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The properties of excitons in semiconducting single-walled carbon nanotubes (SWCNTs), isolated in vacuum or a medium, and their contributions to the optical spectra of nanotubes are studied within the elementary potential model, in which an…

材料科学 · 物理学 2010-12-15 Oleksii A. Smyrnov

The spectrum of large radius exciton in an individual semiconducting single-walled carbon nanotube (SWCNT) is described within the framework of elementary potential model, in which exciton is modeled as bound state of two oppositely charged…

其他凝聚态物理 · 物理学 2010-11-18 Vadym M. Adamyan , Oleksii A. Smyrnov

Exciton effects are studied in single-wall boron-nitride nanotubes. The Coulomb interaction dependence of the band gap, the optical gap, and the binding energy of excitons are discussed. The optical gap of the (5,0) nanotube is about 6eV at…

材料科学 · 物理学 2009-07-07 Kikuo Harigaya

We develop a scaling relationship between the exciton binding energy and the external dielectric function in carbon nanotubes. We show that the electron-electron and electron-hole interaction energies are strongly affected by screening yet…

Single-walled carbon nanotubes are strongly correlated systems with large Coulomb repulsion between two electrons occupying the same $p_z$ orbital. Within a molecular Hamiltonian appropriate for correlated $\pi$-electron systems, we show…

材料科学 · 物理学 2009-02-15 Zhendong Wang , Demetra Psiachos , Roberto F. Badilla , Sumit Mazumdar

Using Coulomb correlation parameters appropriate for $\pi$-conjugated polymers (PCPs), and a nearest neighbor hopping integral that is arrived at by fitting the energy spectra of three zigzag semiconducting single-walled carbon nanotubes…

材料科学 · 物理学 2007-05-23 Zhendong Wang , Hongbo Zhao , Sumit Mazumdar

One- and two-photon luminescence excitation spectroscopy showed a series of distinct excitonic states in single-walled carbon nanotubes. The energy splitting between one- and two-photon-active exciton states of different wavefunction…

材料科学 · 物理学 2007-05-23 J. Maultzsch , R. Pomraenke , S. Reich , E. Chang , D. Prezzi , A. Ruini , E. Molinari , M. S. Strano , C. Thomsen , C. Lienau

Electron-electron interactions and excitons in carbon nanotubes are locally measured by combining Scanning tunneling spectroscopy and optical absorption in bundles of nanotubes. The largest gap deduced from measurements at the top of the…

Photophysics of single-wall carbon nanotubes (SWCNTs) is intensively studied due to their potential application in light harvesting and optoelectronics. Excited states of SWCNTs form strongly bound electron-hole pairs, excitons, of which…

介观与纳米尺度物理 · 物理学 2021-01-28 J. Palotas , M. Negyedi , S. Kollarics , A. Bojtor , P. Rohringer , Th. Pichler , F. Simon

We report first-principles calculations of the effects of quasiparticle self-energy and electron-hole interaction on the optical properties of single-walled BN nanotubes. Excitonic effects are shown to be even more important in BN nanotubes…

材料科学 · 物理学 2007-08-23 Cheol-Hwan Park , Catalin D. Spataru , Steven G. Louie

We calculate the exciton binding energy in single-walled carbon nanotubes with narrow band gaps, accounting for the quasi-relativistic dispersion of electrons and holes. Exact analytical solutions of the quantum relativistic two-body…

介观与纳米尺度物理 · 物理学 2011-08-16 R. R. Hartmann , I. A. Shelykh , M. E. Portnoi

Recent experiments about the low temperature behaviour of a Single Wall Carbon Nanotube (SWCNT) showed typical Coulomb Blockade (CB) peaks in the zero bias conductance and allowed us to investigate the energy levels of interacting…

强关联电子 · 物理学 2009-11-11 S. Bellucci , P. Onorato

Exciton effects are studied in single-wall boron-nitride (BN) nanotubes. Linear absorption spectra are calculated with changing the chiral index of the zigzag nanotubes. We consider the extended Hubbard model with atomic energies at the…

材料科学 · 物理学 2009-07-07 Kikuo Harigaya

Environmental dielectric screening effects on exciton transition energies in single-walled carbon nanotubes (SWNTs) have been studied quantitatively in the range of dielectric constants from 1.0 to 37 by immersing SWNTs bridged over…

Resonant Raman spectroscopy of single carbon nanotubes suspended across trenches displays red shifts of up to 30 meV of the electronic transition energies as a function of the surrounding dielectric environment. We develop a simple scaling…

Optical properties of single-wall carbon nanotubes (SWCNTs) for light polarized parallel to the nanotube axis have been extensively studied, whereas their response to light polarized perpendicular to the nanotube axis has not been well…

介观与纳米尺度物理 · 物理学 2019-01-23 Fumiya Katsutani , Weilu Gao , Xinwei Li , Yota Ichinose , Yohei Yomogida , Kazuhiro Yanagi , Junichiro Kono

We report correlated-electron calculations of optically excited states in ten semiconducting single-walled carbon nanotubes with a wide range of diameters. Optical excitation occurs to excitons whose binding energies decrease with the…

材料科学 · 物理学 2007-05-23 Hongbo Zhao , Sumit Mazumdar

We studied the asymmetry between valence and conduction bands in single-walled carbon nanotubes (SWNTs) through the direct observation of spin-singlet transverse dark excitons using polarized photoluminescence excitation spectroscopy. The…

材料科学 · 物理学 2015-05-14 Yuhei Miyauchi , Hiroshi Ajiki , Shigeo Maruyama

We study quantum optical properties of the single-walled carbon nanotube (SWCNT) by introducing the effective interaction between the quantized electromagnetic field and the confined electrons in the SWCNT. Our purpose is to explore the…

介观与纳米尺度物理 · 物理学 2009-04-30 Z. L. Guo , Z. R. Gong , C. P. Sun

Many-electron effects often dramatically modify the properties of reduced dimensional systems. We report calculations, based on an many-electron Green's function approach, of electron-hole interaction effects on the optical spectra of…

材料科学 · 物理学 2009-11-10 Catalin D. Spataru , Sohrab Ismail-Beigi , Lorin X. Benedict , Steven G. Louie
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