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We have studied the conformational and scaling behaviors of a flexible dendrimer immersed in athermal or good solvents. A self-consistent field theory combined with a pre-averaged excluded volume potential representing the two-body…

Soft Condensed Matter · Physics 2018-08-30 Meng Shi , Yingzi Yang , Feng Qiu

We investigate by means of a number of different dynamical Monte Carlo simulation methods the self-assembly of equilibrium polymers in dilute, semidilute and concentrated solutions under good-solvent conditions. In our simulations, both…

Statistical Mechanics · Physics 2009-10-31 J. P. Wittmer , P. van der Schoot , A. Milchev , J. -L. Barrat

We suggest a theoretical description of the force-induced translocation dynamics of a polymer chain through a nanopore. Our consideration is based on the tensile (Pincus) blob picture of a pulled chain and the notion of propagating front of…

Soft Condensed Matter · Physics 2012-04-17 J. L. A. Dubbeldam , V. G. Rostiashvili , A. Milchev , T. A. Vilgis

Conformational properties of regular dendrimers and more general hyperbranched polymer stars with Gaussian statistics for the spacer chains between branching points are revisited numerically. We investigate the scaling for asymptotically…

Soft Condensed Matter · Physics 2015-08-18 P. Polinska , C. Gillig , J. P. Wittmer , J. Baschnagel

We explore semi-dilute and concentrated oligomers and polymers in a broad range of polymerization indices N ranging from 1 to a 100 and in a range of monomer number densities $\phi$ from 0.1 to 0.8 via molecular dynamics simulations and…

Soft Condensed Matter · Physics 2020-12-01 Ashod Khederlarian , Carmen Almasri , Leonid Klushin

The non-equilibrium structural and dynamical properties of semiflexible polymers confined to two dimensions are investigated by molecular dynamics simulations. Three different scenarios are considered: The force-extension relation of…

Soft Condensed Matter · Physics 2013-01-08 A. Lamura , R. G. Winkler

We consider the thermal breakage of a tethered polymer chain of discrete segments coupled by Morse potentials under constant tensile stress. The chain dynamics at the onset of fracture is studied analytically by Kramers-Langer…

Soft Condensed Matter · Physics 2010-06-24 A. Ghosh , D. I. Dimitrov , V. G. Rostiashvili , A. Milchev , T. A. Vilgis

We elucidate the elastic behavior of a wormlike chain in 3D under compression and provide exact solutions for the experimentally accessible force-extension relation in terms of generalized spheroidal wave functions. In striking contrast to…

Soft Condensed Matter · Physics 2019-11-11 Christina Kurzthaler

We analyse the nature of the confinement of an infinitely long (and finite) linear semiflexible homo-polymer chain confined in between two geometrical constraints (A&B) under good solvent condition in two dimensions. The constraints are…

Soft Condensed Matter · Physics 2017-10-16 Pramod Kumar Mishra

We study the conformational properties of charged polymers in a solvent in the presence of structural obstacles correlated according to a power law $\sim x^{-a}$. We work within the continuous representation of a model of linear chain…

Soft Condensed Matter · Physics 2013-11-25 V. Blavatska , C. von Ferber

We study jamming in model freely rotating polymers as a function of chain length $N$ and bond angle $\theta_0$. The volume fraction at jamming, $\phi_J(\theta_0)$, is minimal for rigid-rod-like chains ($\theta_0 = 0$), and increases…

Soft Condensed Matter · Physics 2017-02-15 Robert S. Hoy

A Brownian dynamics algorithm is used to describe the static behaviour of associative polymer solutions. Predictions for the fractions of stickers bound by intra-chain and inter-chain association, as a function of system parameters, such as…

Soft Condensed Matter · Physics 2021-07-16 Aritra Santra , B. Dünweg , J. Ravi Prakash

Herein, we describe new methods to produce colloidal particle chains of three stiffness regimes that can be observed on a single-particle level, that is, on the level of the monomers that make up the chain; the chains can even be observed…

The emergent fluctuating hydrodynamics of a viscoelastic fluid modeled by the multiparticle collision dynamics (MPC) approach is studied. The fluid is composed of flexible, Gaussian phantom polymers, which interact by local…

Soft Condensed Matter · Physics 2020-01-29 David Toneian , Gerhard Kahl , Gerhard Gompper , Roland G. Winkler

The correlation properties of the nonaffine elastic response in strongly disordered materials are investigated using the theory of correlated random matrices and supported by numerical models. While the nonaffine displacement field itself…

Disordered Systems and Neural Networks · Physics 2026-04-09 D. A. Conyuh , D. V. Babin , I. O. Raikov , Y. M. Beltukov

The equilibrium properties of a tangent-hard-sphere polymer chain in a hard sphere monomer solvent are studied using a Born-Green-Yvon integral equation in conjunction with a two-site solvation potential. The solvation potential is…

Statistical Mechanics · Physics 2009-09-25 Mark P. Taylor , J. E. G. Lipson

We present a Bethe approximation to study lattice models of linear polymers. The approach is variational in nature and based on the cluster variation method (CVM). We focus on a model with $(i)$ a nearest neighbor attractive energy…

Statistical Mechanics · Physics 2009-10-31 Stefano Lise , Amos Maritan , Alessandro Pelizzola

We study a model of a semiflexible long chain polymer confined to a two-dimensional slit of width $w$, and interacting with the walls of the slit. The interactions with the walls are controlled by Boltzmann weights $a$ and $b$, and the…

Statistical Mechanics · Physics 2019-12-03 Nicholas R. Beaton , Leo Li , Jonathon Liu , Thomas Wong

We demonstrate a variant of the Bond Fluctuation lattice Monte Carlo model in which moves through cis conformations are forbidden. Ring polymers in this model have a conserved quantity that amounts to a topological linking number. Increased…

Soft Condensed Matter · Physics 2009-10-31 Joseph S. Plewa , Thomas A. Witten

When the local intrinsic stiffness of a polymer chain varies over a wide range, one can observe both a crossover from rigid-rod-like behavior to (almost) Gaussian random coils and a further crossover towards self-avoiding walks in good…

Soft Condensed Matter · Physics 2015-03-17 Hsiao-Ping Hsu , Wolfgang Paul , Kurt Binder