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Charge separation in light-harvesting complexes occurs in a pair of tightly coupled chlorophylls at the heart of photosynthetic reaction centers of both plants and bacteria. Recently it has been shown that quantum coherence can, in…

生物物理 · 物理学 2016-11-28 M. Qin , H. Z Shen , X. X. Yi

The molecular photo cell, i.e., a single molecule donor-acceptor complex, beside being technologically important, is a paradigmatic example of a many-body system operating in strong non-equilibrium. The quantum transport and the…

介观与纳米尺度物理 · 物理学 2020-07-06 Subhajit Sarkar , Yonatan Dubi

Transition-metal-oxide (TMO) heterostructures are promising candidates for building photon-harvesting devices which can exploit optimal quantum transport of charge excitations generated by light absorption. Here we address the explicit role…

量子物理 · 物理学 2020-04-22 Chahan M. Kropf , G. Luca Celardo , Claudio Giannetti , Fausto Borgonovi

We report some basic results regarding transport in disordered reaction-diffusion systems with birth (A->2A), death (A->0), and binary competition (2A->A) processes. We consider a model in which the growth process is only allowed to take…

无序系统与神经网络 · 物理学 2008-02-04 Andrew R. Missel , Karin A. Dahmen

Giant strides in ultrashort laser pulse technology have enabled real-time observation of dynamical processes in complex molecular systems. Specifically, the discovery of oscillatory transients in the two-dimensional electronic spectra of…

化学物理 · 物理学 2021-03-08 Akihito Ishizaki , Graham R. Fleming

The extent of exciton coherence in protein-pigment complexes has significant implications for the initial light harvesting step in photosynthetic organisms. In this work we model the main antenna protein of photosystem II, namely light…

其他凝聚态物理 · 物理学 2008-12-09 Jiahao Chen , Nancy Makri

The non-equilibrium stationary coherences that form in donor-acceptor systems are investigated to determine their relationship to the efficiency of energy transfer to a neighboring reaction center. It is found that the effects of asymmetry…

化学物理 · 物理学 2020-07-03 Kenneth A. Jung , Paul Brumer

We analyze the translocation of a charged particle across an Alpha-Hemolysin (aHL) pore in the framework of a driven diffusion over an extended energy barrier generated by the electrical charges of the aHL. A one-dimensional electrostatic…

生物大分子 · 定量生物学 2015-10-15 Patrizio Ansalone , Mauro Chinappi , Lamberto Rondoni , Fabio Cecconi

Fenna-Matthews-Olson (FMO) bacteriochlorophylls (BChls) are molecules responsible of the high efficiency energy transfer in the photosynthetic process of green sulfur bacteria, controversially associated to quantum phenomena of long lived…

化学物理 · 物理学 2020-08-19 Bruno González-Soria , Francisco Delgado , Alan Anaya-Morales

In this thesis we derive a hydrodynamical model to describe the dynamics of density excitations localized at the edges of a Quantum Hall bar. In particular we show that the chiral Luttinger liquid model for the edges excitations can be…

介观与纳米尺度物理 · 物理学 2007-05-23 Roberto D'Agosta

Type-II heterostructures (HSs) are essential components of modern electronic and optoelectronic devices. Earlier studies have found that in type-II transition metal dichalcogenide (TMD) HSs, the dominating carrier relaxation pathway is the…

Signal transduction in biological cells is effected by signaling pathways that typically include multiple feedback loops. Here we analyze information transfer through a prototypical signaling module with biochemical feedback. The module…

生物物理 · 物理学 2015-11-06 Gerardo Aquino , Martin Zapotocky

A variety of open quantum networks are currently under intense examination to model energy transport in photosynthetic systems. Here we study the coherent transfer of a quantum excitation over a network incoherently coupled with a…

量子物理 · 物理学 2015-03-18 Lorenzo Campos Venuti , Paolo Zanardi

The recently suggested possibility that weak vibronic transitions can be excitonically enhanced in light-harvesting complexes is studied in detail. A vibronic exciton dimer model which includes ground state vibrations is investigated using…

化学物理 · 物理学 2014-10-09 Jan Schulze , Magne Torbjörnsson , Oliver Kühn , Tõnu Pullerits

The possibility of using single molecule junctions as electron pumps for energy conversion and storage is considered. It is argued that the small dimensions of these systems enable to make use of unique intra-molecular quantum coherences in…

量子物理 · 物理学 2015-05-20 Roie Volkovich , Uri Peskin

Excited-state charge-transfer complexes (exciplexes) have been actively exploited in organic optoelectronic devices to improve performance; however, diffusion of exciplexes has not been actively studied despite its influence on performance…

材料科学 · 物理学 2019-06-25 Hwang-Beom Kim , Jang-Joo Kim

Dissipation is a common occurrence in real-world systems and is generally considered to be detrimental to transport. In this study, we examine the transport properties of a narrow quantum anomalous Hall system with dissipation applied on…

介观与纳米尺度物理 · 物理学 2024-04-02 Ming Lu , Xue-Zhu Liu , Hailong Li , Zhi-Qiang Zhang , Jie Liu , X. C. Xie

Quantum--Mechanical methods that are both computationally fast and accurate are not yet available for electronic excitations having charge transfer character. In this work, we present a significant step forward towards this goal for those…

化学物理 · 物理学 2015-06-12 Michele Pavanello , Troy Van Voorhis , Lucas Visscher , Johannes Neugebauer

We study the effect of density-assisted hopping on different dimerized lattice geometries, such as bilayers and ladder structures. We show analytically that the density-assisted hopping induces an attractive interaction in the lower…

强关联电子 · 物理学 2026-03-10 Franco T. Lisandrini , Edmond Orignac , Roberta Citro , Ameneh Sheikhan , Corinna Kollath

The interaction between molecules and surface plasmons in defined geometries can lead to new light mater hybrid states where light propagation is strongly influenced by molecular photon absorption. Their application range from lasing LEDs…