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Thermoelectric effects, measured by the Seebeck coefficients, refer to the phenomena in which a temperature difference or gradient imposed across a thermoelectric material induces an electrical potential difference or gradient, and vice…

材料科学 · 物理学 2018-12-05 Yi Wang , Yong-Jie Hu , Shun-Li Shang , Bi-Cheng Zhou , Zi-Kui Liu , Long-Qing Chen

The atomic variations of electronic wavefunctions at the surface and electron scattering near a defect have been detected unprecedentedly by tracing thermoelectric voltages given a temperature bias [Cho et al., Nature Mater. 12, 913…

介观与纳米尺度物理 · 物理学 2014-04-02 Eui-Sup Lee , Sanghee Cho , Ho-Ki Lyeo , Yong-Hyun Kim

We report on the first measurement of the Seebeck coefficient in a tunnel-contacted and gate-tunable individual single-quantum dot junction in the Kondo regime, fabricated using the electromigration technique. This fundamental…

介观与纳米尺度物理 · 物理学 2019-01-31 B. Dutta , D. Majidi , A. Garcia Corral , P. Erdman , S. Florens , T. Costi , H. Courtois , C. B. Winkelmann

Theoretical descriptions of the Seebeck coefficient in terms of the differential electrical conductivity given by Cutler and Mott is the foundation of later works in terms of transmission function from the thermoelectric transport theory.…

Creating temperature gradients in magnetic nanostructures has resulted in a new research direction, i.e., the combination of magneto- and thermoelectric effects. Here, we demonstrate the observation of one important effect of this class:…

The Seebeck effect describes the generation of an electric potential in a conducting solid exposed to a temperature gradient. Besides fundamental relevance in solid state physics, it serves as a key quantity to determine the performance of…

The Seebeck coefficient (S) of a serially coupled quantum dot (SCQD) junction system is theoretically studied via a two-level Anderson model. A change of sign in S with respect to temperature is found, which arises from the competition…

介观与纳米尺度物理 · 物理学 2015-05-27 David M. -T. Kuo , Yia-chung Chang

We report the first concurrent determination of conductance (G) and thermopower (S) of single-molecule junctions via direct measurement of electrical and thermoelectric currents using a scanning tunneling microscope-based break-junction…

介观与纳米尺度物理 · 物理学 2012-01-10 J. R. Widawsky , P. Darancet , J. B. Neaton , L. Venkataraman

Novel organic materials formed from functional molecules are attractive for various nanoelectronic applications because they are environmentally friendly, widely available and inexpensive. Recent advancement in bottom-up fabrication methods…

介观与纳米尺度物理 · 物理学 2022-12-14 Abdalghani Daaoub , Renhang Wang , Ross Davidson , Sara Sangtarash , Hatef Sadeghi

We report first-principles calculations of inelastic Seebeck coefficients in an aluminum monatomic junction. We compare the elastic and inelastic Seebeck coefficients with and without local heating. In the low temperature regime, the…

介观与纳米尺度物理 · 物理学 2011-01-27 Bailey C. Hsu , Yu-Shen Liu , Sheng Hsien Lin , Yu-Chang Chen

The electronic thermoelectric coefficients are analyzed in the vicinity of one and two Anderson localization thresholds in three dimensions. For a single mobility edge, we correct and extend previous studies, and find universal approximants…

无序系统与神经网络 · 物理学 2017-10-09 Kaoru Yamamoto , Amnon Aharony , Ora Entin-Wohlman , Naomichi Hatano

We theoretically study the nonequilibrium thermoelectric transport properties of a strongly-correlated molecule (or quantum dot) embedded in a tunnel junction. Assuming that the coupling of the molecule to the contacts is asymmetric, we…

介观与纳米尺度物理 · 物理学 2023-02-22 Anand Manaparambil , Ireneusz Weymann

Single molecule junctions exhibit dynamic structural configurations that strongly influence their electronic and thermoelectric properties. Here, we combine conductance (G) and Seebeck coefficient (S) measurements using the novel AC based…

We look for manifestations of quantum interference effects in the Seebeck coefficient of a molecular junction, when the electronic conductance exhibits pronounced destructive interference features due to the presence of quasi-degenerate…

介观与纳米尺度物理 · 物理学 2015-06-11 Lena Simine , Wei Jia Chen , Dvira Segal

We report a method using scanning tunnelling microscope single molecular break junction to simultaneously measure and correlate the single-molecule thermopower and electrical conductance. In contrast to previously reported approaches, it…

介观与纳米尺度物理 · 物理学 2021-09-24 Joseph M. Hamill , Christopher Weaver , Tim Albrecht

The electronic and thermoelectric properties of molecular junctions formed from iron and ruthenium metal-acetylide were studied using complementary experimental techniques and quantum chemical simulations. We performed physical…

We consider a molecular junction immersed in a solvent where the electron transfer is dominated by Marcus-type steps. However, the successive nature of the charge transfer through the junction does not imply that the solvent reach thermal…

统计力学 · 物理学 2022-03-23 Henning Kirchberg , Abraham Nitzan

The quest for efficient devices has fueled research in thermoelectric materials. In these materials, the goal is to maximize the Figure of Merit $ZT$. One of the components of this quantity is the Seebeck coefficient, which measures the…

While thermoelectric transport theory is well established and widely applied, there remains some degree of confusion on the proper thermodynamic definition of the Seebeck coefficient (or thermoelectric power) which is a measure of the…

材料科学 · 物理学 2016-04-05 Y. Apertet , H. Ouerdane , C. Goupil , Ph. Lecoeur

We study charge and energy transfer in two-site molecular electronic junctions in which electron transport is assisted by a vibrational mode. To understand the role of mode harmonicity/anharmonicity on transport behavior, we consider two…

介观与纳米尺度物理 · 物理学 2015-09-01 Bijay Kumar Agarwalla , Jian-Hua Jiang , Dvira Segal
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