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Theoretical and computational results are presented clarifying the role of long-ranged strain interactions in determining the charge and orbital ordering in colossal magnetoresistance manganites. The strain energy contribution is found to…

强关联电子 · 物理学 2009-11-10 M. J. Calderon , A. J. Millis , K. H. Ahn

A short introduction to the complex phenomena encountered in transition metal oxides with either charge or orbital or joint charge-and-orbital order, usually accompanied by magnetic order, is presented. It is argued that all the types of…

强关联电子 · 物理学 2022-01-27 Andrzej M. Oles

A comprehensive analysis of half-doped manganites is presented using Monte Carlo simulations applied to the double-exchange model with cooperative Jahn-Teller lattice distortions in two dimensions. A variety of novel results are reported:…

强关联电子 · 物理学 2009-11-10 H. Aliaga , D. Magnoux , A. Moreo , D. Poilblanc , S. Yunoki , E. Dagotto

Whenever a symmetry in the ground state of a system is broken, topological defects will exist. These defects are essential for understanding phase transitions in low dimensional systems[1]. Excitingly in some unique condensed matter systems…

材料科学 · 物理学 2009-11-11 Luis Brey , P. B. Littlewood

We use resonant X-ray scattering at the nickel L$_{2,3}$ edges to investigate the interplay between orbital degrees of freedom and charge density waves (CDW) in the superconductor BaNi$_2$(As$_{1-x}$P$_x$)$_2$. Both the incommensurate and…

In the manganite Nd0.5Ca0.5MnO3, charge ordering occurs at much higher temperature than the antiferromagnetic order (TCO=250K,TN=160K). The magnetic behavior of the phase TN<T<TCO is puzzling: its magnetization and susceptibility are…

强关联电子 · 物理学 2016-08-31 F. millange , S. de Brion , G. Chouteau

The nature of orbital order-disorder transition has been studied in the La(1-x)Nd(x)MnO(3) (x = 0.0-1.0) series which covers the entire range between two end points - LaMnO(3) and NdMnO(3) - as well as in La(0.85)Nd(0.1)Sr(0.05)MnO(3) and…

强关联电子 · 物理学 2009-11-10 Dipten Bhattacharya , P. Sujatha Devi , H. S. Maiti

An electronic effect on a macroscopic domain structure is found in a strongly correlated half-doped manganite film Nd$_{0.5}$Sr$_{0.5}$MnO3 grown on a (011) surface of SrTiO3. The sample has a high-temperature (HT) phase free from…

强关联电子 · 物理学 2011-03-01 Y. Wakabayashi , H. Sagayama , T. Arima , M. Nakamura , Y. Ogimoto , Y. Kubo , K. Miyano , H. Sawa

We apply grazing-incidence femtosecond x-ray diffraction to investigate the details of the atomic motion connected with a displacively excited coherent optical phonon. We concentrate on the low frequency phonon associated with the charge…

The exchange interactions and magnetic structure in layered system CuMnO2 (mineral crednerite) and in nonstoichiometric system Cu1.04Mn0.96O2, with triangular layers distorted due to orbital ordering of the Mn3+ ions, are studied by…

强关联电子 · 物理学 2014-01-21 A. V. Ushakov , S. V. Streltsov , D. I. Khomskii

Synchrotron x-ray scattering measurements of the low-temperature structure of the single-layer manganese oxide La$_{1-x}$Sr$_{1+x}$MnO$_4$, over the doping range $0.33 \le x \le 0.67$, indicate the existence of three distinct regions: a…

强关联电子 · 物理学 2009-11-07 S. Larochelle , A. Mehta , N. Kaneko , P. K. Mang , A. F. Panchula , L. Zhou , J. Arthur , M. Greven

In complex electronic materials, coupling between electrons and the atomic lattice gives rise to remarkable phenomena, including colossal magnetoresistance and metal-insulator transitions. Charge-ordered phases are a prototypical…

We report an x-ray scattering study of octahedral tilt ordering in the manganite series Pr$_{1-x}$Ca$_x$MnO$_3$ with x=0.4 and 0.25 and in LaMnO$_3$. The sensitivity to tilt ordering is achieved by tuning the incident x-ray energy to the…

We present a $^{209}$Bi and $^{17}$O NMR study of the Mn electron spin correlations developed in the charge ordered state of Bi$_{0.5}$Sr$_{0.5}$MnO$_{3}$ and Bi$_{0.5}$Ca$_{0.5}$MnO$_{3}$. The unusually large local magnetic field…

The phase diagram of $Pr_{1-x}Ca_xMnO_3$ is modified x $\le$ 0.3, which suggests a reevaluation of the phase diagram of other manganites in that doping region. Rather than an orbital ordered phase reaching up to high temperatures of…

We report the effect of Mn site substitution of Al on the structural, magnetic and transport properties of charge ordered Pr{_0.5}Ca{_0.5}MnO{_3}. This substitution introduces impurities in the Mn-O-Mn network, causes the Mn{^3+}/Mn{^4+}…

凝聚态物理 · 物理学 2007-05-23 Sunil Nair , A. Banerjee

The standard way to find the orbital occupation of Jahn-Teller (JT) ions is to use structural data, with the assumption of a one-to-one correspondence between the orbital occupation and the associated JT distortion, e.g. in O6 octahedron.…

We report on the ultrafast dynamics of charge order and structural response during the photoinduced suppression of charge and orbital order in a mixed-valence manganite. Employing femtosecond time-resolved resonant x-ray diffraction below…

A system of strongly-interacting electron-lattice polarons can exhibit charge and orbital order at sufficiently high polaron concentrations. In this study, the structure of short-range polaron correlations in the layered colossal…

In the mixed-valence manganites, a near-infrared laser typically melts the orbital and spin order simultaneously, corresponding to the photoinduced $d^{1}d^{0}$ $\xrightarrow{}$ $d^{0}d^{1}$ excitations in the Mott-Hubbard bands of…