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A thorough investigation of single crystalline magnetite using broadband dielectric spectroscopy and other methods provides evidence for relaxor-like polar order in Fe3O4. We find long-range ferroelectric order to be im-peded by the…

强关联电子 · 物理学 2011-06-10 F. Schrettle , S. Krohns , P. Lunkenheimer , V. A. M. Brabers , A. Loidl

Recent progress in the field of multiferroics led to the discovery of many new materials in which ferroelectricity is induced by cycloidal spiral orders. The direction of the electric polarization is typically constrained by spin…

We investigate the magnetothermodynamic properties of the perovskite manganite Pr0.46Sr0.54MnO3. Our data imply that the paramagnetic to antiferromagnetic transition at TN = 210 K is first order with an abrupt decrease of volume (~ 0.14 %…

Magnetoelectric phase diagrams of the perovskite manganites, Eu1-xYxMnO3 and Gd1-xTbxMnO3, are theoretically studied. We first construct a microscopic model, and then analyze the model using the Monte-Carlo method. We reproduce the…

强关联电子 · 物理学 2009-10-28 Masahito Mochizuki , Nobuo Furukawa

X-ray resonant magnetic scattering studies of rare earth magnetic ordering were performed on perovskite manganites RMnO3 (R = Dy, Gd) in an applied magnetic field. The data reveal that the field-induced three-fold polarization enhancement…

Multiferroics, materials where spontaneous long-range magnetic and dipolar orders coexist, represent an attractive class of compounds, which combine rich and fascinating fundamental physics with a technologically appealing potential for…

材料科学 · 物理学 2015-05-13 Silvia Picozzi , Claude Ederer

We present sharp magnetization jumps and field induced irreversibility in magnetization in multiferroic Y2CoMnO6. Appearance of magnetic relaxation and field sweep rate dependence of magnetization jumps resemble the martensite like scenario…

强关联电子 · 物理学 2015-06-22 J. Krishna Murthy , K. Devi Chandrasekhar , H. C. Wu , H. D. Yang , J. Y. Lin , A. Venimadhav

The effect of cobalt and nickel substitutions for manganese on the physical properties of the perovskite manganite La1.2Bi0.8Mn2-x(Ni/Co)xO6+d, with x = 0.0-0.8, has been investigated. It is observed that the ferromagnetism is enhanced, TC…

材料科学 · 物理学 2008-09-04 Asish K. Kundu , R. Ranjith , V. Pralong , V. Caignaert , B. Raveau

Using a joint approach of density functional theory and model calculations, we demonstrate that a prototypical charge ordered half-doped manganite, La$_{1/2}$Ca$_{1/2}$MnO$_3$ is multiferroic. The combination of a peculiar charge-orbital…

材料科学 · 物理学 2010-07-15 Gianluca Giovannetti , Sanjeev Kumar , Jeroen van den Brink , Silvia Picozzi

We studied the correlation between magnetic, electrical, structural, and magnetostriction properties of the electron doped manganites Ca$_x$Sm$_{1-x}$MnO$_3$ (x = 0.85, 0.8). The paramagnetic to antiferromagnetic transition in both the…

We present a detailed magnetic study of the perovskite manganite Pr0.7Ca0.3MnO3 at low temperatures including magnetization and a.c. susceptibility measurements. The data appear to exclude a conventional spin glass phase at low fields,…

强关联电子 · 物理学 2009-10-31 I. G. Deac , J. F. Mitchell , P. Schiffer

Structural, magnetic and electric properties of a metal-ordered perovskite YBaMn2O6 have been studied by means of powder X-ray diffraction, DSC, magnetic susceptibility, and electric resistivity. It is found that this material undergoes a…

强关联电子 · 物理学 2009-11-07 T. Nakajima , H. Kageyama , Y. Ueda

This work investigates the magnetically driven ferroelectricity in orthorhombic manganites RMnO3 (R=Gd, Dy or Tb) from the point of view of the symmetry. The method adopted generalizes the one used to characterize the polar properties of…

材料科学 · 物理学 2009-11-13 J. L. Ribeiro

Motivated by the recent discovery of dielectric relaxation by quantum critical magnons in Cs$_2$Cu$_2$Mo$_3$O$_{12}$, we conduct a detailed analysis of its dielectric response and compare it to that in the isostructural compound…

强关联电子 · 物理学 2024-06-19 D. Flavián , P. A. Volkov , S. Hayashida , K. Yu. Povarov , S. Gvasaliya , P. Chandra , A. Zheludev

Recently, the perovskite BiCoO$_3$ has been shown experimentally to be isostructural with PbTiO$_3$, while simultaneously the $d^6$ Co$^{3+}$ ion has a high spin ground state with $C$-type antiferromagnetic ordering. Using hybrid density…

材料科学 · 物理学 2016-05-04 Leigh Weston , Xiangyuan Cui , Simon P. Ringer , Catherine Stampfl

Measurements of the low-frequency (f<=100 kHz) permittivity and conductivity at T<= 150 K are reported for La(1-x)Ca(x)MnO(3) (0<=x<=1) and Ca(1-y)Sr(y)MnO(3) (0<=y<=0.75) having antiferromagnetic, insulating ground states covering a broad…

强关联电子 · 物理学 2009-11-10 J. L. Cohn , M. Peterca , J. J. Neumeier

A single crystal of 7% Fe-doped (La$_{0.7}$Pr$_{0.3}$)$_{0.65}$Ca$_{0.35}$MnO$_3$ shows up as a typical relaxor ferromagnet, where ferromagnetic metallic and charge-orbital-ordered insulating clusters coexist with controllable volume…

强关联电子 · 物理学 2008-03-28 H. Sakai , Y. Tokura

The dielectric behavior of half doped manganites La0.5Ca0.5-xSrxMnO3 (0.1 \leq \times \leq 0.4) with varying magnetic ground states has been studied. The real part of relative permittivity as a function of temperature {\epsilon}^'(T),…

材料科学 · 物理学 2015-05-20 Indu Dhiman , S. K. Deshpande , A. Das

Pressure effects on the charge and spin dynamics in the bilayer manganite compounds $La_{2-2x}Sr_{1+2x}Mn_2O_7$ are studied theoretically by taking into account the orbital degrees of freedom. The orbital degrees are active in the layered…

强关联电子 · 物理学 2009-10-30 Sumio Ishihara , Satoshi Okamoto , Sadamichi Maekawa

The question of how ferroelectric polarization is coupled to magnetism in magnetoelectric multiferroics, in which both types of order are simultaneously present, is of considerable scientific and practical interest. A recent Letter…

材料科学 · 物理学 2009-07-13 Rogerio de Sousa , Joel E. Moore