相关论文: Photoassociation spectroscopy of a Spin-1 Bose-Ein…
We report the high resolution photoassociation (PA) spectroscopy of a $^{87}Rb$ Bose-Einstein condensate (BEC) to excited molecular states near the dissociation limit of $5P_{1/2} +5S_{1/2}$ by optical Bragg scattering. Since the detection…
A dynamical many body theory of single color photoassociation in a Bose-Einstein condensate is presented. The theory describes the time evolution of a condensed atomic ensemble under the influence of an arbitrarily varying near resonant…
We report on the formation of ultra-cold Na$_2$ molecules using single-photon photoassociation of a Bose-Einstein condensate. The photoassociation rate, linewidth and light shift of the J=1, $v=135$ vibrational level of the…
Coherent control of reactants remains a longstanding challenge in quantum chemistry. In particular, we have studied laser-induced molecular formation (photoassociation) in a Raman-dressed spin-orbit-coupled 87Rb Bose-Einstein condensate,…
We investigate theoretically the molecular yield in photoassociation of Bose-Einstein condensed sodium atoms for light intensities of the order of and above those applied in a recent experiment. Our results show that the rate at which…
We simulate numerically the photodissociation of molecules into noncondensate atom pairs that accompanies photoassociation of an atomic Bose-Einstein condensate into a molecular condensate. Such rogue photodissociation sets a limit on the…
We observe light-induced frequency shifts in one-color photoassociative spectra of magnetically trapped $^4$He$^*$ atoms in the metastable $2^3S_1$ state. A pair of ultracold spin-polarized $2^3S_1$ helium atoms is excited into a molecular…
We study coherent photoassociation, phenomena analogous to coherent optical transients in few-level systems, which may take place in photoassociation of an atomic Bose-Einstein condensate but not in a nondegenerate gas. We develop a…
We present experimental observations of seven vibrational levels $v'=20-26$ of the $1^{3}\Sigma_{g}^{+}$ excited state of Li$_2$ molecules by the photoassociation (PA) of a degenerate Fermi gas of $^6$Li atoms. For each vibrational level,…
We report the observation of strongly ferromagnetic $F=1$ spinor Bose-Einstein condensates of $^7$Li atoms. The condensates are generated in an optical dipole trap without using magnetic Feshbach resonances, so that the condensates have…
We theoretically investigate the effect of anomalous quantum correlations on the light-induced frequency shift in the photoassociation spectrum of a Bose-Einstein condensate (BEC). Anomalous quantum correlations arise because, although…
A weakly interacting, spin-orbit coupled, two-component, ultracold Bose gas bound to a Bravais lattice is studied. Motivated by recent experimental advances in the field of synthetically spin-orbit coupled, ultracold, neutral atomic gases…
We report on the first observation of photoassociation near the ${}^2 S _\frac 1 2 + {}^3P_1$-asymptote in a mixture of ${}^{87}$Rb and ${}^{170}$Yb. In a search spanning binding energies between 0.1 GHz and 11 GHz, a single pair of…
We demonstrate coherent one-color photoassociation of a Bose-Einstein condensate, which results in Rabi oscillations between atomic and molecular condensates. We attain atom-molecule Rabi frequencies that are comparable to decoherence rates…
Using parametric conversion induced by a Shapiro-type resonance, we produce and characterize a two-mode squeezed vacuum state in a sodium spin 1 Bose-Einstein condensate. Spin-changing collisions generate correlated pairs of atoms in the…
We describe a Fourier transform spectroscopy technique for directly measuring band structures, and apply it to a spin-1 spin-orbit coupled Bose-Einstein condensate. In our technique, we suddenly change the Hamiltonian of the system by…
We present two-photon photoassociation to the least-bound vibrational level of the X$^1\Sigma_g^+$ electronic ground state of the $^{86}$Sr$_2$ dimer and measure a binding energy of $E_b=-83.00(7)(20)$\,kHz. Because of the very small…
We measure the effect of a magnetic Feshbach resonance (FR) on the rate and light-induced frequency shift of a photoassociation resonance in ultracold $^7$Li. The photoassociation-induced loss rate coefficient, $K_p$, depends strongly on…
We calculate the two-photon 1S-2S spectrum of an atomic hydrogen Bose-Einstein condensate in the regime where the cold collision frequency shift dominates the lineshape. WKB and static phase approximations are made to find the intensities…
Photoassociation of spin-polarized metastable helium to the three lowest rovibrational levels of the J=1, $0_u^+$ state asymptoting to 2$s {}^{3}$S$_{1}+2p {}^{3}$P$_{0}$ is studied using a second-order perturbative treatment of the line…