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In this paper, we investigate the effects of full electronic correlation on the high harmonic generation in the helium atom subjected to laser pulses of extremely high intensity. To do this, we perform real-time propagations of the helium…

We theoretically investigate correlated electron dynamics in high-harmonic generation (HHG), using all-electron \emph{ab initio} simulations for three-dimensional real alkali-metal atoms. The resulting harmonic spectra exhibit a plateau…

原子物理 · 物理学 2019-04-10 Yang Li , Takeshi Sato , Kenichi L. Ishikawa

We theoretically study multielectron effects in high-harmonic generation (HHG), using all-electron first-principles simulations for a one-dimensional (1D) model atom. In addition to usual plateau and cutoff (from a cation in the present…

原子物理 · 物理学 2017-05-24 Iliya Tikhomirov , Takeshi Sato , Kenichi L. Ishikawa

High harmonic generation (HHG) provides a flexible framework for the development of coherent light sources in the extreme-ultraviolet and soft x-ray regimes. However it suffers from low conversion efficiencies as the control of the HHG…

光学 · 物理学 2014-09-16 Alberto Castro , Angel Rubio , E. K. U. Gross

We develop a time-dependent theory to investigate electron dynamics and photoionization processes of diatomic molecules interacting with strong laser fields including electron-electron correlation effects. We combine the recently formulated…

化学物理 · 物理学 2016-02-02 Henrik R. Larsson , Sebastian Bauch , Lasse Kragh Sørensen , Michael Bonitz

The interaction of a helium atom with intense short 800 nm laser pulse is studied theoretically beyond the single-active-electron approximation. For this purpose, the time-dependent Schr\"odinger equation for the two-electron wave packet…

原子与分子团簇 · 物理学 2017-03-08 Anton N. Artemyev , Lorenz S. Cederbaum , Philipp V. Demekhin

High-harmonic generation is one of the most extreme nonlinear-optical processes observed to date. By focusing an intense laser pulse into a gas, the light-atom interaction that occurs during the process of ionising the atoms results in the…

The generation of high harmonics is a strongly nonlinear effect that allows to probe properties of the target and to study electron dynamics in matter. It has been investigated in many different kinds of targets, including molecular gases,…

量子物理 · 物理学 2026-05-06 Lina Bielke , Samuel Schöpa , Falk-Erik Wiechmann , Franziska Fennel , Dieter Bauer

The laser interaction with an electron-positron-ion mixed plasma is studied, from the perspective of the associated high-order harmonic generation. For an idealized mixed plasma which is assumed with a sharp plasma-vacuum interface and…

等离子体物理 · 物理学 2021-01-20 W. L. Zhang , T. Grismayer , K. M. Schoeffler , R. A. Fonseca , L. O. Silva

The generation of high harmonics in laser-irradiated light homonuclear diatomics (H2+, N2 and O2) compared to that in atomic counterparts (of nearly identical binding energy) is studied within the velocity gauge version of conventional…

原子物理 · 物理学 2009-11-11 Vladimir I. Usachenko , Pavel E. Pyak , Shih-I Chu

High-order harmonic generation via single-slit diffraction of relativistic laser pulses is investigated. Using fully kinetic 2D and 3D particle-in-cell simulations, we show that interesting optical phenomena emerge, including the generation…

等离子体物理 · 物理学 2025-05-07 Longqing Yi

Hot dense helium is studied with first-principles computer simulations. By combining path integral Monte Carlo and density functional molecular dynamics, a large temperature and density interval ranging from 1000 to 1000000 K and 0.4 to 5.4…

材料科学 · 物理学 2015-05-13 Burkhard Militzer

The generation of high harmonics (HHG) in atomic systems by the highly non-linear response to an intense laser field is a prominent pathway to the synthesis of ever shorter laser pulses at increasingly higher photon energies. Extensions of…

原子物理 · 物理学 2022-11-23 Mohammad Monfared , Elnaz Irani , Christoph Lemell , Joachim Burgdörfer

A theory for laser-driven electron dynamics and high-harmonic generation in bulk solids with two lattice sites per unit cell of arbitrary dimension is formulated. In tight-binding approximation, such solids can be described by $2\times 2$…

介观与纳米尺度物理 · 物理学 2024-03-12 Daniel Moos , Hannah Jürß , Dieter Bauer

High-harmonic generation (HHG) in crystalline solids have been examined so far on the basis of one-body energy-band structures arising from electron itineracy in a periodic potential. Here, we show emergence of HHG signals which are…

强关联电子 · 物理学 2020-04-22 Shohei Imai , Atsushi Ono , Sumio Ishihara

High-harmonic generation in solids allows probing and controlling electron dynamics in crystals on few femtosecond timescales, paving the way to lightwave electronics. In the spatial domain, recent advances in the real-space interpretation…

We present a theoretical analysis of high-order harmonic generation from ion-atom collisions in the presence of linearly polarized intense laser pulses. Photons with frequencies significantly higher than in standard atomic high-harmonic…

原子物理 · 物理学 2009-11-10 Manfred Lein , Jan M. Rost

We report a detailed study of high-order harmonic generation (HHG) in helium. When comparing predictions from a single-active-electron model with those from all-electron simulations, such as ATTOMESA and R-matrix with time-dependence, which…

原子物理 · 物理学 2024-03-06 A. T. Bondy , S. Saha , J. C. del Valle , A. Harth , N. Douguet , K. R. Hamilton , K. Bartschat

Several correlation and interference effects in strong-field physics are investigated. We show that the interference of continuum wave packets can be the dominant mechanism of high-harmonic generation (HHG) in the over-the-barrier regime.…

We develop a numerical scheme to investigate the high-order harmonic generation (HHG) in intense laser-matter interactions. Tracing the time evolution of every electronic laser-field-free state, we "observe" the HHG in a time-integrated…

原子物理 · 物理学 2008-11-14 Y. J. Chen , J. Liu , Bambi Hu
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