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We study the local structural changes along the jamming transitions in asymmetric bidisperse granu\-lar packings. The local structure of the packing is assessed by the contact orientational order, $\tilde{Q}_{\ell}$, that quantifies the…

软凝聚态物质 · 物理学 2024-11-06 Juan C. Petit , Matthias Sperl

Binary compositions of surface ligands are known to improve the colloidal stability and fluorescence quantum yield of nanocrystals (NCs), due to ligand-ligand interactions and surface organization. Herein, we follow the thermodynamics of a…

软凝聚态物质 · 物理学 2023-06-16 Orian Elimelech , Meirav Oded , Daniel Harries , Uri Banin

We study structural transitions in a system of interacting particles arranged as a crystalline bilayer, as a function of the density $\rho$ and the distance $d$ between the layers. As $d$ is decreased a sequence of transitions involving…

软凝聚态物质 · 物理学 2015-05-13 Tamoghna Das , Surajit Sengupta , Subhasis Sinha

The direct correlation function of a fluid mixture of parallel hard cubes is obtained by using Rosenfeld's fundamental measure approximation. This approximation is thermodynamically consistent (compressibility and virial equations of state…

凝聚态物理 · 物理学 2009-10-28 Jose A. Cuesta

We employ a molecular dynamics (MD) study to explore pattern selection in binary fluid mixtures ($AB$) undergoing surface-directed spinodal decomposition on a chemically patterned amorphous substrate. We chose a checkerboard pattern with…

软凝聚态物质 · 物理学 2025-12-12 Syed Shuja Hasan Zaidi , Hema Teherpuria , Santosh Mogurampelly , Prabhat K. Jaiswal

We investigate sedimentation of model hard sphere-like colloidal dispersions confined in horizontal capillaries using laser scanning confocal microscopy, dynamical density functional theory, and Brownian dynamics computer simulations. For…

软凝聚态物质 · 物理学 2009-11-13 C. Patrick Royall , Joachim Dzubiella , Matthias Schmidt , Alfons van Blaaderen

The structure of polydisperse hard sphere fluids, in the presence of a wall, is studied by the Rosenfeld density functional theory. Within this approach, the local excess free energy depends on only four combinations of the full set of…

软凝聚态物质 · 物理学 2009-10-31 I. Pagonabarraga , M. E. Cates , G. J. Ackland

We use numerical simulations to understand how random deviations from the ideal spherical shape affect the ability of hard particles to form fcc crystalline structures. Using a system of hard spheres as a reference, we determine the…

软凝聚态物质 · 物理学 2010-12-23 William L. Miller , Angelo Cacciuto

We investigate polydispersity effects on the average structure factor of colloidal suspensions of neutral particles with surface adhesion. A sticky hard sphere model alternative to Baxter's one is considered. The choice of factorizable…

统计力学 · 物理学 2009-11-07 Domenico Gazzillo , Achille Giacometti

For the binary discs packed in two dimensions, the packing fraction of disc assembly becomes lower than that of the monodisperse system when the size ratio is close to unity. We show that the suppressed packing fraction is caused by an…

无序系统与神经网络 · 物理学 2007-10-24 Takashi Odagaki , Tsuyoshi Okubo , Ryusei Ogata , Keiji Okazaki

Using Brownian dynamics computer simulations we show that binary mixtures of colloids driven in opposite directions by an oscillating external field exhibit axial segregation in sheets perpendicular to the drive direction. The segregation…

软凝聚态物质 · 物理学 2015-05-13 Adam Wysocki , Hartmut Löwen

Colloidal particles that are confined to an interface such as the air-water interface are an example of a two-dimensional fluid. Such dispersions have been observed to spontaneously form cluster and stripe morphologies in certain systems…

软凝聚态物质 · 物理学 2008-09-17 A. J. Archer

We present the results of an experimental study of patterned segregation in a horizontally shaken shallow layer of a binary mixture of dry particles. An order parameter for the segregated structures is defined and the effect of the…

软凝聚态物质 · 物理学 2009-11-07 Pedro M. Reis , Tom Mullin

We calculate the configurational entropy of colloidal particles in a confined geometry interacting as hard disks using Monte Carlo integration method. In particular, we consider systems with three kinds of boundary conditions: hard,…

软凝聚态物质 · 物理学 2023-01-23 Duanduan Wan

We investigate the phase behaviour of mixtures of two populations of colloidal particles dispersed in a binary solvent system near its critical composition. The surfaces of particles are chemically modified to elicit a specific solvent…

软凝聚态物质 · 物理学 2026-02-16 T. E. Kodger , N. Farahmand Bafi , M. Labbé-Laurent , E. Steijlen , A. Maciolek , P. Schall

The channel size distribution in hard sphere systems, based on the local neighbor correlation of four particle positions, is investigated for all volume fractions up to jamming. For each particle, all three particle combinations of…

无序系统与神经网络 · 物理学 2015-06-19 Vitaliy Ogarko , Nicolas Rivas , Stefan Luding

We use computer simulations to test a simple idea for mapping between long-time self diffusivities obtained from molecular and Brownian dynamics. The strategy we explore is motivated by the behavior of fluids comprising particles that…

软凝聚态物质 · 物理学 2011-10-25 Mark J. Pond , Jeffrey R. Errington , Thomas M. Truskett

Recent observations of supernovae (SNe) have indicated that a fraction of massive stars possess dense circumstellar medium (CSM) at the moment of their core collapses. They suggest the presence of additional activities of the SN progenitor…

太阳与恒星天体物理 · 物理学 2023-12-22 Tomoki Matsuoka , Ryo Sawada

A previously developed fundamental measure fucntional [J. Chem. Phys. vol.107, 6379 (1997)] is used to study the phase behavior of a system of parallel hard cubes. The single-component fluid exhibits a continuous transition to a solid with…

软凝聚态物质 · 物理学 2009-10-31 Y. Martinez-Raton , J. A. Cuesta

Understanding the phase behaviour of mixtures continues to pose challenges, even for systems that might be considered "simple". Here we consider a very simple mixture of two colloidal and one non-adsorbing polymer species which can be…