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Volatile organic compounds (VOCs) are valuable health indicators, with synthetic breath biomarkers offering rapid and disease specific diagnostics. However, their <100 ppb level exhalation requires mass spectrometry, limiting clinical…

An algorithm based on compressive sensing (CS) is proposed for synthetic aperture radar (SAR) imaging of moving targets. The received SAR echo is decomposed into the sum of basis sub-signals, which are generated by discretizing the target…

Information Theory · Computer Science 2011-04-07 Jun Wang , Gang Li , Hao Zhang , Xiqin Wang

We propose a novel femtosecond stimulated Raman spectroscopy (FSRS) technique that combines entangled photons with interference detection to select matter pathways and enhance the resolution. Following photo excitation by an actinic pump,…

Quantum Physics · Physics 2014-07-15 Konstantin E. Dorfman , Frank Schlawin , Shaul Mukamel

Coherent Raman scattering provides highly sensitive vibrational analysis through nonlinear light-matter interactions. However, its application to metal interfaces has remained challenging because the intrinsically large non-resonant…

Surface-enhanced Raman spectroscopy (SERS) sensing of DNA sequences by plasmonic nanopores could pave a way to new generation single-molecule sequencing platforms. The SERS discrimination of single DNA bases depends critically on the time…

Hyperspectral stimulated Raman scattering (SRS) microscopy is a label-free technique for biomedical and mineralogical imaging which can suffer from low signal to noise ratios. Here we demonstrate the use of an unsupervised deep learning…

An accurate treatment of electronic spectra in large systems with a technique such as time dependent density functional theory (TDDFT) is computationally challenging. Due to the Nyquist sampling theorem, direct real time simulations must be…

Materials Science · Physics 2024-01-17 Matthias Kick , Ezra Alexander , Anton Beiersdorfer , Troy Van Voorhis

Coherent Anti Stokes Raman Scattering (CARS) offers many advantages for nonlinear bio-imaging, thanks to its sub-cellular spatial resolution and unique chemical specificity. Its working principle requires two incident pulsed laser beams…

Surface-enhanced Raman scattering (SERS) provides critical insights into analyte structure, dynamic processes, and intermolecular interactions at the single-molecule level. By exploiting the hotspot formation in the vicinity of plasmonic…

Optical time-reversal techniques are being actively developed to focus light through or inside opaque scattering media. When applied to biological tissue, these techniques promise to revolutionize biophotonics by enabling deep-tissue…

Biological Physics · Physics 2016-11-07 Yuecheng Shen , Yan Liu , Cheng Ma , Lihong V. Wang

We use surface enhanced Raman spectroscopy (SERS) in studying functionalized Au nanoparticles (AuNPs) when incorporated in active-carbon (A-C) based super-capacitor cells. We observe a resonance-like enhancement in the graphitic line…

Mesoscale and Nanoscale Physics · Physics 2023-09-18 H. Grebel , Y. Zhang

We present a graphene/Cu nanoparticle hybrids (G/CuNPs) system as a surface-enhanced Raman scattering (SERS) substrate for adenosine detection. The Cu nanoparticles wrapped around a monolayer graphene shell were directly synthesized on flat…

Biological Physics · Physics 2015-03-03 Shicai Xu , Baoyuan Man , Shouzhen Jiang , Jihua Wang , Jie Wei , Shida Xu , Hanping Liu

We present super-resolved coherent anti-Stokes Raman scattering (CARS) microscopy by implementing phase-resolved image scanning microscopy (ISM), achieving up to two-fold resolution increase as compared with a conventional CARS microscope.…

Optics · Physics 2024-11-22 Anna Zhitnitsky , Elad Benjamin , Ora Bitton , Dan Oron

We have developed a coherent Raman imaging platform using broadband coherent anti-Stokes Raman scattering (BCARS) that provides an unprecedented combination of speed, sensitivity, and spectral breadth. The system utilizes a unique…

Complex 3D integration of photonic and electronic integrated circuits is of particular interest to carry the photonics roadmap and to address challenges but involves mechanical stress, often detrimental for the behavior of optical…

We introduce the soft curvature and spectroscopy (SCANS) system: a versatile, electronics-free, fluidically actuated soft manipulator capable of assessing the spectral properties of objects either in hand or through pre-touch caging. This…

Robotics · Computer Science 2025-10-03 Nathaniel Hanson , Austin Allison , Charles DiMarzio , Taşkın Padır , Kristen L. Dorsey

This study examines the Raman scattering and charge transfer properties of molecules adsorbed on the surface of a tetrahedral Au$_{120}$ nanoparticle based on the time-dependent density functional tight-binding (TD-DFTB) method. We study…

Chemical Physics · Physics 2024-09-18 Sajal Kumar Giri , George C. Schatz

Surface-enhanced Raman spectroscopy (SERS) demands reliable, high enhancement substrates in order to be used in different fields of application. Here, we introduce freestanding porous gold membranes (PAuM) as easy to produce, scalable,…

We present experimental demonstration of a recently predicted path interference phenomenon [Nanophotonics 7, 1687 (2018)]. A SERS process becomes resonant when both incident and the converted frequencies match with two plasmon resonances --…

Raman scattering is the inelastic process where photons bounce off molecules, losing energy and becoming red-shifted. This weak effect is unique to each molecular species, making it an essential tool in e.g. spectroscopy and label-free…