相关论文: Femtosecond dynamics and laser control of charge t…
The treatment of the previous paper is extended to molecular wires. Specifically, the effect of electron-vibrational interactions on the electronic transport induced by femtosecond $\omega+2\omega$ laser fields along unbiased molecular…
We investigate coherent electron dynamics in graphene, interacting with the electric field waveform of two orthogonally polarized, few-cycle laser pulses. Recently, we demonstrated that linearly polarized driving pulses lead to…
Femtosecond time-resolved x-ray diffraction is employed to study the dynamics of the periodic lattice distortion (PLD) associated with the charge-density-wave (CDW) in K0.3MoO3. Using a multi-pulse scheme we show the ability to extend the…
We apply dynamical mean field theory to study a prototypical model that describes charge ordering in the presence of both electron-lattice interactions and intersite electrostatic repulsion between electrons. We calculate the optical and…
Electronic decoherence processes in trans-polyacetylene oligomers are considered by explicitly computing the time dependent molecular polarization from the coupled dynamics of electronic and vibrational degrees of freedom in a mean-field…
Fullerene complexes may play a key role in the design of future molecular electronics and nanostructured devices with potential applications in light harvesting using organic solar cells. Charge and energy flow in these systems is mediated…
We identify an intriguing feature of the electron-vibrational dynamics of molecular systems via a computational examination of \emph{trans}-polyacetylene oligomers. Here, via the vibronic interactions, the decay of an electron in the…
A theoretical investigation on the quantum control of optical coherent four-wave mixing interactions in two-level systems driven by two intense synchronized femtosecond laser pulses of central angular frequencies $\omega$ and $3\omega$ is…
We investigate the quantum dynamics of fermionic particles interacting with a laser field in a gaseous medium, in the regime of inelastic diffraction scattering on the phase lattice of a slowed travelling wave, below the critical field of…
We report on coherent control of excitation processes of translationally ultracold rubidium dimers in a magneto-optical trap by using shaped femtosecond laser pulses. Evolution strategies are applied in a feedback loop in order to optimize…
Coherent control of the atomic two-photon absorption with shaped single-cycle pulses is examined theoretically in the weak-field regime. The control over the stabilized carrier-envelope phase (CEP) of the pulses is determined as a key…
We report a study on the optical dipole force on a beam of neutral three-level like atomic system induced by a femtosecond super-Gaussian pulse. We show that maximum coherence between the ground state |1> and the excited state |2> could be…
Coherent control of femtosecond two-photon absorption in the intermediate-field regime is analyzed in detail in the powerful frequency domain using an extended 4th-order perturbative description. The corresponding absorption is coherently…
Ultrafast control of electron dynamics in solid state systems has recently found particular attention. By increasing the electric field strength of laser pulses, the light-matter interaction in solids might turn from a perturbative into a…
We explore the effects of ultrafast shaped pulses for two-level systems that do not have a single photon resonance by developing a multiphoton density-matrix approach. We take advantage of the fact that the dynamics of the intermediate…
We present numerical studies of the transport dynamics of a charged soliton in conjugated polymers under the influence of an external time-dependent electric field. All relevant electron-phonon and electron-electron interactions are nearly…
Irradiation of a molecular system by an intense laser field can trigger dynamics of both electronic and nuclear subsystems. The lighter electrons usually move on much faster, attosecond time scale but the slow nuclear rearrangement damps…
The high field charge injection and transport properties in reinforced silicone dielectrics were investigated by measuring the time-dependent space charge distribution and the current under dc conditions up to the breakdown field, and were…
The transient signals derived from femtosecond pump-probe experiments are analyzed in terms of the coherent evolution of the energy levels perturbed by the excitation pulse. The model system is treated as the sum of independent two-level…
Understanding the fundamental mechanisms ruling laser-induced coherent charge transfer in hybrid organic/inorganic interfaces is of paramount importance to exploit these systems in next-generation opto-electronic applications. In a…