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We perform a time-resolved optical study of Sr$_2$IrO$_4$ to understand the influence of magnetic ordering on the low energy electronic structure of a strongly spin-orbit coupled $J_{eff}$=1/2 Mott insulator. By studying the recovery…

强关联电子 · 物理学 2012-03-21 D. Hsieh , F. Mahmood , D. H. Torchinsky , G. Cao , N. Gedik

We have investigated the temperature evolution of magnetism and its interrelation with structural parameters in perovskite-based layered compound Sr$_2$IrO$_4$, which is believed to be a $J_{eff}$ = 1/2 Mott insulator. The structural…

强关联电子 · 物理学 2014-12-15 Imtiaz Noor Bhatti , R. Rawat , A. Banerjee , A. K. Pramanik

Based on the microscopic model including strong spin-orbit coupling, on-site Coulomb and Hund's interactions, as well as crystal field effects, we have investigated magnetic and optical properties of Sr2IrO4. Taking into account all…

强关联电子 · 物理学 2012-12-11 Beom Hyun Kim , G. Khaliullin , B. I. Min

We use scanning tunneling microscopy to study the temperature evolution of electronic structure in Ca3Cu2O4Cl2 parent Mott insulator of cuprates. We find that the upper Hubbard band moves towards the Fermi energy with increasing…

强关联电子 · 物理学 2021-12-28 Li Haiwei , Ye Shusen , Zhao Jianfa , Jin Changqing , Yayu Wang

Stoichiometric Sr2IrO4 is a ferromagnetic Jeff = 1/2 Mott insulator driven by strong spin-orbit coupling. Introduction of very dilute oxygen vacancies into single-crystal Sr2IrO4-delta with delta < 0.04 leads to significant changes in…

强关联电子 · 物理学 2010-08-30 O. B. Korneta , Tongfei Qi , S. Chikara , S. Parkin L. E. De Long , P. Schlottmann , G. Cao

We investigated Ru-doped single-crystal 5$d$ iridiates, Sr$_2$Ir$_{1-x}$Ru$_x$O$_{4}$, at three different doping concentrations ($x =$ 0.01, 0.07 and 0.10) using optical spectroscopy. The undoped pristine compound (Sr$_2$IrO$_{4}$) is known…

We report the complex dielectric function along and perpendicular to the IrO2 planes in the layered perovskite Sr2IrO4 determined by spectroscopic ellipsometry in the spectral range from 12 meV to 6 eV. Thin high quality single crystals…

We employ molecular beam epitaxy to stabilize Ba2IrO4 thin films and utilize in situ angle-resolved photoemission spectroscopy to investigate the evolution of its electronic structure through the Neel temperature TN. Our measurements…

强关联电子 · 物理学 2015-06-22 M. Uchida , Y. F. Nie , P. D. C. King , C. H. Kim , C. J. Fennie , D. G. Schlom , K. M. Shen

We have investigated the electronic structure of Sr2IrO4 within the density-functional theory using the generalized gradient approximation while taking into account strong Coulomb correlations in the framework of the fully relativistic…

强关联电子 · 物理学 2023-10-13 V. N. Antonov , D. A. Kukusta , L. V. Bekenov

We investigate the detailed electronic structure of PrCoO$_3$ and its temperature evolution using state-of-the-art photoemission spectroscopy and ab initio band structure calculations. We observe that in addition to the correlation effect,…

强关联电子 · 物理学 2009-11-13 S. K. Pandey , Swapnil Patil , V. R. R. Medicherla , R. S. Singh , Kalobaran Maiti

Layered 5d transition metal oxides (TMOs) have attracted significant interest in recent years because of the rich physical properties induced by the interplay between spin-orbit coupling, bandwidth and on-site Coulomb repulsion. In Sr2IrO4,…

We have investigated the excitation spectra of $j_{eff}$=$\frac{1}{2}$ Mott insulator Na$_2$IrO$_3$. Taking into account a relativistic multiplet structure of Ir ions, we have calculated the optical conductivity $\sigma(\omega)$ and…

强关联电子 · 物理学 2014-02-25 Beom Hyun Kim , G. Khaliullin , B. I. Min

We examined the temperature (T) evolution of the optical conductivity spectra of Sr$_3$Ir$_2$O$_7$ over a wide range of 10-400 K. The system was barely insulating, exhibiting a small indirect bandgap of $\sim$0.1 eV. The low-energy features…

强关联电子 · 物理学 2015-06-18 H. J. Park , C. H. Sohn , D. W. Jeong , G. Cao , K. W. Kim , S. J. Moon , Hosub Jin , Deok-Yong Cho , T. W. Noh

Sr2IrO4 hosts a novel Jeff =1/2 Mott state and quasi-two-dimensional antiferromagnetic order, providing a unique avenue of exploring emergent states of matter and functions that are extraordinarily sensitive to any structural variations.…

强关联电子 · 物理学 2023-09-19 H. W. Wang , L. Y. Zhang , N. Hu , B. You , Y. T. Chang , S. L. Yuan , C. L. Lu , J. M. Liu

The electronic band structure can change with temperature in Mott and Kondo insulators, even without a phase transition. Here, to clarify the underlying mechanism, the spectral function at nonzero temperature is studied. By considering…

强关联电子 · 物理学 2023-11-10 Masanori Kohno

Sr$_2$IrO$_4$ has attracted a lot of attention due to its structural and electronic similarities to La$_2$CuO$_4$ which is the parent compound of high-T$_c$ superconducting cuprates. It was proposed to be a strong spin-orbit coupled…

The low-energy electronic structure of the J_{eff}=1/2 spin-orbit insulator Sr3Ir2O7 has been studied by means of angle-resolved photoemission spectroscopy. A comparison of the results for bilayer Sr3Ir2O7 with available literature data for…

Sr2IrO4 and Sr3Ir2O7 form two families of spin-orbit Mott insulators with quite different charge gaps and an antiferromagnetic (AF) ground state. This offers a unique opportunity to study the impact of long-range magnetic order in Mott…

Compounds with intermediate-size transition metals such as Fe or Mn are close to the transition between charge-transfer systems and Mott-Hubbard systems. We study the optical conductivity \sigma(\omega) of insulating layered LaSrFeO_4 in…

强关联电子 · 物理学 2014-05-08 J. Reul , L. Fels , N. Qureshi , K. Shportko , M. Braden , M. Grüninger

With optical spectroscopy we provide evidence that the insulator-metal transition in Sr$_2$Ir$_{1-x}$Rh$_{x}$O$_{4}$ occurs close to a crossover from the Mott- to the Slater-type. The Mott-gap at $x = 0$ persists to high temperature and…

强关联电子 · 物理学 2020-01-17 B. Xu , P. Marsik , E. Sheveleva , F. Lyzwa , A. Louat , V. Brouet , D. Munzar , C. Bernhard
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