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Ab initio quantum chemistry calculations are performed for the mixed alkali triatomic system. Global minima of the ground and first excited doublet states of the trimer are found and Born-Oppenheimer potential energy surfaces of the Li atom…

化学物理 · 物理学 2018-03-14 Patryk Jasik , Tymon Kilich , Jan Kozicki , Józef E. Sienkiewicz

In a recent experiment by Schaetz group \cite{weckesser2021}, the quantum $s$-wave regime has been attained for alkali and alkaline-earth atom-ion combination (Li-Ba$^+$). We investigate possible outcomes from interaction of this ion-atom…

原子物理 · 物理学 2023-05-10 D. Sardar , S. Naskar

The non-additive three-body interaction potential for helium was computed using the coupled-cluster theory and the full configuration interaction method. The obtained potential comprises an improved nonrelativistic Born--Oppenheimer energy…

We report state-of-the-art ab initio calculations of the potential energy curve for the $a^3\Sigma_u^+$ state of the lithium dimer conducted to achieve spectroscopic accuracy ($<$1cm$^{-1}$) without any prior adjustment to fit the…

化学物理 · 物理学 2021-01-27 Michał Lesiuk , Monika Musiał , Robert Moszynski

In this thesis, the electrostatic interaction between two chemically identical colloids, both carrying constant surface potential is studied in the limit of short inter-particle separation at the interface of two immiscible fluids. Using an…

软凝聚态物质 · 物理学 2020-01-01 Rick Bebon

The interactions between atoms and molecules may be described by a potential energy function of the nuclear coordinates. Non-bonded interactions are dominated by repulsive forces at short range and attractive dispersion forces at long…

A potential energy surface for the lowest quartet electronic state of lithium trimer is developed and used to study spin-polarized Li + Li_2 collisions at ultralow kinetic energies. The potential energy surface allows barrierless atom…

化学物理 · 物理学 2009-11-13 Marko T. Cvitas , Pavel Soldan , Jeremy M. Hutson , Pascal Honvault , Jean-Michel Launay

We present a theoretical investigation of cold reactive and non-reactive collisions of Li and Rb atoms with C$_{2}^{-}$. The potential energy surfaces for the singlet and triplet states of the Li--C$_{2}^{-}$ and Rb--C$_{2}^{-}$ systems…

原子物理 · 物理学 2019-04-17 Milaim Kas , Jérôme Loreau , Jacques Liévin , Nathalie Vaeck

We have measured the dependence of the relative integral cross section of the reaction Li+HF-->LiF+H on the collision energy using crossed molecular beams. By varying the intersection angle of the beams from 37{\deg} to 90{\deg} we covered…

化学物理 · 物理学 2011-12-19 Rolf Bobbenkamp , Hansjurgen Loesch , Marcel Mudrich , Frank Stienkemeier

We study theoretically interaction potentials and low energy collisions between different alkali atoms and alkali ions. Specifically, we consider systems like X + Y$^{+}$, where X(Y$^{+})$ is either Li(Cs$^+$) or Cs(Li$^+$), Na(Cs$^+$) or…

原子物理 · 物理学 2016-09-13 Arpita Rakshit , Chedli Ghanmi , Hamid Berriche , Bimalendu Deb

Potential Energy Surface for the ($\mathrm{\bar{p}} - \mathrm{He}^{2+} - \mathrm{He}$) system is calculated in the framework of the restricted (singlet spin state) Hartree-Fock method with subsequent account of the electronic correlations…

核理论 · 物理学 2017-06-29 S. N. Yudin , I. V. Bodrenko , G. Ya. Korenman

Potential energy surfaces of the hydrogen molecular ion H$_2^+$ in the Born-Oppenheimer approximation are computed by means of the Riccati-Pad\'e method (RPM). The convergence properties of the method are analyzed for different states. The…

化学物理 · 物理学 2022-10-25 Francisco Marcelo Fernández , Javier Garcia

In this thesis we study the lateral electrostatic interaction between a pair of non-identical, moderately charged colloidal particles trapped at an electrolyte interface in the limit of short inter-particle separations. Using a simplified…

软凝聚态物质 · 物理学 2017-10-17 Timo Schmetzer

The lowest doublet electronic state for the lithium trimer (2A') is calculated for use in three-body scattering calculations using the valence electron FCI method with atomic cores represented using an effective core potential. It is shown…

化学物理 · 物理学 2015-05-13 Jason N. Byrd , John A. Montgomery , H. Harvey Michels , Robin Côté

Reactive cross-sections for the collision of open shell S(^1D) atoms with ortho- and para-hydrogen, in the kinetic energy range 1-120 K, have been calculated using the hyperspherical quantum reactive scattering method developed by Launay et…

化学物理 · 物理学 2017-09-13 Manuel Lara , F. Dayou , J. -M. Launay

The long range potential of helium-helium interaction, which requires accurate 'ab initio' calculation, due to the small value of the potential depth, approximately 11 K (0.091 kJ/mol) at 2.96 angstrom, will be obtained in this study by an…

化学物理 · 物理学 2025-02-17 Éderson D'M. Costa , Nelson H. T. Lemes , João P. Braga

The accurate modeling of non-covalent interactions between helium and graphitic materials is important for understanding quantum phenomena in reduced dimensions, with the helium-benzene complex serving as the fundamental prototype. However,…

A four-dimensional potential energy surface for the interaction between He and HCN with vibrational bending is presented. Ab initio calculations were carried out at the coupled-cluster level with single and double excitations and a…

Correlated {\em ab initio} electronic structure calculations are reported for the polymers lithium hydride chain $[LiH]_{\infty}$ and beryllium hydride $[Be_{2}H_{4}]_{\infty}$. First, employing a Wannier-function-based approach, the…

凝聚态物理 · 物理学 2009-10-31 Ayjamal Abdurahman , Alok Shukla , Michael Dolg

We have determined an atom-surface interaction potential for the He$-$Bi$_2$Te$_3$(111) system by analysing ultrahigh resolution measurements of selective adsorption resonances. The experimental measurements were obtained using $^3$He…

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