相关论文: The challenge of attosecond pulse metrology
Ultrafast processes in matter can be captured and even controlled by using sequences of few-cycle optical pulses, which need to be well characterized, both in amplitude and phase. The same degree of control has not yet been achieved for…
Shaping electron beams with the cycles of light provides femtosecond and attosecond time resolution in electron microscopy and enables fundamental quantum-coherent measurements. However, efficient light-electron control requires a prolonged…
We employ the recently developed multi-photon R-matrix method for molecular above-threshold photoionization to obtain second-order ionization amplitudes that govern the interference in RABITT experiments. This allows us to extract RABITT…
Recollision physics and attosecond pulse generation meld the precision of optics with collision physics. As a follow-up to our previous work, we reveal a new direction for the study of electronic structure and multielectron dynamics by…
Semiconductor lasers offer native bifunctionality enabling coherent light emission and linear photodetection. They can also operate as sensitive two-photon absorption detectors due to the third-order nonlinearity of the heterostructure…
Atomic motion dynamics during structural changes or chemical reactions have been visualized by picosecond and femtosecond pulsed electron beams via ultrafast electron diffraction and microscopy. Imaging the even faster dynamics of electrons…
We investigate the problem of two-level atoms driven by an ultrashort pulse train in the frequency domain. At low intensity regime, we obtain a perturbative analytical solution that allows us to discuss the role of the mode number of the…
The evolution of electron wavepackets determines the course of many physical and chemical phenomena and attosecond spectroscopy aims to measure and control such dynamics in real-time. Here, we investigate radial electron wavepacket motion…
We report on attosecond-scale control of high-harmonic and electron emission from plasma mirrors driven by relativistic-intensity near-single-cycle lightwaves at kHz repetition rate. By controlling the waveform of the intense light…
Attosecond light pulses in the extreme ultraviolet have drawn a great deal of attention due to their ability to interrogate electronic dynamics in real time. Nevertheless, to follow charge dynamics and excitations in materials, element…
I discuss two-particle intensity interferometry as a method to extract from measured 1- and 2-particle momentum spectra information on the space-time geometry and dynamics of the particle emitting source. Particular attention is given to…
We employ Reconstruction of Attosecond Beating By Interference of Two-photon Transitions with an advanced energy resolution (rainbow RABBITT) to resolve under-threshold discrete excitations and above-threshold auto-ionizing states in the He…
This tutorial presents an introduction to the interaction of light and matter on the attosecond timescale. Our aim is to detail the theoretical description of ultra-short time-delays, and to relate these to the phase of extreme ultraviolet…
Transient absorption is a very powerful observable in attosecond experiments on atoms, molecules and solids and is frequently used in experiments employing phase-locked few-cycle infrared and XUV laser pulses derived from high harmonic…
We report on new routes to generating a train of attosecond pulses. The methods are extremely simple and robust; we need to place only a few thin dispersive materials in the optical path. We numerically demonstrate the generation of a train…
Different hypotheses about a quantum system such as the logical state of a qubit or the value of physical interaction parameters can be investigated by the interaction with a probe field. Such fields may be prepared in particularly…
We demonstrate the complete reconstruction of the electric field of visible-infrared pulses with energy as low as a few tens of nanojoules. The technique allows for the reconstruction of the instantaneous electric field vector direction and…
We propose a new technique to fully characterize the temporal structure of extreme ultraviolet pulses by ionizing a bound coherent electronic wavepacket. The populated energy levels make it possible to interfere different spectral…
We show that light-pulse atom interferometry with atomic point sources and spatially resolved detection enables multi-axis (two rotation, one acceleration) precision inertial sensing at long interrogation times. Using this method, we…
It is shown that, in the presence of correlations in particle emission, the measured HBT radii are related to the correlation range rather than to the size of the interaction volume. Only in the case of weak correlations the standard…