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We report on the optical spectroscopy of the spin of two magnetic atoms (Mn) embedded in an individual quantum dot interacting with either a single electron, a single exciton and single trion. As a result of their interaction to a common…

介观与纳米尺度物理 · 物理学 2015-06-05 L. Besombes , C. L. Cao , S. Jamet , H. Boukari , J. Fernandez-Rossier

We show that through the resonant optical excitation of spin-polarized excitons into CdMnTe magnetic quantum dots, we can induce a macroscopic magnetization of the Mn impurities. We observe very broad (4 meV linewidth) emission lines of…

软凝聚态物质 · 物理学 2009-11-10 T. Gurung , S. Mackowski , H. E. Jackson , L. M. Smith , W. Heiss , J. Kossut , G. Karczewski

A system of two coupled CdTe quantum dots, one of them containing a single Mn ion, was studied in continuous wave and modulated photoluminescence, photoluminescence excitation, and photon correlation experiments. Optical writing of…

其他凝聚态物理 · 物理学 2011-01-13 M. Goryca , T. Kazimierczuk , M. Nawrocki , A. Golnik , J. A. Gaj , P. Kossacki , P. Wojnar , G. Karczewski

Two electrons in a quantum dot (QD) can form triplet states. We analyze the exchange coupling of the triplet states of the negatively charged exciton in a QD (X$^-$, two electrons and one hole) with the spin of a magnetic atom (Mn). Two…

介观与纳米尺度物理 · 物理学 2023-07-12 L. Besombes , S. Ando , S. Kuroda , H. Boukari

The exciton recombination and spin dynamics in (In,Al)As/AlAs quantum dots (QDs) with indirect band gap and type-I band alignment are studied. The negligible (less than $0.2~\mu$eV) value of the anisotropic exchange interaction in these QDs…

介观与纳米尺度物理 · 物理学 2023-01-27 T. S. Shamirzaev , A. V. Shumilin , D. S. Smirnov , D. Kudlacik , S. V. Nekrasov , Yu. G. Kusrayev , D. R. Yakovlev , M. Bayer

We use the spin-polarized excitons in a single quantum dot to design optical controls for basic operations in quantum computing. We examine the ultrafast nonlinear optical processes required and use the coherent nonlinear optical responses…

介观与纳米尺度物理 · 物理学 2009-10-31 Pochung Chen , C. Piermarocchi , L. J. Sham

Optical control of the spin coherence of quantum well electrons by short laser pulses with circular or linear polarization is studied experimentally and theoretically. For that purpose the coherent electron spin dynamics in a n-doped…

介观与纳米尺度物理 · 物理学 2010-09-15 E. A. Zhukov , D. R. Yakovlev , M. M. Glazov , L. Fokina , G. Karczewski , T. Wojtowicz , J. Kossut , M. Bayer

We demonstrate that the spin of a Cr atom in a quantum dot (QD) can be controlled optically and we discuss the main properties of this single spin system. The photoluminescence of individual Cr-doped QDs and their evolution in magnetic…

介观与纳米尺度物理 · 物理学 2019-11-27 L. Besombes , H. Boukari , V. Tiwari , A. Lafuente-Sampietro , S. Kuroda , K. Makita

A photo-excited II-VI semiconductor nanocrystal doped with a few Mn spins is considered. The effects of spin-exciton interactions and the resulting multi-spin correlations on the photoluminescence are calculated by numerical diagonalization…

介观与纳米尺度物理 · 物理学 2009-11-11 J. Fernández-Rossier

The spin-flip rate that couples dark and bright excitons in self-assembled quantum dots is obtained from time-resolved spontaneous emission measurements in a modified local density of optical states. Employing this technique, we can…

其他凝聚态物理 · 物理学 2010-03-18 Jeppe Johansen , Brian Julsgaard , Søren Stobbe , Jørn M. Hvam , Peter Lodahl

The electron and hole states in a CdTe quantum dot containing a single magnetic impurity in an external magnetic field are investigated, using the multiband approximation which includes the heavy hole-light hole coupling effects. The…

介观与纳米尺度物理 · 物理学 2010-08-10 Aram Manaselyan , Tapash Chakraborty

The optically induced spin dynamics of a single Mn atom embedded into a single semiconductor quantum dot can be strongly influenced by using the optical Stark effect. The exchange interaction gives rise to simultaneous spin flips between…

介观与纳米尺度物理 · 物理学 2013-05-24 D. E. Reiter , V. M. Axt , T. Kuhn

The spin structure and spin dynamics of excitons in an ensemble of (In,Al)As/AlAs quantum dots (QDs) with type-I band alignment, containing both direct and indirect band gap dots, are studied. Time-resolved and spectral selective techniques…

介观与纳米尺度物理 · 物理学 2019-05-15 J. Rautert , T. S. Shamirzaev , S. V. Nekrasov , D. R. Yakovlev , P. Klenovský , Yu. G. Kusrayev , M. Bayer

Using the emission of the positively charged exciton as a probe, we analyze the dynamics of the optical pumping and the dynamics of the relaxation of a Mn spin exchange-coupled with a confined hole spin in a II-VI semiconductor quantum dot.…

介观与纳米尺度物理 · 物理学 2015-06-22 B. Varghese , H. Boukari , L. Besombes

The spin dynamics of a single Mn atom in a laser driven CdTe quantum dot is addressed theoretically. Recent experimental results\cite{Le-Gall_PRL_2009,Goryca_PRL_2009,Le-Gall_PRB_2010}show that it is possible to induce Mn spin polarization…

介观与纳米尺度物理 · 物理学 2015-05-28 C. L. Cao , L. Besombes , J. Fernández-Rossier

We report on the spin properties of individual Mn atoms in II-VI semiconductor strain free quantum dots. Strain free Mn-doped CdTe quantum dots are formed by width fluctuations in thin quantum wells lattice matched on a CdTe substrate.…

介观与纳米尺度物理 · 物理学 2015-06-18 L. Besombes , H. Boukari

We provide a theoretical description of the optical orientation of a single Mn$^{2+}$ ion spin under quasi-resonant excitation demonstrated experimentally by Goryca et al. [Phys. Rev. Lett. 103, 087401 (2009)]. We build and analyze a…

介观与纳米尺度物理 · 物理学 2018-02-14 T. Smoleński , Ł. Cywiński , P. Kossacki

Excitons in diluted magnetic semiconductors represent excellent probes for studying the magnetic properties of these materials. Various magneto-optical effects, which depend sensitively on the exchange interaction of the excitons with the…

In order to explain the recently observed phenomenon of optical orientation of a single Mn spin residing inside a quantum dot, a process of Mn spin relaxation with characteristic timescale of tens of nanoseconds had been invoked. We show…

介观与纳米尺度物理 · 物理学 2010-08-24 Lukasz Cywinski

We report on the micro-photoluminescence spectroscopy of InAs/GaAs quantum dots (QD) doped by a single Mn atom in a magnetic field either longitudinal or perpendicular to the optical axis. In both cases the spectral features of positive…

材料科学 · 物理学 2015-05-14 Olivier Krebs , Emile Benjamin , Aristide Lemaître
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