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When the phonon spectrum of a material is measured in a scattering experiment, selection rules preclude the observation of phonons that are odd under reflection by the scattering plane. Understanding these rules is crucial to correctly…

介观与纳米尺度物理 · 物理学 2015-01-16 Fernando de Juan , Antonio Politano , Gennaro Chiarello , Herbert A. Fertig

We compute lattice dynamical properties of iron at the bcc-fcc phase transition using dynamical mean-field theory implemented with the frozen-phonon method. Electronic correlations are found to have a strong effect on the lattice stability…

材料科学 · 物理学 2015-05-30 I. Leonov , A. I. Poteryaev , V. I. Anisimov , D. Vollhardt

The standard theoretical understanding of the lattice thermal conductivity, $\kappa_{\ell}$, of semiconductor alloys assumes that mass disorder is the most important source of phonon scattering. In contrast, we show that the hitherto…

材料科学 · 物理学 2018-10-03 Marco Arrigoni , Jesús Carrete , Natalio Mingo , Georg K. H. Madsen

The occurrence of thermal transport phenomena is widespread, exerting a pivotal influence on the functionality of diverse electronic and thermo-electric energy-conversion devices. The traditional first-principles theory governing the…

材料科学 · 物理学 2026-05-20 Soham Mandal , Manish Jain , Prabal K. Maiti

The four A1-TO Gamma phonon frequencies in lithium tantalate are calculated in the frozen-phonon approach from first principles using the full-potential linearized augmented plane wave method. A good agreement with the experimental data…

材料科学 · 物理学 2009-11-07 V. Caciuc , A. V. Postnikov

Lithium transition metal phospho-olivines are useful electrode materials, owing to their stability, high safety, low cost and cyclability. We report phonon studies using neutron inelastic scattering experiments, ab-initio density functional…

We investigated the lattice dynamics of the unconventional superconductor LiFeAs using inelastic neutron scattering experiments and density-functional theory (DFT) calculations. By comparing the neutron scattering intensities with…

Near-forward Raman scattering combined with ab initio phonon and bond length calculations is used to study the phonon-polariton transverse optical modes (with mixed electrical and mechanical character) of the II-VI ZnSeS mixed crystal under…

Grimme's DFT-D dispersion contribution to interatomic forces constants, required for the computation of the phonon band structures in density-functional perturbation theory, has been derived analytically. The implementation has then been…

材料科学 · 物理学 2018-01-29 Benoit Van Troeye , Marc Torrent , Xavier Gonze

We propose a new semiclassical approach based on the dynamical mean field theory to treat the interactions of electrons with local lattice fluctuations. In this approach the classical (static) phonon modes are treated exactly whereas the…

强关联电子 · 物理学 2009-11-07 S. Blawid , A. Deppeler , A. J. Millis

Three-nucleon forces (3NF) are investigated from two-flavor lattice QCD simulations. We utilize the Nambu-Bethe-Salpeter (NBS) wave function to determine two-nucleon forces (2NF) and 3NF in the same framework. As a first exploratory study,…

We show an efficient way to compute the electron-phonon coupling constant, $\lambda$, and the superconducting transition temperature, Tc from first-principles calculations. This approach gives rapid convergence of Tc with respect to the…

超导电性 · 物理学 2017-10-11 Takashi Koretsune , Ryotaro Arita

A sharp stability analysis of atomistic-to-continuum coupling methods is essential for evaluating their capabilities for predicting the formation and motion of lattice defects. We formulate a simple one-dimensional model problem and give a…

数值分析 · 数学 2010-07-19 Matthew Dobson , Mitchell Luskin , Christoph Ortner

Electron-phonon and exciton-phonon interactions in nanoclusters are formulated and computed under the framework of GW-BSE (Bethe-Salpeter equation) approach. The phonon effect is modeled with the two-particle representation for the first…

介观与纳米尺度物理 · 物理学 2021-02-24 Taofang Zeng , Yi He

Phonon transmission across an interface between dissimilar crystalline solids is calculated using molecular dynamics simulations with interatomic force constants obtained from first principles. The results reveal that although inelastic…

计算物理 · 物理学 2015-06-09 Takuru Murakami , Takuma Hori , Takuma Shiga , Junichiro Shiomi

Raman spectroscopy experiments on single crystals of CuSb2O6 and CoSb2O6 quasi-one-dimensional antiferromagnets with trirutile crystal structure were performed, with a focus on the first material. The observed Raman-active phonon modes and…

强关联电子 · 物理学 2018-03-21 D. T. Maimone , A. B. Christian , J. J. Neumeier , E. Granado

We describe a semiconductor multilayer structure based in acoustic phonon cavities and achievable with MBE technology, designed to display acoustic phonon Bloch oscillations. We show that forward and backscattering Raman spectra give a…

材料科学 · 物理学 2009-11-10 N. D. Lanzillotti Kimura , A. Fainstein , B. Jusserand

Many calculations require a simple classical model for the interactions between sp^2-bonded carbon atoms, as in graphene or carbon nanotubes. Here we present a new valence force model to describe these interactions. The calculated phonon…

材料科学 · 物理学 2015-05-13 Vasili Perebeinos , J. Tersoff

Ga$_2$O$_3$ is a wide-bandgap material of interest for a wide variety of devices, many of these requiring heterostructures, for instance to achieve carrier confinement. A common method to create such heterostructures is to alloy with…

材料科学 · 物理学 2024-01-26 Sierra Seacat , John L. Lyons , Hartwin Peelaers

Understanding and predicting lattice dynamics in strongly anharmonic crystals is one of the long-standing challenges in condensed matter physics. Here we propose a first-principles method that gives accurate quasiparticle (QP) peaks of the…

材料科学 · 物理学 2022-11-09 Terumasa Tadano , Wissam A. Saidi