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We demonstrate gold coated polymer surface enhanced Raman scattering (SERS) substrates with a pair of complementary structures--positive and inverted pyramids array structures fabricated by multiple-step molding and replication process. The…

Optics · Physics 2014-02-10 Zhida Xu , Logan Liu

Spontaneous Raman spectroscopy (SRS) is a conventional in-situ laser diagnostic method that has been widely used for measurements of temperature and major species. However, SRS in sooting flames suffers from strong interference including…

Optics · Physics 2023-02-15 Hu Meng , Yihua Ren , Heinz Pitsch

Coherent Raman scattering (CRS) spectroscopy techniques have been widely developed and optimized for different applications in biomedicine and fundamental science. The most utilized CRS technique has been coherent anti-Stokes Raman…

Optics · Physics 2020-03-05 Pavel Kolesnichenko , Jonathan O. Tollerud , Jeffrey A. Davis

The scanning electron microscope (SEM) produces an image of a sample by scanning it with a focused beam of electrons. The electrons interact with the atoms in the sample, which emit secondary electrons that contain information about the…

Computer Vision and Pattern Recognition · Computer Science 2017-09-08 Shahar Tsiper , Or Dicker , Idan Kaizerman , Zeev Zohar , Mordechai Segev , Yonina C. Eldar

Time-resolved scanning near-field optical microscopy (tr-SNOM) enables the measurement of the dynamic optical response of functional surfaces beyond the diffraction limit. Experimental challenges are imposed both by the use of a pulsed…

Optics · Physics 2026-04-16 Philipp Schwendke , Julia Stähler , Samuel Palato

Surface-enhanced Raman spectroscopy (SERS) is enabled by local surface plasmon resonances (LSPRs) in metallic nanogaps. When SERS is excited by direct illumination of the nanogap, the background heating of lattice and electrons can prevent…

Mesoscale and Nanoscale Physics · Physics 2023-08-23 Shusen Liao , Yunxuan Zhu , Qian Ye , Stephen Sanders , Jiawei Yang , Alessandro Alabastri , Douglas Natelson

Accurate detection and analysis of traces of persistent organic pollutants in water is important in many areas, including environmental monitoring and food quality control, due to their long environmental stability and potential…

Machine Learning · Computer Science 2024-02-02 Vishnu Jayaprakash , Jae Bem You , Chiranjeevi Kanike , Jinfeng Liu , Christopher McCallum , Xuehua Zhang

Noble-metal-free surface-enhanced Raman scattering (SERS) substrates have attracted great attention for their abundant sources, good signal uniformity, superior biocompatibility, and high chemical stability. However, the lack of…

Applied Physics · Physics 2022-04-14 Leilei Lan , Haorun Yao , Guoqun Li , Xingce Fan , Mingze Li , Teng Qiu

Ag nanorod arrays/dielectrics/mirror-structured multilayer thin-film are well known, highly sensitive surface-enhanced Raman scattering (SERS) substrates that enhance the Raman scattering cross-section by the interference of light. However,…

Applied Physics · Physics 2020-10-08 Samir Kumar , Misa Kanagawa , Kyoko Namura , Takao Fukuoka , Motofumi Suzuki

Miniaturized photonic cavities generating nonlinear optical states of light are central to telecommunications and metrology applications. The emergence of such states is primarily underpinned by the ubiquitous Kerr nonlinearity that is…

We present a method for deriving limits on Raman scattering in structured media and exploit it to constrain the maximum Raman signal resulting from a planewave incident on either a single Raman molecule in the vicinity of a structured…

The electromagnetic enhancement for surface enhanced Raman spectroscopy (SERS) of graphene is studied by inserting a layer of Al2O3 between epitaxial graphene and Au nanoparticles. Different excitation lasers are utilized to study the…

Raman spectroscopy reveals chemically specific information and provides label-free insight into the molecular world. However, the signals are intrinsically weak and call for enhancement techniques. Here, we demonstrate Purcell enhancement…

Tip-enhanced Raman spectroscopy (TERS) is a powerful method for imaging vibrational motion and chemically characterizing surface-bound systems. Theoretical simulations of TERS images often consider systems in isolation, ignoring any…

Materials Science · Physics 2025-09-17 Krystof Brezina , Yair Litman , Mariana Rossi

Herein we report experimental evidence of directional SERS from molecules situated inside a single nanowire-nanoparticle junction cavity. The emission was confined to a narrow range of wavevectors perpendicular to the axis of the cavity. In…

Wearable sensing technology capable of point-of-care, continuous and non-invasive analysis of exosomes in biofluid such as tears and sweat is an essential part for future personalized medicine. Major detection and identification methods of…

Mesoscale and Nanoscale Physics · Physics 2026-05-26 Yang Li , Xiaoming Lyu , Ling Xia , Kuo Zhan , Haoyu Ji , Lei Qin , Seppo J. Vainio , Jian-An Huang

Single-shot terahertz (THz) spectroscopy probes sub-picosecond, non-repetitive events by combining the advantages of laser absorption techniques with the phase-sensitive detection of interferometric methods. However, its usage as a…

Optics · Physics 2025-01-07 Charan R. Nallapareddy , Thomas C. Underwood

Coherent anti-Stokes Raman scattering (CARS) and, in particular, femtosecond adaptive spectroscopic techniques (FAST CARS) have been successfully used for molecular spectroscopy and microscopic imaging. Recent progress in ultrafast…

Surface Enhanced Raman Scattering (SERS) and Surface-Enhanced Fluorescence (SEF) are studied within the framework of modified Spontaneous Emission (SE), and similarities and differences are highlighted. This description sheds new light into…

Chemical Physics · Physics 2007-05-23 E. C. Le Ru , P. G. Etchegoin

This paper presents a quadrature compressive sampling (QuadCS) and associated fast imaging scheme for synthetic aperture radar (SAR). Different from other analog-to-information conversions (AIC), QuadCS AICs using independent spreading…

Information Theory · Computer Science 2018-01-12 Huizhang Yang , Shengyao Chen , Feng Xi , Zhong Liu