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We present a study of dissociative electron attachment and vibrational excitation processes in electron collisions with the CF$_3$Cl molecule. The calculations are based on the two-dimensional nuclear dynamics including the C-Cl symmetric…

化学物理 · 物理学 2011-12-09 Michal Tarana , Karel Houfek , Jiří Horáček , Ilya I. Fabrikant

We study the rotational predissociation of atom - molecule complexes with very small binding energy. Such complexes can be produced by Feshbach resonance association of ultracold molecules with ultracold atoms. Numerical calculations of the…

化学物理 · 物理学 2011-10-03 Alisdair O. G. Wallis , Roman V. Krems

The assumptions underpinning the adiabatic Born-Oppenheimer (BO) approximation are broken for molecules interacting with attosecond laser pulses, which generate complicated coupled electronic-nuclear wavepackets that generally will have…

化学物理 · 物理学 2024-05-17 Aleksander P. Woźniak , Ludwik Adamowicz , Thomas Bondo Pedersen , Simen Kvaal

Measurements of energy-resolved positron-molecule annihilation show the existence of positron binding and vibrational Feshbach resonances. The existing theory describes this phenomenon successfully for the case of infrared-active…

原子物理 · 物理学 2017-09-25 M. R. Natisin , J. R. Danielson , G. F. Gribakin , A. R. Swann , C. M. Surko

We propose a mechanism which allows one to control the transmission of single electrons through a molecular junction. The principle utilizes the emergence of transmission sidebands when molecular vibrational modes are coupled to the…

介观与纳米尺度物理 · 物理学 2010-03-26 Thomas Olsen , Jakob Schiøtz

The adsorption of iron phthalocyanine (FePc) on the passivated H/Si(111) surface is explored from first principles. We find that the organic molecule is predominantly physisorbed with a distance to the surface of $2.6 \pm 0.1$ Angstrom, but…

材料科学 · 物理学 2019-05-06 Benjamin Geisler , Peter Kratzer

We report on the preparation of a pure ultracold sample of bosonic DyK Feshbach molecules, which are composed of the fermionic isotopes 161Dy and 40K. Employing a magnetic sweep across a resonance located near 7.3 G, we produce up to 5000…

量子气体 · 物理学 2023-11-14 E. Soave , A. Canali , Zhu-Xiong Ye , M. Kreyer , E. Kirilov , R. Grimm

We model combined photoassociation and Feshbach resonances in a Bose-Einstein condensate, where the shared dissociation continuum allows for quantum interference in losses from the condensate, as well as a dispersive-like shift of…

量子气体 · 物理学 2015-05-14 Matt Mackie , Catherine DeBrosse

This work reports an ESR study of low energy, low fluence phosphorus ion implantation into silicon in order to observe the activation of phosphorus donors placed in close proximity to the Si-SiO2 interface. Electrical measurements, which…

We show that the complete photoemission dynamics in situations of electron-ion entanglement can be retrieved from photoelectron spectral measurements without information on the ion. To this end, we develop an energy-time analysis of the…

We report a first principles study of the structure and the vibrational properties of the Si(100)-H(2 \times 1) surface in an electric field. The calculated vibrational parameters are used to model the vibrational modes in the presence of…

材料科学 · 物理学 2009-10-31 K. Stokbro

We study the real-time dynamics of a highly excited charge carrier coupled to quantum phonons via a Holstein-type electron-phonon coupling. This is a prototypical example for the non-equilibrium dynamics in an interacting many-body system…

强关联电子 · 物理学 2015-03-11 F. Dorfner , L. Vidmar , C. Brockt , E. Jeckelmann , F. Heidrich-Meisner

We present a perturbation approach rooted in time-dependent density-functional theory to calculate electron hole (eh)-pair excitation spectra during the non-adiabatic vibrational damping of adsorbates on metal surfaces. Our analysis for the…

化学物理 · 物理学 2017-11-22 Simon P. Rittmeyer , Jörg Meyer , Karsten Reuter

We reveal the existence of high-density Feshbach resonances in the collision between the ground and metastable states of $^{171}$Yb and coherently produce the associated Feshbach molecules by photoassociation. The extremely small transition…

原子物理 · 物理学 2016-02-01 Shintaro Taie , Shunsuke Watanabe , Tomohiro Ichinose , Yoshiro Takahashi

We present quantitative measurements of the photoassociation of cesium molecules inside a far-detuned optical dipole trap. A model of the trap depletion dynamics is derived which allows to extract absolute photoassociation rate coefficients…

原子物理 · 物理学 2009-11-10 R. Wester , S. D. Kraft , M. Mudrich , M. U. Staudt , J. Lange , N. Vanhaecke , O. Dulieu , M. Weidemuller

We determine the wavefunctions of electrons bound to a positively charged mesoscopic metallic cluster covered by an insulating surface layer. The radius of the metal core and the thickness of the insulating surface layer are of the order of…

介观与纳米尺度物理 · 物理学 2007-05-23 K. Dietrich , M. Garny , K. Pomorski

We study the steady state of a zero-temperature Bose gas near a Feshbach or photoassociation resonance using a two-channel mean-field model that incorporates atomic and molecular condensates, as well as correlated atom pairs originating…

其他凝聚态物理 · 物理学 2009-11-13 Andrew Carmichael , Juha Javanainen

We study the association and dissociation dynamics of weakly bound heteronuclear Feshbach molecules using transverse RF-fields for expected parameters accessible through the microgravity environment of NASA's Cold Atom Laboratory (CAL)…

原子物理 · 物理学 2017-02-01 J. P. D'Incao , M. Krutzik , E. Elliott , J. R. Williams

We present experimental results for dissociative electron attachment to acetylene near the 3 eV $^2\Pi_g$ resonance. In particular, we use an ion-momentum imaging technique to investigate the dissociation channel leading to C$_2$H$^-$…

化学物理 · 物理学 2014-10-29 M. Fogle , D. J. Haxton , A. L. Landers , A. E. Orel , T. N. Rescigno

We prove the limiting absorption principle for a dressed electron at a fixed total momentum in the standard model of non-relativistic quantum electrodynamics. Our proof is based on an application of the smooth Feshbach-Schur map in…

数学物理 · 物理学 2012-10-25 T. Chen , J. Faupin , J. Froehlich , I. M. Sigal