相关论文: Photon Statistics for Single Molecule Non-Linear S…
We apply input-output theory with quantum pulses [AH Kiilerich, K M\o lmer, Phys. Rev. Lett. {\bf 123}, 123604 (2019)] to a model of a new type of two-photon detector consisting of one molecule that can detect two photons arriving…
In recent studies [Liew et al., Phys. Rev. Lett. 104, 183601 (2010); Bamba et al., Phys. Rev. A 83, 021802(R) (2011)], due to destructive interference between different paths for two-photon excitation, strong photon antibunching can be…
We study the fundamental limits of the precision of estimating parameters of a quantum matter system when it is probed by a travelling pulse of quantum light. In particular, we focus on the estimation of the interaction strength between the…
Using cumulant expansion in Gaussian approximation, the internal quantum statistics of damped soliton-like pulses in Kerr media are studied numerically, considering both narrow and finite bandwidth spectral pulse components. It is shown…
We suggest an approach to detect the conformation of single molecule by using the photon counting statistics. The generalized Smoluchoswki equation is employed to describe the dynamical process of conformational change of single molecule.…
We theoretically study how time- and angle-resolved photoemission spectroscopy can be applied for imaging coherent electron dynamics in molecules. We consider a process in which a pump pulse triggers coherent electronic dynamics in a…
Statistical properties of optical fields in nonlinear couplers composed of two waveguides in which Raman or Brillouin processes (with classical pumping) are in operation and which are mutually connected through the Stokes and/or anti-Stokes…
We apply the Kubo-Anderson stochastic theory of molecular spectral lineshape to the case of polaritons formed in the collective strong coupling regime. We investigate both the fast and slow limits of the random frequency modulation of the…
We investigate the distribution of number of photons emitted by a single molecule undergoing a spectral diffusion process and interacting with a continuous wave field. Using a generating function formalism an exact analytical formula for…
Streaking of photoelectrons has long been used for the temporal characterization of attosecond extreme ultraviolet pulses. When the time-resolved photoelectrons originate from a coherent superposition of electronic states, they carry an…
The widely used experimental technique of continuous-wave detection assumes counting pulses of photocurrent from a click-type detector inside a given measurement time window. With such a procedure we miss out the photons detected after each…
We derive photon counting statistics for an output field of a single-photon wave packet interacting with a quantum system (e.g. a quantum harmonic oscillator or a two-level atom). We determine the exclusive probability densities for the…
The nonlinear photon-photon interaction mediated by a single two-level atom is studied theoretically based on a one-dimensional model of the field-atom interaction. This model allows us to determine the effects of an atomic nonlinearity on…
We introduce a stochastic multi-photon dynamics on reciprocal space. Assuming isotropy, we derive the diffusion limit for a tagged photon to be a nonlinear Markov process on frequency. The nonlinearity stems from the stimulated emission. In…
Single molecule spectroscopy aims at unveiling often hidden but potentially very important contributions of single entities to a system's ensemble response. Albeit contributing tremendously to our ever growing understanding of molecular…
A practical quantum measurement method based on the quantum nature of anti-bunching photon emission has been developed to detect single particles without the restriction of the diffraction limit. By simultane- ously counting the…
We investigate the photon statistics of light emitted from a system of collectively interacting dipoles in the low-intensity regime, incorporating double-excitation states to capture beyond-single-excitation effects. By analyzing the…
The generation of non-classical states of light via photon blockade with time-modulated input is analyzed. We show that improved single photon statistics can be obtained by adequately choosing the parameters of the driving laser pulses. An…
In the solid state, a large variety of single-photon emitters present high quality photophysical properties together with a potential for integration. However, in many cases, the host matrix induces fluctuations of the emission wavelength…
Revivals of optical coherence of molecular photoassociation driven by two ultrashort laser pulses are addressed in the Condon approach. Based on textbook examples and numerical simulation of KrF excimer molecules, a prediction is made about…