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In 5d transition metal oxides such as the iridates, novel properties arise from the interplay of electron correlations and spin-orbit interactions. We investigate the electronic structure of the pyrochlore iridates, (such as…

强关联电子 · 物理学 2015-05-19 Xiangang Wan , Ari Turner , Ashvin Vishwanath , Sergey Y. Savrasov

Angle-resolved photoemission measurements have been performed on Bi2Ir2O7 single crystals, a prototypical example of the pyrochlore iridates. The density of states, the Fermi surface, and the near Fermi level band dispersion in the plane…

强关联电子 · 物理学 2013-11-14 Q. Wang , Y. Cao , X. G. Wan , J. D. Denlinger , T. F. Qi , O. B. Korneta , G. Cao , D. S. Dessau

The interplay of spin-orbit interactions and electronic correlations dominates the physical properties of pyrochlore iridates, R2Ir2O7 (R = Y, rare earth element), which are typically magnetic insulators. We report an…

强关联电子 · 物理学 2015-06-03 T. F. Qi , O. B. Korneta , Xiangang Wan , L. E. DeLong , P. Schlottmann , G. Cao

Electrons in the pyrochore iridates experience a large interaction energy in addition to a strong spin-orbit interaction. Both features make the iridates promising for realizing novel states such as the Topological Mott Insulator. The…

强关联电子 · 物理学 2017-09-21 Tian Liang , Timothy H. Hsieh , Jun J. Ishikawa , Satoru Nakatsuji , Liang Fu , N. P. Ong

The magnetic properties of the pyrochlore iridate material Eu$_2$Ir$_2$O$_7$ (5$d^5$) have been studied based on the first principle calculations, where the crystal field splitting $\Delta$, spin-orbit coupling (SOC) $\lambda$ and Coulomb…

强关联电子 · 物理学 2017-11-08 Yilin Wang , Hongming Weng , Liang Fu , Xi Dai

We perform combined density functional and dynamical mean-field calculations to study the pyrochlore iridates Lu$_2$Ir$_2$O$_7$, Y$_2$Ir$_2$O$_7$ and Eu$_2$Ir$_2$O$_7$. Both single-site and cluster dynamical mean-field calculations are…

强关联电子 · 物理学 2017-01-27 Runzhi Wang , Ara Go , Andrew J. Millis

Non-Fermi liquid behavior in some fermionic systems have attracted significant interest in last few decades. Certain pyrochlore iridates with stronger spin-orbit coupling strength have recently been added to the list. Here, we provide…

Metal-insulator transitions in pyrochlore iridates (A2Ir2O7) are believed to occur due to subtle interplay of spin-orbit coupling, geometric frustration, and electron interactions. In particular, the nature of magnetic ordering of iridium…

强关联电子 · 物理学 2014-07-29 Eric Kin-Ho Lee , Subhro Bhattacharjee , Yong Baek Kim

Magnetic-rare-earth pyrochlore iridates exhibit a rich variety of unconventional phases, driven by the complex interactions within and between the rare-earth and the iridium sublattices. In this study, we investigate the peculiar magnetic…

We address the concomitant metal-insulator transition (MIT) and antiferromagnetic ordering in the novel pyrochlore iridate Eu2Ir2O7 by combining x-ray absorption spectroscopy, x-ray and neutron diffractions and density functional theory…

Novel phases of two dimensional electron systems resulting from new surface or interface modified electronic structures have generated significant interest in material science. We utilize photoemission spectroscopy to show that the…

We study the prototype 5d pyrochlore iridate Y2Ir2O7 from first principles using the local density approximation and dynamical mean-field theory (LDA+DMFT). We map out the phase diagram in the space of temperature, onsite Coulomb repulsion…

强关联电子 · 物理学 2015-10-14 Hiroshi Shinaoka , Shintaro Hoshino , Matthias Troyer , Philipp Werner

Geometrical frustration and spin-orbit coupling effect together play vital role to influence properties in pyrochlore based iridium oxides. Here we have investigated detailed structural, magnetic, thermodynamic and transport properties of…

强关联电子 · 物理学 2017-02-06 Harish Kumar , A. K. Pramanik

The magnetic ground states of $R_2$Ru$_2$O$_7$ and $A_2$Ru$_2$O$_7$ with $R=$ Pr, Gd, Ho, and Er, as well as $A=$ Ca, Cd are predicted devising a combination of the cluster-multipole (CMP) theory and spin-density-functional theory (SDFT).…

强关联电子 · 物理学 2022-02-22 Marie-Therese Huebsch , Yuske Nomura , Shiro Sakai , Ryotaro Arita

In the pyrochlore iridates, \textit{R}$_{2}$Ir$_{2}$O$_{7}$ (\textit{R} = Lanthanide, Y), determination of the magnetic structure of the iridium moments remains an outstanding problem despite the role this is expected to play in the…

强关联电子 · 物理学 2014-06-23 Steven M. Disseler

The $f$-$d$ magnetic exchange interaction is considered to be a key ingredient for many exotic topological phases in pyrochlore iridates. Here, we have investigated the evolution of structural, magnetic and electronic properties in doped…

强关联电子 · 物理学 2020-02-07 Harish Kumar , K. C. Kharkwal , Kranti Kumar , K. Asokan , A. Banerjee , A. K. Pramanik

A2Ir2O7 iridates were proven to crystallise in the geometrically frustrated pyrochlore structure, which remains stable upon rare-earth cation substitution, temperature variation, and external pressure application. However, the change of…

强关联电子 · 物理学 2024-08-05 Daniel Staško , Petr Proschek , Jiří Prchal , Milan Klicpera

The interplay between spin-orbit coupling (SOC) and electron correlation ($U$) is considered for many exotic phenomena in iridium oxides. We have investigated the evolution of structural, magnetic and electronic properties in pyrochlore…

强关联电子 · 物理学 2017-03-08 Harish Kumar , R. S. Dhaka , A. K. Pramanik

The electronic structure and magnetism of Sr$_2$CeIrO$_6$, an Ir-based double perovskite system has been investigated using first-principles calculations. We found that a strong spin-orbit coupling dictate the electronic and magnetic…

强关联电子 · 物理学 2013-01-29 S. K. Panda , I. Dasgupta

We report the low temperature properties of a new series of pyrochlore iridates R2Ir2O7 (R = rare-earth elements). We found that the compounds with R = Pr, Sm, Nd, and Eu exhibit metallic conductivity, whereas those with smaller rare-earth…

强关联电子 · 物理学 2009-11-07 D. Yanagishima , Y. Maeno
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