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We conduct polarization-dependent ultrafast spectroscopy to study the dynamics of singlet fission in tetracene single crystals. The spectrotemporal species for singlet and triplet excitons in transient absorption spectra are found to be…

材料科学 · 物理学 2015-06-23 Bo Zhang , Chunfeng Zhang , Yanqing Xu , Rui Wang , Bin He , Yunlong Liu , Shimeng Zhang , Xiaoyong Wang , Min Xiao

In semiconductors, quantum confinement can greatly enhance the interaction between band carriers (electrons and holes) and dopant atoms. One manifestation of this enhancement is the increased stability of exciton magnetic polarons in…

介观与纳米尺度物理 · 物理学 2017-04-27 W. D. Rice , W. Liu , V. Pinchetti , D. R. Yakovlev , V. I. Klimov , S. A. Crooker

We employ five {\pi}-conjugated model materials of different molecular shape --- oligomers and cyclic structures --- to investigate the extent of exciton self-trapping and torsional motion of the molecular framework following optical…

Polaritons, formed as a result of strong hybridization of matter with light, are promising for important applications including organic solar cells, optical logic gates, and qubits. Owing to large binding energies of Frenkel excitons…

Exciton dynamics can be strongly affected by lattice vibrations through electron-phonon coupling. This is rarely explored in two-dimensional magnetic semiconductors. Focusing on bilayer CrI3, we first show the presence of strong…

The interactions between charges and excitons involve complex many-body interactions at high densities. The exciton-polaron model has been adopted to understand the Fermi sea screening of charged excitons in monolayer transition metal…

介观与纳米尺度物理 · 物理学 2023-09-14 Xin Cong , Parisa Ali Mohammadi , Mingyang Zheng , Kenji Watanabe , Takashi Taniguchi , Daniel Rhodes , Xiao-Xiao Zhang

We use path integral Monte Carlo to study the energetics of excitons in layered, hybrid organic-inorganic perovskites in order to elucidate the relative contributions of dielectric confinement and electron-phonon coupling. While the…

材料科学 · 物理学 2025-03-26 Rohit Rana , David T. Limmer

We provide a self-contained review of master equation approaches to modelling phonon effects in optically driven self-assembled quantum dots. Coupling of the (quasi) two-level excitonic system to phonons leads to dissipation and dephasing,…

介观与纳米尺度物理 · 物理学 2016-06-14 Ahsan Nazir , Dara P. S. McCutcheon

Biluminescent organic emitters show simultaneous fluorescence and phosphorescence at room temperature. So far, the optimization of the room temperature phosphorescence (RTP) in these materials has drawn the attention of research. However,…

The fluorescence of triplet excitons and color-centers is strongly dependent on magnetic field that mixes the zero field spin eigenstates that determine the radiative recombination rates back into the singlet ground state through spin-orbit…

介观与纳米尺度物理 · 物理学 2025-12-08 Yan Sun , A. D. Chepelianskii

We investigate theoretically the magnetoplasmon (cyclotron) resonance in a hybrid system consisting of spatially separated two-dimensional layers of electron and dipolar exciton gases coupled via the Coulomb forces. We study the dynamics of…

介观与纳米尺度物理 · 物理学 2018-04-25 M. V. Boev , V. M. Kovalev , I. G. Savenko

In organic semiconductor based bulk heterojunction solar cells, the presence of acceptor increases the formation of charge transfer (CT) excitons, thereby leading to higher exciton dissociation probabilities. In this work we used steady…

Strong light-matter coupling to form exciton- and vibropolaritons is increasingly touted as a powerful tool to alter the fundamental properties of organic materials. It is proposed that these states and their facile tunability can be used…

Several microscopic pathways have been proposed to explain the large magnetic effects observed in organic semiconductors, but identifying and characterising which microscopic process actually influences the overall magnetic field response…

介观与纳米尺度物理 · 物理学 2015-06-11 T. L. Keevers , W. J. Baker , D. R. McCamey

Charged magneto-excitons X- in a dilute 2D electron gas in narrow and symmetric quantum wells are studied using exact diagonalization techniques. An excited triplet X- state with a binding energy of about 1 meV is found. This state and the…

介观与纳米尺度物理 · 物理学 2009-10-31 Arkadiusz Wojs , John J. Quinn , Pawel Hawrylak

We analyze theoretically magnetoresistance of high mobility two-dimensional electron systems being illuminated by multiple radiation sources. In particular, we study the influence on the striking effect of microwave-induced resistance…

介观与纳米尺度物理 · 物理学 2015-05-28 Jesus Inarrea

Thin films of high-refractive-index excitonic materials enable self-coupling by simultaneously supporting intrinsic excitonic transitions and optical resonances. These optical resonances take the form of Fabry-Perot resonances in thick…

We studied the possibility of exciton condensation in Mott insulating bilayers. In these strongly correlated systems an exciton is the bound state of a double occupied and empty site. In the strong coupling limit the exciton acts as a…

强关联电子 · 物理学 2014-01-01 Louk Rademaker , Jeroen van den Brink , Jan Zaanen , Hans Hilgenkamp

Polarization resolved photoluminescence (PL) spectroscopy of individual CdTe/ZnTe quantum dots is investigated in the presence of external in-plane magnetic field. We find that the excitonic fine structure strongly depends on the magnitude…

其他凝聚态物理 · 物理学 2009-02-25 K. Kowalik , O. Krebs , A. Golnik , J. Suffczynski , P. Wojnar , J. Kossut , J. A. Gaj , P. Voisin

Layered 2D organic-inorganic perovskite semiconductors support strongly confined excitons that offer significant potential for ultrathin polaritonic devices due to their tunability and huge oscillator strength. The application of a magnetic…

介观与纳米尺度物理 · 物理学 2025-02-26 Jonas K. König , Jamie M. Fitzgerald , Ermin Malic