sugawara , H. Sato

X-ray powder diffraction, magnetic susceptibility $\chi(T)$, and electrical resistivity $\rho(T)$ measurements were made on single crystals of the filled skutterudite series Pr(Os$_{1-x}$Ru$_x$)$_4$Sb$_{12}$. One end of the series ($x = 0$)…

超导电性 · 物理学 2009-11-10 N. A. Frederick , T. D. Do , P. -C. Ho , N. P. Butch , V. S. Zapf , M. B. Maple

Transport and magnetic properties of a 4$f^{2}$ fcc lattice compound, PrCdNi$_4$, were studied. The magnetic susceptibility, $\chi(T)$, follows the Curie--Weiss law from 300 K to 20 K, as expected for a free Pr$^{3+}$ ion. As the…

Filled skutterudite compound EuFe$_4$As$_{12}$ shows the highest magnetic ordering temperature of $T_{\rm C}$ = 154 K among Eu-based skutterudite compounds, but its magnetic ground state has not been determined yet. Here, we performed…

强关联电子 · 物理学 2020-08-26 Q. -P. Ding , H. -C. Lee , K. Nishine , Y. Kawamura , C. Sekine , Y. Furukawa

Motivated by current research efforts towards exploring the interplay between magnetism and superconductivity in multiband electronic systems, we have investigated the effects of Eu substitution through thermodynamic measurements on the…

强关联电子 · 物理学 2018-08-22 R. B. Adhikari , D. L. Kunwar , I. Jeon , M. B. Maple , M. Dzero , C. C. Almasan
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