通过汉紫中的锶替代揭示三维量子临界性
强关联电子
2021-06-16 v2
摘要
经典与量子相变(QPTs)及其伴随的临界性与普适性概念,是统计热力学的基石。一个典型的受控量子相变是带隙量子磁体在磁场诱导下的磁有序。尽管已知众多“准一维”耦合自旋链与自旋梯材料的有序转变是三维(3D)的,但准二维系统因若干物理原因而特殊。受古代颜料汉紫(BaCuSiO,一种呈现反常临界性质的准二维材料)的启发,我们给出了对 BaSrCuSiO 的完整分析。我们通过中子谱测量零场磁激发并推导出磁哈密顿量。我们结合磁化率、比热、转矩与磁热测量以及近量子相变处的低温核磁共振研究,探测了磁场诱导的转变。通过贝叶斯统计分析与大规模量子蒙特卡洛模拟,我们明确证明:汉紫中轻量锶替代所引起的结构简化,恢复了可观测的三维量子临界标度。
引用
@article{arxiv.2103.06860,
title = {Revealing three-dimensional quantum criticality by Sr-substitution in Han Purple},
author = {Stephan Allenspach and Pascal Puphal and Joosep Link and Ivo Heinmaa and Ekaterina Pomjakushina and Cornelius Krellner and Jakob Lass and Gregory S. Tucker and Christof Niedermayer and Shusaku Imajo and Yoshimitsu Kohama and Koichi Kindo and Steffen Krämer and Mladen Horvatić and Marcelo Jaime and Alexander Madsen and Antonietta Mira and Nicolas Laflorencie and Frédéric Mila and Bruce Normand and Christian Rüegg and Raivo Stern and Franziska Weickert},
journal= {arXiv preprint arXiv:2103.06860},
year = {2021}
}
备注
19 pages, 5 figures