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High-order harmonic generation (HHG) from aligned acetylene molecules interacting with mid infra-red (IR), linearly polarized laser pulses is studied theoretically using a mixed quantum-classical approach in which the electrons are…

原子物理 · 物理学 2018-05-18 Peter Mulholland , Daniel Dundas

The degree of elliptical polarization of intense short laser pulses is shown to be related to the timing of strong-field non-sequential double ionization. Higher ellipticity is predicted to force the initiation of double ionization into a…

原子物理 · 物理学 2010-08-20 Xu Wang , J. H. Eberly

We predict high-order harmonics in which the polarization within the spectral bandwidth of each harmonic varies continuously and significantly. For example, the interaction of counter-rotating circularly-polarized bichromatic drivers having…

光学 · 物理学 2014-10-24 Avner Fleischer , Ofer Kfir , Pavel Sidorenko , Oren Cohen

Present photoionization experiments cannot measure molecular frame photoelectron angular distributions (MFPAD) from the outermost valence electrons of molecules. We show that details of the MFPAD can be retrieved with high-order harmonics…

原子物理 · 物理学 2009-05-24 Anh-Thu Le , R. R. Lucchese , M. T. Lee , C. D. Lin

The role of the Coulomb potential on the generation of elliptically polarized high-order harmonics from atoms driven by elliptically polarized laser is investigated analytically. It is found that the Coulomb effect makes a contribution to…

原子物理 · 物理学 2013-03-05 Xiaosong Zhu , Meiyan Qin , Qingbin Zhang , Weiyi Hong , Zhizhan Xu , Peixiang Lu

We present a theoretical analysis of high-order harmonic generation from ion-atom collisions in the presence of linearly polarized intense laser pulses. Photons with frequencies significantly higher than in standard atomic high-harmonic…

原子物理 · 物理学 2009-11-10 Manfred Lein , Jan M. Rost

We study high-order harmonic generation in aligned molecules close to the ionization threshold. Two distinct contributions to the harmonic signal are observed, which show very different responses to molecular alignment and ellipticity of…

原子物理 · 物理学 2011-09-16 H. Soifer , P. Botheron , D. Shafir , A. Diner , O. Raz , B. D. Bruner , Y. Mairesse , B. Pons , N. Dudovich

We report on experimental and theoretical investigations of the polarization dependence of magnetic resonance generated by synchronous optical pumping. Magnetic resonances with narrow linewidth are generated experimentally using a rubidium…

原子物理 · 物理学 2020-09-09 Raghwinder Singh Grewal , Gour Pati , Renu Tripathi

We investigate high-order harmonic spectra from aligned diatomic molecules in intense driving fields whose components have orthogonal polarizations. We focus on how the driving-field ellipticity influences structural interference patterns…

The generation of high harmonics is a strongly nonlinear effect that allows to probe properties of the target and to study electron dynamics in matter. It has been investigated in many different kinds of targets, including molecular gases,…

量子物理 · 物理学 2026-05-06 Lina Bielke , Samuel Schöpa , Falk-Erik Wiechmann , Franziska Fennel , Dieter Bauer

We study numerically the interaction between an intense circularly polarized laser field and an electron moving in a potential which has a discrete cylindrical symmetry with respect to the laser pulse propagation direction. This setup…

原子物理 · 物理学 2009-11-07 F. Ceccherini , D. Bauer

The generation of harmonics by atoms or ions in a two-color, coplanar field configuration with commensurate frequencies is investigated through both, an analytical calculation based on the Lewenstein model and the numerical ab initio…

原子物理 · 物理学 2009-11-07 F. Ceccherini , D. Bauer , F. Cornolti

We show that circularly polarized femtosecond laser pulses produce field-free alignment in linear and planar molecules. We study the rotational wavepacket evolution of O$_2$ and benzene created by circularly polarized light. For benzene, we…

化学物理 · 物理学 2014-06-06 C T L Smeenk , P B Corkum

We present a theoretical model of high-harmonic generation from diatomic molecules. The theory includes effects of alignment as well as nuclear motion and is used to predict results for N$_2$, O$_2$, H$_2$ and D$_2$. The results show that…

原子物理 · 物理学 2007-05-23 Christian Bruun Madsen , Lars Bojer Madsen

We show that a linear molecule subjected to a short specific elliptically polarized laser field yields postpulse revivals exhibiting alignment alternatively located along the orthogonal axis and the major axis of the ellipse. The effect is…

量子物理 · 物理学 2007-05-23 D. Daems , S. Guérin , E. Hertz , H. R. Jauslin , B. Lavorel , O. Faucher

Based upon our previous works (Eur.Phys.J.D 6, 319(1999); Chin.Phys.Lett. 18, 236(2001)), we develop a classical approach to calculate the high-order harmonic generation of the laser driven atoms and molecules. The Coulomb singularities in…

原子物理 · 物理学 2007-05-23 Chaohong Lee , Yiwu Duan , Wing-Ki Liu , Jian-Min Yuan , Lei Shi , Xiwen Zhu , Kelin Gao

The method proposed in [I.R. Khairulin et al., JETP Letters 117(9), 652 (2023)] for converting the linearly polarized radiation of high-order harmonics of an optical field into the circularly polarized in an optically modulated active…

光学 · 物理学 2024-08-20 Vladimir A. Antonov , Ilias R. Khairulin , Mikhail Yu. Ryabikin

The use of bichromatic counter-rotating laser field is known to generate high-order harmonics with non-zero ellipticity. By combining such laser field with a plasmonic-enhanced spatially inhomogeneous field, we propose a way to influence…

Ultrafast extreme ultraviolet (XUV) sources with a controllable polarization state are powerful tools for investigating the structural and electronic as well as the magnetic properties of materials. However, such light sources are still…

等离子体物理 · 物理学 2016-08-18 Zi-Yu Chen , Alexander Pukhov

We consider the formation of RbCs by an elliptically polarized laser pulse. By varying the ellipticity of the laser for sufficiently large laser intensity, we see that the formation probability presents a strong dependence, especially…

原子物理 · 物理学 2019-02-06 J. Pablo Salas , Cristel Chandre , J Salas