原子物理
The motion of an ion in a radiofrequency (rf) Paul trap is described by the Mathieu equation and the associated stability parameters that are proportional to the rf and dc electric field gradients. Here, a higher-order, iterative method to…
Robust and accurate acceleration tracking remains a challenge in many fields. For geophysics and economic geology, precise gravity mapping requires onboard sensors combined with accurate positioning and navigation systems. Cold-atom-based…
We report the measurement of the hyperfine splitting in the $7D_{5/2}$ state of $^{133}$Cs using high resolution Doppler-free two-photon spectroscopy enabled by precise frequency scans using an acousto-optic modulator. All the six hyperfine…
Closed analytical formulas are derived for the differential and total cross sections of the non-relativistic photoelectric effect in the three main classes of few-electron atomic systems: (1) neutral atoms and positively charged atomic ions…
It is demonstrated that the use of a Micrometric Thin $^{39}$K vapor Cell (MTC) and Saturated Absorption spectroscopy (SA) allows to form narrow atomic lines in transmission spectrum without unwanted Cross-Over (CO) resonances. Another…
The measurement precision of the static atomic gravimetry is limited by white Gaussian noise in short term, which costs previous works an inevitable integration to reach the precision demanded. Here, we propose a statistical model based on…
Molecular design principles provide guidelines for augmenting a molecule with a smaller group of atoms to realize a desired property or function. We demonstrate that these concepts can be used to create an optical cycling center that can be…
We report new experimental hyperfine structure (HFS) constants of neutral and singly ionized scandium (Sc I and Sc II). We observed spectra of Sc-Ar and Sc-Ne hollow cathode discharges in the region 200-2500 nm (50,000-4000 cm$^{-1}$) using…
Molecular hydrogen ions in weakly bound states close to the first dissociation threshold are attractive quantum sensors for measuring the proton-to-electron mass ratio and hyperfine-induced ortho-para mixing. The experimental accuracy of…
We report on the fragmentation dynamics of triply charged, diatomic, molecular ions of NO and CO. Dissociative fragmentation after multiple ionization of NO and CO is studied under the impact of 200 keV proton beam using recoil-ion momentum…
Michel Barat passed away in November 2018 at the age of 80 after a rich career in atomic and molecular collisions. He had participated actively in formalizing to the electron promotion model, contributed to low energy reactive collisions at…
Prompted by recent experimental developments, a theory of surface scattering of fast atoms at grazing incidence is developed. The theory gives rise to a quantum mechanical limit for ordered surfaces that describes coherent diffraction peaks…
The Matter-wave laser Interferometric Gravitation Antenna (MIGA) is an underground instrument using cold-atom interferometry to perform precision measurements of gravity gradients and strains. Following its installation at the low noise…
This work discusses a protocol for constructing highly accurate potential energy curves (PECs) for the lowest two states of Rb$_{2}^+$, i.e. $X\,{}^2{\Sigma}{_g^+}$ and $(1) {}^2\Sigma{_u^+}$, using an additivity scheme based on…
Laser cooling is a key ingredient for quantum control of atomic systems in a variety of settings. In divalent atoms, two-stage Doppler cooling is typically used to bring atoms to the uK regime. Here, we implement a pulsed radial cooling…
Motivated by the challenge of identifying intruder ions in a cold ion crystal, we investigate calorimetry from emitted fluorescence light. Under continuous Doppler cooling, the ion crystal reaches a temperature equilibrium with a fixed…
We have developed a Fock-space relativistic coupled-cluster theory based method for the calculation of electric dipole polarizability of one-valence atoms and ions. We employ this method to compute the ground-state and spin-orbit coupled…
We study the effect of Coulomb potential on high-order harmonic generation (HHG) numerically and analytically. We focus on the influence of Coulomb potential on emission times of HHG associated with specific electron trajectories. By using…
High-precision laser spectroscopy of atomic hydrogen has led to an impressive accuracy in tests of bound-state quantum electrodynamics (QED). At the current level of accuracy many systematics have to be studied very carefully and only…
The current status of tests of quantum electrodynamics with heavy ions is reviewed. The theoretical predictions for the Lamb shift and the hyperfine splitting in heavy ions are compared with available experimental data. Recent achievements…