软凝聚态物质
The observation of Liquid-Liquid Phase Separation (LLPS) in biological cells has dramatically shifted the paradigm that soluble proteins are uniformly dispersed in the cytoplasm or nucleoplasm. The LLPS region is preceded by a one-phase…
Knits and crochets are mechanical metamaterials with a long history and can typically be produced from a single yarn. Despite the simplicity of the manufacturing process, they exhibit a wide range of structural configurations with diverse…
The low complexity domain of Fused in Sarcoma (FUS-LC consisting of 214 residues) undergoes phase separation, resulting in a dense liquid-like phase that forms early and slowly matures to reach ordered gel-like state on long time scales.…
The environmental risks posed by traditional oil and grease-based lubricants can be significantly mitigated by adopting water-based alternatives engineered with superior rheological performance. In this work, we present a fundamentally new…
This paper deals with the condensation of liquid droplets on hydrophobic and hydrophilic surfaces. A stochastic mesoscale model based on the theory of fluctuating hydrodynamics and the thermodynamics of a diffuse interface approach shows…
The interaction lifetimes between condensate-forming biomolecules can dictate both the specificity of the condensate-forming species as well as the fluidity and exchange dynamics of these condensates. Using a heuristic modeling approach, we…
We present results of LAMMPS Molecular Dynamics simulations of 2D gravity-driven flows of 30,000 soft uniform spheres through a vertical silo. We vary the gravitational field (g), elastic modulus of the particles (E), and silo outlet…
This study employs modified Poisson-Boltzmann theory to systematically investigate the influence of zwitterionic osmolyte additives to an electrolyte solution on disjoining pressure and electric differential capacitance within charged…
Liquid crystalline networks (LCNs) are stimuli-responsive materials formed from polymeric chains cross-linked with rod-like mesogenic segments, which, in the nematic phase, align along a non-polar director. A key characteristic of these…
We study the self-assembly of magnetic colloids using the Stockmayer (SM) model characterized by short-range Lennard-Jones interactions and long-range dipole-dipole interactions. Using molecular dynamics simulations, we design cooling…
We analyze the stress tensor and the gyration tensor of an unentangled polymer melt under flow by using a Rouse-type single chain model. We employ the bead-spring type single chain model, in which beads interact each other via nonlinear…
We establish how active stress globally affects the morphology of disclination lines of a three dimensional active nematic liquid crystal under chaotic flow. Thanks to a defect detection algorithm based on the local nematic orientation, we…
This work establishes an exact relationship between the zero-shear viscosity and the radius of gyration for generalized Rouse model with arbitrary network configurations. Building on this fundamental relationship, we develop a random graph…
Molecular simulations provide an effective route for investigating morphology evolution and structure-property relationship in polymer-clay nanocomposites (PCNCs) incorporating layered silicates like montmorillonite (MMT), an important…
Vitrimers are a class of polymers characterized by dynamic covalent networks, where specific monomer units, which are know as stickers, form reversible crosslinks that enable network rearrangement without loss of overall connectivity. The…
Active nematic systems consist of rod-like internally driven subunits that interact with one another to form large-scale coherent flows. They are important examples of far-from-equilibrium fluids, which exhibit a wealth of nonlinear…
A nanocomposite film containing highly polarizable inclusions in a fluid background is explored when an external electric field is applied perpendicular to the planar film. For small electric fields, the induced dipole moments of the…
We use a semi-supervised, neural-network based machine learning technique, the confusion method, to investigate structural transitions in magnetic polymers, which we model as chains of magnetic colloidal nanoparticles characterized by…
For the fragile, low-molecular-weight liquid diglycidyl ether of bisphenol A (DGEBA), we report on the dynamic glass transition and a further acoustic anomaly in the vicinity of the thermal glass transition based on hypersonic…
The exceptional adhesion properties of biological fibrillar structures -- such as those found in geckos -- have inspired the development of synthetic adhesive surfaces. Among these, mushroom-shaped fibrils have demonstrated superior…