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We report calculations of the high-order harmonic spectra of few-atomic clusters of two noble gases, helium and krypton, subjected to laser pulses of intensities above $10^{13}$ W/cm\textsuperscript{2}. We employ a fully \textit{ab intio}…

化学物理 · 物理学 2023-12-05 Aleksander P. Woźniak , Robert Moszyński

Double photoelectron emission from He atoms by intense laser pulses with a wave length of $394.5\,nm$ is computed for intensities $3.5 - 9.2\times 10^{14}W/cm^2$. Joint momentum distributions confirm the characteristics seen in classical…

原子物理 · 物理学 2020-07-01 Jinzhen Zhu , Armin Scrinzi

High-order harmonic generation (HHG) from aligned acetylene molecules interacting with mid infra-red (IR), linearly polarized laser pulses is studied theoretically using a mixed quantum-classical approach in which the electrons are…

原子物理 · 物理学 2018-05-18 Peter Mulholland , Daniel Dundas

An accurate analytic model describing high-harmonic generation (HHG) in solids is derived. Extensive first-principles simulations within a time-dependent density-functional framework corroborate the conclusions of the model. Our results…

High-harmonic generation (HHG) spectrum from a LiH molecule induced by an intense laser pulse is computed and analyzed with potential energy surfaces for electron motion (ePES) constructed from a model of localized electron wave packets…

化学物理 · 物理学 2020-03-18 Koji Ando

When a high power laser beam irradiates a small aperture on a solid foil target, the strong laser field drives surface plasma oscillation at the periphery of this aperture, which acts as a "relativistic oscillating window". The diffracted…

等离子体物理 · 物理学 2021-04-07 Longqing Yi

An approach to electron correlation effects in atoms that uses quantum trajectories is presented. A comparison with the exact quantum mechanical results for 1D Helium atom shows that the major features of the correlated ground state…

原子物理 · 物理学 2025-02-07 Ivan P. Christov

We explore the roles of electronic band structure and Coulomb interactions in solid-state HHG by studying the optical response of linear atomic chains and carbon nanotubes to intense ultrashort pulses. Specifically, we simulate electron…

介观与纳米尺度物理 · 物理学 2020-03-18 Sandra de Vega , Joel D. Cox , Fernando Sols , F. Javier García de Abajo

Applying time-dependent local density approximation (TDLDA), we study the high-order harmonic generation (HHG) of ethylene subjected to the one-color ($\omega=2.72$ eV) and the two-color ($\omega_1=2.72$ eV and $\omega_2=5.44$ eV)…

原子与分子团簇 · 物理学 2009-03-31 Z. P. Wang , P. M. Dinh , P. -G. Reinhard , E. Suraud , F. S. Zhang

We consider harmonics generation and wave-mixing by two-color multi photon resonant excitation of three-level atoms/molecules in strong laser fields. The coherent part of the spectra corresponding to multicolor harmonics generation is…

原子物理 · 物理学 2016-08-24 H. K. Avetissian , B. R. Avchyan , G. F. Mkrtchian

It is demonstrated by single-atom simulations that X-ray signals in the 3.4 to 4 keV region from an 8 micron laser driven high harmonic generation can be increased by more than two orders of magnitude when a single-cycle pulse centered at…

原子物理 · 物理学 2019-04-24 Zenghu Chang

By deriving the 3/2 dimensional Hamiltonian equations for electrons in the intense laser radiation and quasi-static transverse electric and longitudinal magnetic fields, the electron heating mechanisms are examined both for low harmonic…

等离子体物理 · 物理学 2019-07-24 Yanzeng Zhang , Sergei Krasheninnikov

We perform a detailed analysis of high-order harmonic generation in diatomic molecules within the strong-field approximation, with emphasis on quantum-interference effects. Specifically, we investigate how the different types of electron…

原子物理 · 物理学 2011-11-10 C. Figueira de Morisson Faria

Anomalously high generation efficiency of coherent higher field-harmonics in collisions between {\em oppositely charged particles} in the field of femtosecond lasers is predicted. This is based on rigorous numerical solutions of a quantum…

凝聚态物理 · 物理学 2009-10-31 H. Haberland , M. Bonitz , D. Kremp

We formulate the concept of dominant interaction Hamiltonians to obtain an integrable approximation to the dynamics of an electron exposed to a strong laser field and an atomic potential leading to high harmonic generation. The concept…

原子物理 · 物理学 2012-01-20 Carlos Zagoya , Christoph-Marian Goletz , Frank Grossmann , Jan M. Rost

We discuss a method of solving the time dependent Schrodinger equation for atoms with two active electrons in a strong laser field, which we used in a previous paper [A. Scrinzi and B. Piraux, Phys. Rev. A 56, R13 (1997)] to calculate…

原子物理 · 物理学 2014-05-19 Armin Scrinzi , Bernard Piraux

High-order harmonic generation is investigated for H$_2^+$ and D$_2^+$ with and without Born-Oppenheimer approximation by numerical solution of full dimensional electronic time-dependent Schr\"{o}dinger equation under 4-cycle intense laser…

原子物理 · 物理学 2014-10-22 Hamed Ahmadi , Ali Maghari , Hassan Sabzyan , Ali Reza Niknam , Mohsen Vafaee

We scrutinize the behavior of eigenvalues of an electron of Helium atom as it interacts with electric field directed along $z$-axis and exposed to linearly polarized intense laser field radiation. In order to achieve this, we freeze one…

When an atom or molecule absorbs a high-energy photon, an electron is emitted with a well-defined energy and a highly-symmetric angular distribution, ruled by energy quantization and parity conservation. These rules seemingly break down…

In this work we report ab initio calculations for the $H_2^+$ molecule interacting with ultrashort intense laser pulses. We analyse several observables that can, in principle, be available experimentally, in order to get a deeper…

原子物理 · 物理学 2017-05-25 R. E. F. Silva