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The phase diagrams of LaMnO$_3$ perovskites have been intensely studied due to the colossal magnetoresistance (CMR) exhibited by compositions around the $\frac{3}{8}^{th}$ doping level. However, phase segregation between ferromagnetic (FM)…

The coupling of multiple degrees of freedom - charge, spin, and lattice - in manganites has mostly been considered at the microscopic level. However, on larger length scales, these correlations may be affected by strain and disorder, which…

强关联电子 · 物理学 2007-09-25 J. J. Turner , K. J. Thomas , J. P. Hill , M. Pfeifer , K. Chesnel , Y. Tomioka , Y. Tokura , S. D. Kevan

The evolution of charge and orbital ordering phenomena in optimally-doped \textit{RE}\textsubscript{5/8}Ca\textsubscript{3/8}MnO\textsubscript{3} (RECMO, \textit{RE} $=$ rare-earth) manganite perovskites has been investigated through…

强关联电子 · 物理学 2024-09-04 Ben R. M. Tragheim , Clemens Ritter , Mark S. Senn

Phase diagrams in the plane of $r_A$ (the average ionic radius, related to one-electron bandwidth $W$) and $\sigma^2$ (the ionic radius variance, measuring the quenched disorder), or ``bandwidth-disorder phase diagrams'', have been…

材料科学 · 物理学 2007-05-23 R. Mathieu , M. Uchida , Y. Kaneko , J. P. He , X. Z. Yu , R. Kumai , T. Arima , Y. Tomioka , A. Asamitsu , Y. Matsui , Y. Tokura

Structural study of orbital-ordered manganite thin films has been conducted using synchrotron radiation, and a ground state electronic phase diagram is made. The lattice parameters of four manganite thin films, Nd0.5Sr0.5MnO3 (NSMO) or…

强关联电子 · 物理学 2011-03-08 Y. Wakabayashi , D. Bizen , Y. Kubo , H. Nakao , Y. Murakami , M. Nakamura , Y. Ogimoto , K. Miyano , H. Sawa

The three dimensional perovskite manganites in the range of hole-doping $x > 0.5$ are studied in detail using a double exchange model with degenerate $e_g$ orbitals including intra- and inter-orbital correlations and near-neighbour Coulomb…

强关联电子 · 物理学 2009-11-10 Tulika Maitra , A. Taraphder

Self-interaction corrected local spin density approximation calculations were performed for La$_{(1-x)}$Sr$_x$MnO$_3$ (LSMO) ($0.0<x<0.5$). The influence and inter-relationship of Sr doping, magnetic structure, O displacements and phase…

强关联电子 · 物理学 2009-11-10 G. Banach , W. M. Temmerman

We have performed powder neutron diffraction on $^7$Li-enriched sample of LiMn$_2$O$_4$ at 300 K. The crystal structure determined by Rietveld analysis is a cubic spinel with space group of $Fd\bar{3}m$ in which all Mn atoms are…

The magnetic and orbital orders for the bilayer manganites in the doping region $0.5 < x <1.0$ have been investigated from a model that incorporates the two $e_g$ orbitals at each Mn site, the inter-orbital Coulomb interaction and lattice…

强关联电子 · 物理学 2009-11-10 Tulika Maitra , A. Taraphder

Based on the Hamiltonian of small polarons with the strong nearest neighbor repulsion, we have investigated the charge ordering phenomena observed in half-doped manganites R_{1/2}A_{1/2}MnO_3. We have explored possible consequences of the…

凝聚态物理 · 物理学 2009-10-30 J. D. Lee , B. I. Min

We studied the charge-orbital ordering in the superlattice of charge-ordered insulating Pr$_{0.5}$Ca$_{0.5}$MnO$_3$ and ferromagnetic metallic La$_{0.5}$Sr$_{0.5}$MnO$_3$ by resonant soft x-ray diffraction. A temperature-dependent…

强关联电子 · 物理学 2014-08-07 H. Wadati , J. Okamoto , M. Garganourakis , V. Scagnoli , U. Staub , M. Nakamura , M. Kawasaki , Y. Tokura

Magnetic structures and the relationship between spin and charge-orbital orderings of an A-site ordered double-perovskite manganite SmBaMn2O6, an anticipated multiferroic material, were investigated by means of neutron diffraction. The spin…

Charge-lattice fluctuations are observed in the layered perovskite manganite LaSr2Mn2O7 by Raman spectroscopy as high as 340 K and with decreasing temperature they become static and form a charge ordered (CO) phase below TCO=210 K. In the…

We present a total energy study as a function of volume in the cubic phase of LaMnO$_{3}$. A charge disproportionated state into planes of Mn$^{3+}$O$_{2}$/Mn$^{4+}$O$_{2}$ was found. It is argued that the pressure driven…

强关联电子 · 物理学 2009-11-10 G. Banach , W. M. Temmerman

Taking the orbital degeneracy of $e_g$ conduction bands and the Coulomb interaction into account in a double-exchange model, we investigate charge dynamics of perovskite Mn oxides by the Lancz$\ddot{\rm o}$s diagonalization method. In the…

强关联电子 · 物理学 2009-10-31 Hiroki Nakano , Yukitoshi Motome , Masatoshi Imada

The roles of crystal-field splitting and Jahn-Teller distortions on the orbital ordering transition are investigated in the single-layer manganites near half doping. Crystal-field splitting of energy levels favoring the $d_{3z^2-r^2}$…

强关联电子 · 物理学 2017-06-29 Dheeraj Kumar Singh , Tetsuya Takimoto

In layered manganites with orbital and charge orderings, the degeneracy of the Mn $4p$ orbitals as well as the $3d$ ones is lifted by the effects of the $4p$ bands and the local Coulomb interactions. We formulate the atomic scattering…

强关联电子 · 物理学 2009-10-31 Sumio Ishihara , Sadamichi Maekawa

The competition of charge, orbital, and ferromagnetic interactions in layered manganites is investigated by magneto-Raman scattering spectroscopy. We find that the colossal magnetoresistance effect in the layered compounds results from the…

强关联电子 · 物理学 2009-10-31 D. B. Romero , Y. Moritomo , J. F. Mitchell , H. D. Drew

Charge and orbital ordering in the low-temperature monoclinic structure of magnetite (Fe_3O_4) is investigated using LSDA+U. While the difference between t_{2g} minority occupancies of Fe^{2+}_B and Fe^{3+}_B cations is large and gives…

强关联电子 · 物理学 2016-11-02 I. Leonov , A. N. Yaresko , V. N. Antonov , M. A. Korotin , V. I. Anisimov

It is proposed that the observation of orbital ordering in manganite materials should be possible at the L_II and L_III edges of manganese using X-ray resonant scattering. If performed, dipole selection rules would make the measurements…

凝聚态物理 · 物理学 2009-10-31 C. W. M. Castleton , M. Altarelli