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We examine the quantum tunneling of magnetization in molecular spin in weak interaction with a bath subject to Redfield master equation. By designing a microscopic model for a multilevel spin system using only a generic Hamiltonian and…

材料科学 · 物理学 2022-12-27 Le Tuan Anh Ho , Liviu Ungur , Liviu F. Chibotaru

The crossover between thermally assisted and pure quantum tunneling has been studied in single crystals of high spin (S=10) uniaxial molecular magnet Mn12 using micro-Hall-effect magnetometry. Magnetic hysteresis and relaxation experiments…

介观与纳米尺度物理 · 物理学 2009-11-07 Louisa Bokacheva , Andrew D. Kent , Marc A. Walters

Quantum annealing, which involves quantum tunnelling among possible solutions, has state-of-the-art applications not only in quickly finding the lowest-energy configuration of a complex system, but also in quantum computing. Here we report…

强关联电子 · 物理学 2024-11-28 Yuqian Zhao , Zhaohua Ma , Zhangzhen He , Haijun Liao , Yan-Cheng Wang , Junfeng Wang , Yuesheng Li

We perform a quantum simulation of the Ising model with a transverse field using a collection of three trapped atomic ion spins. By adiabatically manipulating the Hamiltonian, we directly probe the ground state for a wide range of fields…

We investigate the thermally activated magnetization switching of small ferromagnetic particles driven by an external magnetic field. For low uniaxial anisotropy the spins can be expected to rotate coherently, while for sufficient large…

统计力学 · 物理学 2009-10-31 D. Hinzke , U. Nowak

Using exact diagonalization method,we studied the ground state of the anisotropic molecular magnets and find a critical point in the transverse field,which may divide the quantum tunneling region into two different parts. Possible ways to…

介观与纳米尺度物理 · 物理学 2007-05-23 Yongjin Jiang , Haijin Li , Ruibao Tao

We have studied the crossover between thermally assisted and pure quantum tunneling in single crystals of high spin (S=10) uniaxial single molecule magnet Mn12-acetate using micro-Hall effect magnetometry. Magnetic hysteresis experiments…

介观与纳米尺度物理 · 物理学 2007-05-23 Louisa Bokacheva , Andrew D. Kent , Marc A. Walters

In an effort to understand the low temperature behavior of recently synthesized molecular magnets we present numerical evidence for the existence of a rotational band in systems of quantum spins interacting with nearest-neighbor…

材料科学 · 物理学 2009-10-31 J. Schnack , Marshall Luban

It is shown that a single molecular magnet placed in a rapidly oscillating magnetic field displays the phenomenon of quenching of tunneling processes. The results open a way to manipulate the quantum states of molecular magnets by means of…

介观与纳米尺度物理 · 物理学 2015-12-09 María José Santander , Alvaro S. Nunez , A. Roldán-Molina , Roberto E. Troncoso

The spin-1/2 Hamiltonian for two coupled isosceles Heisenberg triangles, which is well suited for describing the V$_6$-type magnetic molecules, is studied by exact diagonalization. The quantum phase transition diagram, at zero temperature,…

统计力学 · 物理学 2020-12-30 J. Torrico , J. A. Plascak

The time-dependent transport through single-molecule magnets coupled to magnetic or non-magnetic electrodes is studied in the framework of the generalized master equation method. We investigate the transient regime induced by the periodic…

介观与纳米尺度物理 · 物理学 2015-09-02 V. Moldoveanu , I. V. Dinu , B. Tanatar , C. P. Moca

We consider transport through a single-molecule magnet strongly coupled to metallic electrodes. We demonstrate that for half-integer spin of the molecule electron- and spin-tunneling \emph{cooperate} to produce both quantum tunneling of the…

强关联电子 · 物理学 2009-11-11 C. Romeike , M. R. Wegewijs , W. Hofstetter , H. Schoeller

We consider a prototypical system of an infinite range transverse field Ising model coupled to a bosonic bath. By integrating out the bosonic degrees, an effective anisotropic Heisenberg model is obtained for the spin system. The phase…

统计力学 · 物理学 2011-04-29 Subhasis Sinha , Sushanta Dattagupta

The behavior of molecular nanomagnets in periodic magnetic field transverse to the easy axis direction is investigated. It is shown that at sufficiently strong field the tunneling time can be considerably reduced.

介观与纳米尺度物理 · 物理学 2009-11-07 N. A. Sinitsyn

The quantum tunneling of the magnetization vector are studied theoretically in single-domain ferromagnetic nanoparticles placed in an external magnetic field at an arbitrarily directed angle in the $ZX$ plane. We consider the…

统计力学 · 物理学 2009-10-31 Rong Lu , Jia-Lin Zhu , Zhi-Rong Liu , Lee Chang , Bing-Lin Gu

The reversal of the magnetization of crystals of molecular magnets that have a large spin and high anisotropy barrier generally proceeds below the blocking temperature by quantum tunneling. This is manifested as a series of controlled steps…

介观与纳米尺度物理 · 物理学 2013-02-21 Myriam P. Sarachik

Traditional simulated annealing utilizes thermal fluctuations for convergence in optimization problems. Quantum tunneling provides a different mechanism for moving between states, with the potential for reduced time scales. We compare…

凝聚态物理 · 物理学 2007-05-23 J. Brooke , D. Bitko , T. F. Rosenbaum , G. Aeppli

The systems exhibiting quantum phase transitions (QPT) are investigated within the Ising model in the transverse field and Heisenberg model with easy-plane single-site anisotropy. Near QPT a correspondence between parameters of these models…

凝聚态物理 · 物理学 2009-10-31 V. Yu. Irkhin , A. A. Katanin

How nanoscale uniaxial magnets respond to an alternating field is studied by direct numerical calculation. A nontrivial oscillation of the magnetization is found, which is analyzed in terms of the non-adiabatic transition due to the time…

凝聚态物理 · 物理学 2009-10-30 Seiji Miyashita , Keiji Saito , Hans De Raedt

We discuss numerical and theoretical results for models of magnetization switching in nanoparticles and ultrathin films. The models and computational methods include kinetic Ising and classical Heisenberg models of highly anisotropic…

材料科学 · 物理学 2007-05-23 Per Arne Rikvold , Gregory Brown , Steven J. Mitchell , M. A. Novotny
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