相关论文: Control the high-order harmonics cutoff through th…
The selection rules of high harmonic generation (HHG) are investigated using three-dimensional time-dependent density functional theory (TDDFT). From the harmonic spectra obtained with various real molecules and different forms of laser…
Highly-efficient optical generation of narrowband terahertz (THz) radiation enables unexplored technologies and sciences from compact electron acceleration to charge manipulation in solids. State-of-the-art conversion efficiencies are…
Harmonic generation is a general characteristic of driven nonlinear systems, and serves as an efficient tool for investigating the fundamental principles that govern the ultrafast nonlinear dynamics. In atomic gases, high-harmonic radiation…
High-order harmonic generation (HHG) from molecular ion HeH$^{2+}$ in two initial states of $1s\sigma$ (ground state) and $2p\sigma$ (first excited state) is investigated theoretically, in homogeneous and plasmonic-enhanced laser fields.…
We show how to optimize the process of high-harmonic generation (HHG) by gating the interaction using the field gradient of a driving pulse with a linear ramp waveform. Since maximized field gradients are efficiently generated by…
A new method to coherently control the electron dynamics is proposed using a few-cycle laser pulse in combination with a controlling field. It is shown that this method not only broadens the attosecond pulse bandwidth, but also reduces the…
The interaction of relativistically strong tailored laser pulses with an atomic system is considered. Due to a special tailoring of the laser pulse, the suppression of the relativistic drift of the ionized electron and a dramatic…
High harmonic generation in polarizable multi-electron systems is investigated in the framework of multi-configuration time-dependent Hartree-Fock. The harmonic spectra exhibit two cut offs. The first cut off is in agreement with the well…
High harmonic spectra generated in condensed matter carry the fingerprints of sub-cycle electronic motion and the energy structure of the studied system. Here we show that tailoring the waveform of mid-infrared driving light by using a…
From the famous classical "simple man" model to the recent multichannel model for polyatomic molecules, this tutorial will guide you through the several landmarks in our understanding of high harmonic generation and high harmonic…
We perform an experimental two-color high-order harmonic generation study in argon with the fundamental of an ytterbium ultrashort pulse laser and its second harmonic. The intensity of the second harmonic and its phase relative to the…
High order harmonic generation from clusters is a controversial topic: conflicting theories exist, with different explanations for similar experimental observations. From an experimental point of view, separating the contributions from…
The generation of high-order harmonics in finite, hexagonal nanoribbons is simulated. Ribbons with armchair and zig-zag edges are investigated by using a tight-binding approach with only nearest neighbor hopping. By turning an alternating…
In the past two decades high-harmonic generation (HHG) has become a key process in ultra-fast science due to the extremely short time-structure of the underlying electron dynamics being imprinted in the emitted harmonic light bursts. After…
The interaction of intense mid-infrared laser fields with atoms and molecules leads to a range of new opportunities, from the production of bright, coherent radiation in the soft x-ray range to imaging molecular structures and dynamics with…
Quantum-mechanical investigation is presented to study single attosecond pulse generation by gating high-order harmonic emission from H$_2^+$ molecule in intense laser pulses with time-dependent ellipticity. The high-order harmonic…
We experimentally observe longer than long trajectory influence in high order harmonic generation (HHG) by varying the peak intensity of the driving laser field through either direct attenuation, or by chirping the laser pulse. Using a…
In this work, we demonstrate experimentally the efficient generation and tunability of energetic highly-elliptical high-harmonics in Ar gas, driven by intense two-color counter rotating laser electric fields. A bi-chromatic beam tailored by…
We study high-order harmonic generation (HHG) from aligned molecules in strong elliptically polarized laser fields numerically and analytically. Our simulations show that the spectra and polarization of HHG depend strongly on the molecular…
We measure spectrally and spatially resolved high-order harmonics generated in argon using chirped multi-cycle laser pulses. Using a stable, high-repetition rate laser we observe detailed interference structures in the far-field. The…