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We investigate the absorption line shapes of laser-dressed atoms beyond the single-atom response, by using extreme ultraviolet (XUV) attosecond pulse trains to probe an optically thick helium target under the influence of a strong infrared…

原子物理 · 物理学 2015-06-24 Chen-Ting Liao , Arvinder Sandhu , Seth Camp , Kenneth J. Schafer , Mette B. Gaarde

Attosecond pulses can be used to initiate and control electron dynamics on a sub-femtosecond time scale. The first step in this process occurs when an atom absorbs an ultraviolet photon leading to the formation of an attosecond electron…

原子物理 · 物理学 2007-12-11 P. Johnsson , J. Mauritsson , T. Remetter , A. LHuillier , K. J. Schafer

We present an innovative beamline for extreme ultraviolet (XUV)-infrared (IR) pump-probe reflection spectroscopy in solids with attosecond temporal resolution. The setup uses an actively stabilized interferometer, where attosecond pulse…

Attosecond pulses in the soft-X-ray (SXR) to water-window energy region offer the tools for creating and studying target specific localized inner-shell electrons or holes in materials, enable monitoring or controlling charge and energy…

原子与分子团簇 · 物理学 2020-03-25 Zhao Xi , Wang Su-Ju , Yu Wei-Wei , Wei Hui , Lin C. D

The harmonic emission from cluster nanoplasmas subject to short, intense infrared laser pulses is analyzed by means of particle-in-cell simulations. A pronounced resonant enhancement of the low-order harmonic yields is found when the Mie…

等离子体物理 · 物理学 2009-11-13 M. Kundu , S. V. Popruzhenko , D. Bauer

The motion of electrons and ions in medium-sized rare gas clusters (1000 atoms) exposed to intense laser pulses is studied microscopically by means of classical molecular dynamics using a hierarchical tree code. Pulse parameters for optimum…

原子与分子团簇 · 物理学 2007-05-23 Ulf Saalmann , Jan-Michael Rost

The ability to perform attosecond-pump attosecond-probe spectroscopy (APAPS) is a longstanding goal in ultrafast science. While first pioneering experiments demonstrated the feasibility of APAPS, the low repetition rates (10-120 Hz) and the…

We combine different wavelengths from an intense high-order harmonics source with variable delay at the focus of a split-mirror interferometer to conduct pump-probe experiments on gas-phase molecules. We report measurements of the time…

化学物理 · 物理学 2015-05-27 T. K. Allison , T. W. Wright , A. M. Stooke , C. Khurmi , J. van Tilborg , Y. Liu , R. W. Falcone , A. Belkacem

The early stage density oscillations of the electronic charge in molecules irradiated by an attosecond XUV pulse takes place on femto- or subfemtosecond timescales. This ultrafast charge migration process is a central topic in attoscience…

介观与纳米尺度物理 · 物理学 2018-03-16 E. Perfetto , D. Sangalli , A. Marini , G. Stefanucci

Ultrafast laser excitation can create coherent superpositions of electronic states in molecules and trigger ultrafast flow of electron density on few- to sub-femtosecond time scales. While recent attosecond experiments have addressed…

化学物理 · 物理学 2020-11-18 Yuki Kobayashi , Daniel M. Neumark , Stephen R. Leone

Parametric amplification of attosecond coherent pulses around 100 eV at the single-atom level is demonstrated for the first time by using the 3D time-dependent Schr{\"o}dinger equation in high-harmonic generation processes from excited…

光学 · 物理学 2020-08-26 C. Serrat , J. Seres , E. Seres , T-H. Dinh , N. Hasegawa , M. Nishikino , S. Namba

The interaction of high-intensity laser pulses and solid targets provides a promising way to create compact, tunable and bright XUV attosecond sources that can become a unique tool for a variety of applications. However, it is important to…

等离子体物理 · 物理学 2018-10-17 M. Blanco , M. T. Flores-Arias , A. Gonoskov

Clusters excited by intense laser pulses are a unique source of warm dense matter, that has been the subject of intensive experimental studies. The majority of those investigations concerns atomic clusters, whereas the evolution of…

原子与分子团簇 · 物理学 2015-06-18 M. Negro , H. Ruf , B. Fabre , F. Dorchies , M. Devetta , D. Staedter , C. Vozzi , Y. Mairesse , S. Stagira

This work theoretically investigates high-order harmonic generation in rare gas atoms driven by two temporally delayed ultrashort laser pulses. Apart from their temporal delay, the two pulses are identical. Using a single-atom model of the…

Sub-angstrom spatial resolution of electron density coupled with sub-femtosecond temporal resolution is required to directly observe the dynamics of the electronic structure of a molecule after photoinitiation or some other ultrafast…

Manipulation of intense pulse propagation in gas-filled capillaries is desirable for various high-field applications. Tuning the parameters of the driving laser pulse and the working gas is the conventional approach, and it provides limited…

光学 · 物理学 2023-09-27 Lize Han , Xiaohui Gao

The processing of energy by transfer and redistribution plays a key role in the evolution of dynamical systems. At the ultrasmall and ultrafast scale of nanosystems, quantum coherence could in principle also play a role and has been…

Context: Long-period intensity pulsations were recently detected in the EUV emission of coronal loops, and have been attributed to cycles of plasma evaporation and condensation driven by thermal non-equilibrium (TNE). Numerical simulations…

太阳与恒星天体物理 · 物理学 2020-02-12 Gabriel Pelouze , Frédéric Auchère , Karine Bocchialini , Clara Froment , Susanna Parenti , Elie Soubrié

Tremendous advances in laser pump-probe techniques open the door for the observation in real time of ultrafast \textit{electronic} processes. Particularly attractive is the visualization of interatomic processes where one can follow the…

原子与分子团簇 · 物理学 2007-05-23 Alexander I. Kuleff , Lorenz S. Cederbaum

We examine the effect of cluster size on the interaction of Ar$_{55}$-Ar$_{2057}$ with intense extreme ultraviolet (XUV) pulses, using a model we developed earlier that includes ionization via collisional excitation as an intermediate step.…

原子物理 · 物理学 2015-05-20 Edward Ackad , Nicolas Bigaouette , Kyle Briggs , Lora Ramunno