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The activated surface diffusion of interacting adsorbates is described in terms of the so-called interacting single adsorbate approximation, which is applied to the diffusion of Na atoms on Cu(001) for coverages up to 20% in quasielastic He…

统计力学 · 物理学 2008-03-11 R. Martinez-Casado , J. L. Vega , A. S. Sanz , S. Miret-Artes

Here, an approach in terms of shot noise is proposed to study and characterize surface diffusion and low vibrational motion when having interacting adsorbates on surfaces. In what we call statistical limit, that is, at long times and high…

统计力学 · 物理学 2007-06-13 R. Martinez-Casado , J. L. Vega , A. S. Sanz , S. Miret-Artes

The experimental line shape broadening observed in adsorbate diffusion on metal surfaces with increasing coverage is usually related to the nature of the adsorbate-adsorbate interaction. Here we show that this broadening can also be…

统计力学 · 物理学 2007-06-13 R. Martinez-Casado , J. L. Vega , A. S. Sanz , S. Miret-Artes

The diffusion and low vibrational motions of adsorbates on surfaces can be well described by a purely stochastic model, the so-called interacting single adsorbate model, for low-moderate coverages (\theta \lesssim 0.12). Within this model,…

统计力学 · 物理学 2010-02-16 R. Martinez-Casado , A. S. Sanz , G. Rojas-Lorenzo , S. Miret-Artes

Surface diffusion of small adsorbates is analyzed in terms of the so-called intermediate scattering function and dynamic structure factor, observables in experiments using the well-known quasielastic Helium atom scattering and Helium spin…

统计力学 · 物理学 2018-09-26 S. Miret-Artés

Diffusion studies of adsorbates moving on a surface are often analyzed using 2D Langevin simulations. These simulations are computationally cheap and offer valuable insight into the dynamics, however, they simplify the complex interactions…

材料科学 · 物理学 2015-05-28 Moshe Diamant , Saar Rahav , Riccardo Ferrando , Gil Alexandrowicz

Nanoscopic diffusion at surfaces normally takes place when an adsorbate jumps from one adsorption site to the other. Jump diffusion can be measured via quasi-elastic scattering experiments, and the results can often be interpreted in terms…

计算物理 · 物理学 2021-05-18 Yaqing Xy Wang , Jack Kelsall , Nadav Avidor

A quantum Markovian activated atom-surface diffusion model with interacting adsorbates is proposed for the intermediate scattering function, which is shown to be complex-valued and factorizable into a classical-like and a quantum-mechanical…

统计力学 · 物理学 2008-11-14 R. Martinez-Casado , A. S. Sanz , S. Miret-Artes

The ad-atom dynamic equation, a Langevin type equation is analyzed and solved using some non-linear analytical and numerical tools. We noticeably show that the effect of the surface acoustic wave is to induce an effective potential that…

其他凝聚态物理 · 物理学 2012-03-14 Nicolas Combe , C. Taillan , J. Morillo

The effect of a standing acoustic wave on the diffusion of an ad-atom on a crystalline surface is theoretically studied. We used an unidimensional space model to study the ad-atom+substrate system. The dynamic equation of the ad-atom, a…

其他凝聚态物理 · 物理学 2015-06-04 Nicolas Combe , C. Taillan , J. Morillo

Activated surface diffusion with interacting adsorbates is analyzed within the Linear Response Theory framework. The so-called interacting single adsorbate model is justified by means of a two-bath model, where one harmonic bath takes into…

统计力学 · 物理学 2010-05-11 R. Martinez-Casado , A. S. Sanz , J. L. Vega , G. Rojas-Lorenzo , S. Miret-Artes

Collective diffusion coefficient in a one dimensional lattice gas adsorbate is calculated using variational approach. Particles interact via either a long-range, or a long range electron-gas-mediated (for a metallic substrate), or a…

材料科学 · 物理学 2009-05-26 Filip Krzyżewski , Magdalena A. Załuska-Kotur

Atomic diffusion is usually understood as a succession of random, independent displacements of an adatom over the surface's potential energy landscape. Nevertheless, an analysis of Molecular Dynamics simulations of self-diffusion on Cu(111)…

其他凝聚态物理 · 物理学 2016-08-16 J. Ferrón , L. Gómez , J. J. de Miguel , R. Miranda

A simple manner to describe the diffusive relaxation of a colloidal fluid adsorbed in a porous medium is to model the porous medium as a set of spherical particles fixed in space at random positions with prescribed statistical structural…

Surface nanobubbles are nanoscopic spherical-cap shaped gaseous domains on immersed substrates which are stable, even for days. After the stability of a {\it single} surface nanobubble has been theoretically explained, i.e. contact line…

流体动力学 · 物理学 2020-02-06 Xiaojue Zhu , Roberto Verzicco , Xuehua Zhang , Detlef Lohse

We present a numerical study of classical particles diffusing on a solid surface. The particles' motion is modeled by an underdamped Langevin equation with ordinary thermal noise. The particle-surface interaction is described by a periodic…

统计力学 · 物理学 2009-11-10 J. M. Sancho , A. M. Lacasta , K. Lindenberg , I. M. Sokolov , A. H. Romero

The behavior of colloidal particles with a hard core and a soft shell has attracted the attention for researchers in the physical-chemistry interface not only due the large number of applications, but due the unique properties of these…

软凝聚态物质 · 物理学 2021-02-23 Murilo S. Marques , José Rafael Bordin

We study the dynamics of generic reaction-diffusion fronts, including pulses and chemical waves, in the presence of multiplicative noise. We discuss the connection between the reaction-diffusion Langevin-like field equations and the…

统计力学 · 物理学 2009-11-07 A. Rocco , L. Ramirez-Piscina , J. Casademunt

We derive and study stochastic dissipative dynamics on coadjoint orbits by incorporating noise and dissipation into mechanical systems arising from the theory of reduction by symmetry, including a semidirect-product extension. Random…

动力系统 · 数学 2017-08-02 Alexis Arnaudon , Alex L. Castro , Darryl D. Holm

Advances in nanotechnology have allowed scientists to study biological processes on an unprecedented nanoscale molecule-by-molecule basis, opening the door to addressing many important biological problems. A phenomenon observed in recent…

应用统计 · 统计学 2008-07-25 S. C. Kou
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