原子物理
The accurate evaluation of the second-order Doppler frequency shift (SODFS) of trapped ions in a linear Paul trap has been studied with experiments and molecular dynamics (MD) simulations. The motion of trapped ions in the trap has three…
We obtain the interaction potential for NaCs by fitting to experiments on ultracold scattering and spectroscopy in optical tweezers. The central region of the potential has been accurately determined from Fourier-Transform spectroscopy at…
Previous work on imaging wave packet dynamics with x-ray scattering revealed that the scattering patterns deviate substantially from the notion of instantaneous momentum density of the wave packet. Here we show that scattering patterns can…
In this work, we apply the Monte Carlo wave packet method to study the ultrafast nuclear dynamics following inner-shell photoionization of N2 exposed to an ultrashort intense X-ray pulse. The photon energy of the X-ray pulse is large enough…
A detailed analysis of the bremsstrahlung spectrum at nonrelativistic electron scattering on argon and xenon is carried out. It is shown that the approximate formulas widely used for the description of bremsstrahlung spectra lead to…
Using radiometrically calibrated instrumentation of Physikalisch-Technische Bundesanstalt, the L-shell fluorescence yields and Coster-Kronig factors of tantalum (including the uncertainty budget) were experimentally determined based on…
The knowledge of atomic fundamental parameters, such as the fluorescence yields with low uncertainties, is of decisive importance in elemental quantification involving X-ray fluorescence analysis techniques. However, especially for the…
While it is straightforward to count laser-cooled trapped ions by fluorescence imaging, detecting the number of dark ions embedded and sympathetically cooled in a mixed ion crystal is more challenging. We demonstrate a method to track the…
We identify laser-accessible transitions in group 16-like highly charged ions as candidates for high-accuracy optical clocks, including S-, Se-, and Te-like systems. For this class of ions, the ground $^{3}P_{J}$ fine structure manifold…
Electromagnetically induced transparency (EIT) in atomic systems involving Rydberg states is known to be a sensitive probe of incident microwave (MW) fields, in particular those resonant with Rydberg-to-Rydberg transitions. Here we propose…
We report the measurement of hyperfine splitting in the $7d$ $^{2}D_{3/2}$ state of $^{133}$Cs using high resolution Doppler-free two-photon spectroscopy in a Cs vapor cell. We determine the hyperfine coupling constants $A = 7.3509(9)$ MHz…
Studies on the interactions between an alkali atom and an alkaline earth ion at low energy are important in the field of cold chemistry. In this paper we, extensively, study the structure, interactions, and dynamics of (MgCs)$^+$ molecular…
Quantum state-resolved spectroscopy was recently achieved for C60 molecules when cooled by buffer gas collisions and probed with a midinfrared frequency comb. This rovibrational quantum state resolution for the largest molecule on record is…
Optically trapped laser-cooled polar molecules hold promise for new science and technology in quantum information and quantum simulation. Large numerical aperture optical access and long trap lifetimes are needed for many studies, but these…
Large scale ab initio calculations of the electric contribution (i.e. the electric field gradient) to the electric quadrupole hyperfine interaction constants $B$ for the $5p~^2P_{3/2}$ state in $^{109}$Cd$^+$ ion and the $5s5p~^3P_{1,2}$…
We prepare mixtures of ultracold $^{39}$K atoms in various hyperfine spin states and $^{23}$Na$^{39}$K molecules in an optical dipole trap at a fixed magnetic field and study inelastic two-body atom-molecule collisions. We observe…
Light is a precious tool to probe matter, as it captures microscopic and macroscopic information on the system. We here report on the transition from a thermal (classical) to a spontaneous emission (quantum) mechanism for the loss of light…
We demonstrate a miniaturised and highly robust system for performing Doppler-free spectroscopy on thermal atomic vapour for three frequencies as required for cold atom-based quantum technologies. The application of additive manufacturing…
We report a high-finesse bow-tie cavity designed for atomic physics experiments with Rydberg atom arrays. The cavity has a finesse of $51,000$ and a waist of $7.1$ $\mu$m at the cesium D2 line ($852$ nm). With these parameters, the cavity…
On-resonance Rydberg atom-based radio-frequency (RF) electric field sensing methods remain limited by the narrow frequency signal detection bands available by resonant transitions. The use of an additional RF tuner field to dress or shift a…