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We explore the nematic ordering of the rod-like liquid crystals 5CB and 6CB, embedded into parallel-aligned nanochannels in mesoporous silicon and silica membranes as a function of mean channel radius (4.7<=R <=8.3 nm), and thus geometrical…

软凝聚态物质 · 物理学 2012-08-15 Sylwia Calus , Daniel Rau , Patrick Huber , Andriy V. Kityk

The present high-resolution inelastic neutron scattering experiment on ice XVII, containing molecular hydrogen with different ortho/para ratio, allows to assign the H$_2$ motion spectral bands to rotational and center-of-mass translational…

Ionic liquids constrained at interfaces or restricted in subnanometric pores are increasingly employed in modern technologies, including energy applications. Understanding the details of their behavior in these conditions is therefore…

材料科学 · 物理学 2018-09-25 Stefano Mossa

The molecular structure of neutral n-triacontanol mesophases at the n-hexane - water interface has been studied by diffuse X-ray scattering using synchrotron radiation. According to the experimental data, a transition to the multilayer…

软凝聚态物质 · 物理学 2017-12-15 Aleksey M. Tikhonov

X-ray diffraction patterns of ethanol confined in parallel-aligned channels of approx. 10 nm diameter and 50 micrometer length in mesoporous silicon have been recorded as a function of filling fraction, temperature and for varying cooling…

软凝聚态物质 · 物理学 2015-03-17 Anke Henschel , Klaus Knorr , Patrick Huber

We have established the detailed phase diagram of the prototypical deep eutectic solvent ethaline (ethylene glycol / choline chloride 2:1) as a function of the hydration level, in the bulk state and confined in the nanochannels of…

软凝聚态物质 · 物理学 2022-01-05 Benjamin Malfait , Aicha Jani , Denis Morineau

Investigating properties of phase change materials (PCMs) is an important issue due to their extensive use in heat storage systems and thermal regulation devices. Improvement of the efficiency of such systems should be based on a better…

应用物理 · 物理学 2022-07-18 L. Klochko , J. Noel , N. R. Sgreva , S. Leclerc , C. Métivier , D. Lacroix , M. Isaiev

A possibility was assessed to modify physico-chemical properties of ferronematic mixtures by introducing additional mesogenic and non-mesogenic components. The mixture, consisting of RM734 and DIO at the 70:30 weight ratio of the…

Crystallization of alkane mixtures has been studied extensively for decades. However, majority of the available data consider the behaviour of alkanes with chain length of 21 C-atoms or more. Furthermore, important information about the…

材料科学 · 物理学 2023-12-13 Diana Cholakova , Martin Pantov , Slavka Tcholakova , Nikolai Denkov

We implement molecular dynamics simulations in canonical ensemble to study the effect of confinement on a $2d$ crystal of point particles interacting with an inverse power law potential proportional to $r^{-12}$ in a narrow channel. This…

软凝聚态物质 · 物理学 2014-09-30 M. Ebrahim Foulaadvand , Neda Ojaghlou

Hydrocarbon films confined between smooth mica surfaces have long provided an experimental playground for model studies of structure and dynamics of confined liquids. However fundamental questions regarding the phase behavior and shear…

软凝聚态物质 · 物理学 2019-12-11 Alexander M. Smith , James E. Hallett , Susan Perkin

Spatial confinement in nanoporous media affects the structure, thermodynamics and mobility of molecular soft matter often markedly. This article reviews thermodynamic equilibrium phenomena, such as physisorption, capillary condensation,…

软凝聚态物质 · 物理学 2015-02-17 Patrick Huber

We report the results of molecular dynamics (MD) simulations of a complete monolayer of hexane physisorbed onto the basal plane of graphite. At low temperatures the system forms a herringbone solid. With increasing temperature, a solid to…

软凝聚态物质 · 物理学 2009-11-10 M. W. Roth , C. L. Pint , Carlos Wexler

The viscosity of liquids under nanoconfinement remains controversial. Reports range from spontaneous solidification to no change in the viscosity at all. Here, we present thorough measurements with a small-amplitude linear atomic force…

软凝聚态物质 · 物理学 2012-10-15 Shah H. Khan , Peter M. Hoffmann

We report combined optical birefringence and neutron scattering measurements on the liquid crystal 12CB nanoconfined in mesoporous silicon layers. This liquid crystal exhibits strong nematic-smectic coupling responsible for a discontinuous…

介观与纳米尺度物理 · 物理学 2010-05-04 Gilbert Chahine , Andriy V. Kityk , Klaus Knorr , Ronan Lefort , Mohammed Guendouz , Denis Morineau , Patrick Huber

In this paper we present a review on our recent experimental investigations into the phase behavior of the deeply cooled water confined in a nanoporous silica material, MCM-41, with elastic neutron scattering technique. Under such strong…

软凝聚态物质 · 物理学 2016-12-13 Zhe Wang , Kanae Ito , Sow-Hsin Chen

The remaining dynamical degrees of freedom of molecular fluids confined into capillaries of nano to sub-nanometer diameter are of fundamental relevance for future developments in the field of nanofluidics. These properties cannot be simply…

The optical birefringence of rod-like nematogens (7CB, 8CB), imbibed in parallel silica channels with 10 nm diameter and 300 micrometer length, is measured and compared to the thermotropic bulk behavior. The orientational order of the…

软凝聚态物质 · 物理学 2016-09-08 Andriy V. Kityk , Matthias Wolff , Klaus Knorr , Denis Morineau , Ronan Lefort , Patrick Huber

We present a neutron and X-rays scattering study of the phase transitions of 4-n-octyl-4'-cyanobiphenyl (8CB) confined in unidirectional nanopores of porous alumina and porous silicon (PSi) membranes with an average diameter of 30 nm.…

Nanocrystalline Ni can adopt a hexagonal close-packed (hcp) structure,which does not appear in a bulk form under any conditions.Structural studies found its $>$ 20% expansion of volume per atom compared with face-centered cubic (fcc)…